Separator Active-Layer Amine Quantification Using EDS Depth Profiles

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Solution Overview

Problem

Existing methods fail to accurately measure the amount of monomer present on the ultrafiltration layer surface, which affects the performance of the reverse osmosis membrane's active layer, as they rely on total weight differences post-coating, lacking surface reaction area analysis.

Innovation Solution

A method using energy dispersive spectrometry (EDS) to analyze the distribution of amine compounds by depth on a support layer, employing multiple line scans to quantify the amine compound accurately, allowing for better prediction of membrane performance.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If total weight difference method is used to estimate monomer amount, then measurement process is simple, but measurement precision is insufficient to predict reverse osmosis layer formation

Engineering Contradiction:
Improvesimplicity of measurement processVSAvoidaccuracy of monomer amount measurement
Core Design Contradiction:
Ease of manufactureVSMeasurement precision

Solution Approach 1:

The patent replaces the mechanical weighing method with X-ray photoelectron spectroscopy (XPS), an optical/electromagnetic measurement technique. XPS directly measures the chemical composition and concentration of elements on the ultrafiltration layer surface, providing precise quantification of amine compound distribution without relying on indirect weight differences.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Solution Approach 2:

The patent introduces XPS as an intermediary measurement tool that bridges the gap between simple measurement and accurate prediction. XPS serves as a mediator that provides detailed surface chemical information, enabling accurate determination of amine compound concentration and distribution, which then allows reliable prediction of reverse osmosis layer formation.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Loss of time

If conventional measurement methods are used, then measurement time is short, but information on monomer distribution in reaction area is not obtained

Engineering Contradiction:
Improvemeasurement timeVSAvoidsurface reaction area analysis
Core Design Contradiction:
Loss of timeVSLoss of information

Solution Approach 1:

The patent transitions from one-dimensional bulk weight measurement to two-dimensional surface spatial distribution analysis. XPS provides not only the total amount of amine compounds but also their spatial distribution across the ultrafiltration layer surface, revealing heterogeneous distribution patterns and identifying specific reaction areas with high or low monomer concentration.

Inventive Principle:
Principle #17Another dimension (Dimensionality change)

3Measurement precision

If accurate surface monomer quantification is achieved through XPS, then prediction of reverse osmosis layer formation is improved, but device complexity increases

Engineering Contradiction:
Improvesurface monomer quantification accuracyVSAvoidcomplexity of analysis equipment
Core Design Contradiction:
Measurement precisionVSDevice complexity

Solution Approach 1:

The patent employs XPS, which is an established and self-contained analytical technique with automated data processing capabilities. The instrument performs both quantitative analysis and spatial distribution mapping through its inherent spectral analysis functions, reducing the need for additional auxiliary equipment or complex manual processing procedures.

Inventive Principle:
Principle #25Self-service

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The EDS method provides clear distribution profiles of nitrogen atoms, enabling precise determination of amine compound dispersion and amount, thereby optimizing membrane manufacturing conditions for improved performance.

Implementation Method 1

analyzing distribution of the amine compound by depth from the coated surface on the support using an energy dispersive spectrometer (EDS) method

Methodology Applied
Scientific EffectEnergy dispersive spectroscopy (EDS): X-Ray

Data Source

PatentEP3709009B1Method for quantifying amine compound constituting separator active layer prior to preparation of separator active layer, method for quantifying polyamide or unreacted amine compound in separator active layer, and method for setting preparation conditions of separator active layer or establishment standards for preparation conditions of separator active layer
Publication Date: 2025.10.15 LG CHEM LTD
  • EP3709009B1 patent drawingFigure 1~2
  • EP3709009B1 patent drawingFigure 3~4
  • EP3709009B1 patent drawingFigure 5

AI summary

The present specification relates to a method for quantifying an amine compound forming a membrane active layer before preparing the membrane active layer, a method for quantifying polyamide or an unreacted amine compound in a membrane active layer, and method for determining setting criteria for a manufacturing condition of a membrane active layer or a method for setting a manufacturing condition.