Battery Separator Resin Composition for Viscosity and Thickness Control

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Solution Overview

Problem

Conventional resin compositions for separators in batteries face challenges in controlling viscosity and thickness, leading to issues like reduced hydrogen ion conductivity and durability, and the remnants of additives affecting battery performance after drying.

Innovation Solution

A resin composition comprising a sulfonated polymer, an amide group-containing organic solvent, and water, with specific weight ratios and amounts, allowing for controlled viscosity and thickness of the separator without residual additives post-drying, using a method that involves mixing the sulfonated polymer with water and adding the amide solvent, followed by shaping and heat treatment to remove the solvent.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If the thickness of separator is increased to reduce vanadium ion permeation, then crossover phenomenon is suppressed, but hydrogen ion conductivity and durability are reduced

Engineering Contradiction:
Improvecrossover preventionVSAvoidhydrogen ion conductivity
Core Design Contradiction:
ReliabilityVSStrength

Solution Approach 1:

The patent changes the chemical composition parameters of the separator by incorporating specific sulfonated polymers with controlled sulfonate content (5-20 mmol/g) and using specific solvent systems (N,N-dimethylacetamide with water). This allows optimization of the membrane's ion transport properties to achieve both low vanadium permeation and high hydrogen ion conductivity without increasing thickness

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite separator structure by combining sulfonated polymers (such as sulfonated polyether ether ketone or sulfonated polyarylene) with specific additives and solvents. This composite approach enables the separator to simultaneously exhibit low vanadium ion permeability and high hydrogen ion conductivity through synergistic material interactions

Inventive Principle:
Principle #40Composite materials

2Ease of manufacture

If conventional resin compositions are used for separator fabrication, then manufacturing is simplified, but additive residues remain after drying and affect battery performance

Engineering Contradiction:
Improvefabrication simplicityVSAvoidadditive residues
Core Design Contradiction:
Ease of manufactureVSObject-generated harmful factors

Solution Approach 1:

The patent removes harmful additive residues from the separator fabrication process by using a minimal-component resin composition consisting only of sulfonated polymer, N,N-dimethylacetamide, and water. The amide solvent and water completely evaporate during drying, leaving no residual additives that could contaminate the battery

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent employs volatile solvents (N,N-dimethylacetamide and water) that serve their purpose during fabrication and then completely evaporate without residue. These short-living solvent molecules fulfill their function of enabling polymer processing and then disappear, leaving a clean separator without persistent harmful residues

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Manufacturing precision

If viscosity control agents are added to resin composition to control separator thickness, then thickness uniformity is improved, but conductivity and durability are reduced due to remaining additives

Engineering Contradiction:
Improvethickness controlVSAvoidconductivity and durability
Core Design Contradiction:
Manufacturing precisionVSReliability

Solution Approach 1:

The patent employs the N,N-dimethylacetamide solvent itself to provide the necessary viscosity control for the resin composition without requiring additional thickening agents. The solvent's inherent properties and its interaction with the sulfonated polymer enable controlled film formation and uniform thickness, while the solvent completely evaporates afterward, leaving no residual additives to compromise conductivity or durability

Inventive Principle:
Principle #25Self-service

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composition effectively enhances and controls viscosity, ensuring a separator with optimal thickness and performance, preventing additive residues that could impair battery efficiency, thereby improving battery capacity and efficiency.

Implementation Method 1

a resin composition for fabricating a separator comprising: a sulfonated polymer, an amide group-containing organic solvent, and water

Methodology Applied
Scientific EffectSolvation: Solvation

Implementation Method 2

heating to 70 to 220 °C to remove the amide group-containing organic solvent

Methodology Applied
Scientific EffectEvaporation: Evaporation

Data Source

PatentEP3689949B1Resin composition for manufacturing separator, preparation method therefor, and battery comprising same
Publication Date: 2023.12.06 LG CHEM LTD
  • EP3689949B1 patent drawingFigure 1

AI summary

The present invention relates to a resin composition for fabricating a separator which is easy to control viscosity, a method of preparing the same, and a battery comprising the same.