Separator Coating Slurry for Battery Safety

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Solution Overview

Problem

Commercial polyolefin-based separators for electrochemical devices have poor wetting characteristics, adhesive properties, and low melting temperatures, leading to low electrolyte uptake, poor conductivity, and mechanical instability, particularly at high temperatures, which affects the performance and safety of electrochemical devices.

Innovation Solution

A coating slurry comprising a polymer with an intrinsic viscosity ranging from 0.5 to 3.0 mL/g, an inorganic filler, and a solvent is applied to a porous base membrane, forming a coating layer that enhances adhesion, heat resistance, and porosity, thereby improving the mechanical strength and cycle life of the separator.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If a polyolefin-based separator is used, then cost is reduced and chemical stability is improved, but wetting characteristics deteriorate and adhesive property deteriorates

Engineering Contradiction:
ImprovecostVSAvoidwetting characteristics
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent applies composite materials by forming a coating layer comprising both adhesive polymer and inorganic particles on the polyolefin microporous membrane. This composite structure combines the cost advantages and chemical stability of polyolefin with the improved wetting and adhesion properties of the coating layer, resolving the contradiction between low cost and poor wetting characteristics.

Inventive Principle:
Principle #40Composite materials

2Stability of the object's composition

If a polyolefin-based separator is used, then chemical stability is improved, but adhesive property deteriorates

Engineering Contradiction:
Improvechemical stabilityVSAvoidadhesive property
Core Design Contradiction:
Stability of the object's compositionVSStrength

Solution Approach 1:

The patent segments the separator into two functional parts: a polyolefin microporous membrane base layer that provides chemical stability, and a separate coating layer comprising adhesive polymer and inorganic particles that provides adhesive property. This segmentation allows each layer to independently fulfill its specific function without compromising the other.

Inventive Principle:
Principle #1Segmentation

3Ease of manufacture

If a polyolefin-based separator is used, then low cost is achieved, but melting temperature is reduced

Engineering Contradiction:
Improvelow costVSAvoidmelting temperature
Core Design Contradiction:
Ease of manufactureVSTemperature

Solution Approach 1:

The patent applies local quality by creating a coating layer with different thermal properties on the polyolefin membrane surface. The coating layer comprising adhesive polymer and inorganic particles provides localized high-temperature stability at the critical interface regions, while the bulk polyolefin membrane maintains its cost advantage and inherent chemical stability.

Inventive Principle:
Principle #3Local quality

4Strength

If a coating layer is formed on polyolefin membrane, then adhesive property is improved, but device complexity increases

Engineering Contradiction:
Improveadhesive propertyVSAvoidstructure complexity
Core Design Contradiction:
StrengthVSDevice complexity

Solution Approach 1:

The patent uses porous materials by forming a porous coating layer comprising adhesive polymer and inorganic particles on the microporous polyolefin membrane. The porous structure of the coating layer maintains compatibility with the electrolyte and facilitates ion transport while providing the necessary adhesive property, achieving functional improvement without excessive structural complexity.

Inventive Principle:
Principle #31Porous materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The coated separator exhibits improved adhesive properties, mechanical strength, and cycle performance, ensuring low internal resistance and enhanced safety for electrochemical devices, particularly in high-energy density and high-power density applications.

Implementation Method 1

removing the at least one solvent from the wet coating layer to form a coating layer

Methodology Applied
Scientific EffectEvaporation: Evaporation

Data Source

PatentUS11158905B2Coating slurries for preparing separators, separators for electrochemical devices and preparation methods therefor
Publication Date: 2021.10.26 SHANGHAI ENERGY NEW MATERIALS TECHNOLOGY CO LTD

AI summary

Disclosed are a coating slurry for preparing a separator for an electrochemical device, comprising at least one polymer having an intrinsic viscosity ranging from 0.5 to 3.0 mL/g, at least one inorganic filler, and at least one solvent; a method for preparing the coating slurry; and a method for preparing a separator for an electrochemical device using the coating slurry; as well as a separator and an electrochemical device comprising the separator.