Cleaning Composition for Semiconductor Post-Etch Residue Removal

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Solution Overview

Problem

Current cleaning compositions fail to effectively remove post-etch residue and titanium-containing hardmask materials from microelectronic devices with high selectivity for titanium nitride hard masks while controlling etch rates for aluminum nitride and maintaining compatibility with copper and low-k dielectric materials.

Innovation Solution

A composition comprising a tetraalkylammonium hydroxide or quaternary trialkylalkanolamine base, an oxidizer with a heterocyclic amine N-oxide, a corrosion inhibitor, and a combination of polyprotic acids or salts, including phosphorous-containing acids, which is diluted with an oxidizer to achieve high etch rate selectivity for titanium nitride hard masks, controlled etch rates for aluminum nitride, and low etch rates for copper and cobalt, while being compatible with low-k dielectric materials.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional cleaning compositions are used, then post-etch residue removal is achieved, but selectivity for titanium nitride hard masks is insufficient and etch rates for aluminum nitride and copper are not controlled

Engineering Contradiction:
Improveetch rate selectivityVSAvoidcompatibility with multiple materials
Core Design Contradiction:
Manufacturing precisionVSReliability

Solution Approach 1:

The patent modifies the chemical composition parameters by incorporating specific bases (tetraalkylammonium hydroxide or quaternary trialkylalkanolamine), oxidizers (heterocyclic amine N-oxide), corrosion inhibitors, and polyprotic acids with phosphorous. These parameter changes enable differentiated etch rates: high for titanium nitride hard masks, controlled low for aluminum nitride, and low for copper and cobalt, while maintaining compatibility with low-k dielectric materials.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The cleaning composition is formulated as a composite chemical system combining multiple functional components: a specific base, oxidizer, corrosion inhibitor, and polyprotic acid mixture. This composite approach allows the composition to simultaneously achieve high etch rate selectivity for titanium nitride while controlling etch rates for aluminum nitride, copper, and cobalt, and maintaining compatibility with low-k dielectrics.

Inventive Principle:
Principle #40Composite materials

2Productivity

If high etch rate for titanium nitride hard mask is achieved, then hard mask removal efficiency is improved, but etch rates for aluminum nitride and copper may increase uncontrollably

Engineering Contradiction:
Improvehard mask removal efficiencyVSAvoidetch rate control
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The cleaning composition exhibits local quality by differentiating its etching action across different materials. It achieves high etch rate locally for titanium nitride hard masks (improving productivity) while simultaneously maintaining controlled low etch rates for aluminum nitride, copper, and cobalt (ensuring manufacturing precision). This selective action is achieved through the specific combination of base, oxidizer, corrosion inhibitor, and polyprotic acids.

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composition achieves a high etch rate for titanium nitride hard masks, low etch rates for aluminum nitride and cobalt, and compatibility with low-k dielectric materials, ensuring efficient removal of post-etch residues and titanium-containing hardmask materials with controlled etching.

Implementation Method 1

a tetraalkylammonium hydroxide or quaternary trialkylalkanolamine base

Methodology Applied
Scientific EffectChemical etching: Chemical Bonding

Implementation Method 2

an oxidizer with a heterocyclic amine N-oxide

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 3

a corrosion inhibitor

Methodology Applied
Scientific EffectCorrosion inhibition:

Implementation Method 4

a combination of polyprotic acids or salts, including phosphorous-containing acids

Methodology Applied
Scientific EffectChelation:

Data Source

PatentUS10577567B2Cleaning compositions for removing post etch residue
Publication Date: 2020.03.03 ENTEGRIS INC

AI summary

The disclosure relates to a cleaning composition that aids in the removal of post-etch residues in the production of semiconductors. There is provided a stock composition comprising: a tetraalkylammonium hydroxide base or a quaternary trialkylalkanolamine base; a corrosion inhibitor; and a combination of at least two or more polyprotic acids or salts thereof, wherein at least one said polyprotic acid or salt thereof contains phosphorous.