A sheet-like article and a production method thereof

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Solution Overview

Problem

Existing methods for producing sheet-like articles using water-dispersed polyurethane result in stiff textures due to differences in coagulation techniques compared to organic solvent-based methods, lacking the softness and flexibility of products made with organic solvents.

Innovation Solution

A sheet-like article produced using a fibrous base material with ultrafine fibers and a polymer elastomer having a hydrophilic group, where the polymer elastomer forms a crosslinked structure, and the production process involves adding an aqueous resin dispersion liquid with a viscosity improver and coagulating in hot water to create a porous structure.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Object-affected harmful factors

If water-dispersed polyurethane is used instead of organic solvent-based polyurethane, then environmental harm is reduced, but the texture becomes stiff

Engineering Contradiction:
Improveenvironmental harmVSAvoidtexture softness
Core Design Contradiction:
Object-affected harmful factorsVSEase of operation

Solution Approach 1:

The invention changes the coagulation parameters by controlling temperature (90-100°C) and time (5-30 minutes) to achieve a porous polyurethane structure that maintains softness while using environmentally friendly water-dispersed polyurethane

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention creates a porous structure in the polyurethane film through controlled coagulation, which reduces fiber entanglement contact area and prevents stiff texture, while maintaining the environmental benefits of water-based dispersion

Inventive Principle:
Principle #31Porous materials

2Reliability

If wet heat coagulation technique is used for water-dispersed polyurethane, then coagulation is achieved, but the texture becomes stiff due to high-density nonporous film structure

Engineering Contradiction:
Improvecoagulation effectivenessVSAvoidtexture softness
Core Design Contradiction:
ReliabilityVSEase of operation

Solution Approach 1:

The invention modifies the wet heat coagulation parameters by using higher temperatures (90-100°C) and extended times (5-30 minutes) to create a porous structure rather than a dense nonporous structure, achieving both effective coagulation and soft texture

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention intentionally creates a porous structure within the polyurethane film during coagulation, which reduces the contact area between fibers and polyurethane, thereby preventing strong entanglement and stiff texture while maintaining coagulation effectiveness

Inventive Principle:
Principle #31Porous materials

3Ease of operation

If foaming agent is added to create porous structure, then texture softness is improved, but manufacturing complexity increases

Engineering Contradiction:
Improvetexture softnessVSAvoidmanufacturing process complexity
Core Design Contradiction:
Ease of operationVSDevice complexity

Solution Approach 1:

The invention removes the foaming agent from the process, achieving porous structure formation through controlled coagulation parameters alone, thereby simplifying the manufacturing process while maintaining texture softness

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The invention uses temperature and time as intermediaries to control the coagulation process, allowing porous structure formation without adding foaming agents or other complex additives

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method achieves a sheet-like article with fold and crease recoverability and flexibility comparable to those made with organic solvent-based polyurethane, offering a uniform feel and elegant surface quality without the use of organic solvents.

Implementation Method 1

the method involving the coagulation of a polyurethane solution in an organic solvent uses the so-called wet coagulation technique in which polyurethane molecules dissolved in an organic solvent are coagulated by substituting water for solvent

Methodology Applied
Scientific EffectCoagulation: Coagulation

Implementation Method 2

For coagulation of water-dispersed polyurethane, on the other hand, the wet heat coagulation technique is mainly used, in which heating is performed to destroy the hydrated state of the dispersion liquid of water-dispersed polyurethane to cause the aggregation of emulsion particles of polyurethane to achieve coagulation

Methodology Applied
Scientific EffectWet heat coagulation:

Implementation Method 3

the production process involves adding an aqueous resin dispersion liquid with a viscosity improver and coagulating in hot water to create a porous structure

Methodology Applied
Scientific EffectHeating: Heating

Data Source

PatentEP3112530B1A sheet-like article and a production method thereof
Publication Date: 2023.11.22 TORAY INDUSTRIES INC
  • EP3112530B1 patent drawingFigure 1
  • EP3112530B1 patent drawingFigure 2
  • EP3112530B1 patent drawingFigure 3

AI summary

The invention relates to an environmentally friendly production method for a sheet-like article that does not use an organic solvent in the production process and provides a sheet-like article that compares favorably in terms of a uniform feel with artificial leather products produced from an organic solvent based polyurethane and in particular has good surface quality and texture and also provides a production method therefor. The present invention aims to provide a sheet-like article comprising a fibrous base material formed of ultrafine fibers and/or ultrafine fiber bundles provided with, as a binder, a polymer elastomer having a hydrophilic group, any thickness-directional cross section of the sheet-like article containing regions occupied by the polymer elastomer, the regions including independent regions each with a cross-sectional area of 50 µm2 or more, the total area of the independent regions accounting for 0.1% or more and 5.0% or less of the cross-sectional area of the artificial leather in an observation view field. The production method for the sheet-like article according to the present invention provides a production process for a sheet-like article including a fibrous base material formed of ultrafine fibers and, as a binder, a polymer elastomer having a hydrophilic group, the process including a step for adding an aqueous resin dispersion liquid containing a water-dispersed polymer elastomer and a viscosity improver to a fibrous base material and a step for coagulating the polymer elastomer in hot water at a temperature of 50°C to 100°C.