Shell Catalyst for Acrolein Oxidation with Mo-V-W Composition

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Solution Overview

Problem

Existing catalysts used in the heterogeneously catalyzed partial gas phase oxidation of acrolein to acrylic acid suffer from deactivation over time, leading to reduced activity and increased operating costs due to the need for frequent replacement or temperature adjustments, which complicates the process and increases costs.

Innovation Solution

A shell catalyst comprising a support body with a finely divided multi-element oxide containing Mo and V, combined with a finely divided molybdenum oxide substance that forms under elevated temperature and molecular oxygen, is applied to the support body using a binder, effectively delaying deactivation and maintaining catalytic effectiveness.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If the temperature of the fixed catalyst bed is gradually increased to compensate for activity reduction, then the acrolein conversion is maintained, but the aging process of the catalyst accelerates

Engineering Contradiction:
Improveacrolein conversionVSAvoidcatalyst service life
Core Design Contradiction:
ReliabilityVSDuration of action of stationary object

Solution Approach 1:

The patent applies parameter changes by modifying the chemical composition of the catalyst (changing from conventional Mo-V oxides to Mo-V-W oxides with specific molar ratios) to maintain catalytic activity without requiring temperature increases, thereby extending catalyst service life while maintaining reliability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses composite materials by combining multiple metal oxides (Mo, V, W) in specific proportions to create a catalyst with enhanced stability and resistance to aging, allowing the catalyst to maintain activity over longer periods without temperature compensation

Inventive Principle:
Principle #40Composite materials

2Reliability

If the fixed catalyst bed is completely replaced to restore activity, then the catalytic performance is renewed, but the production process is interrupted and costs increase

Engineering Contradiction:
Improvecatalyst activityVSAvoidproduction interruption time
Core Design Contradiction:
ReliabilityVSLoss of time

Solution Approach 1:

The patent applies preliminary action by pre-optimizing the catalyst composition with specific Mo-V-W ratios and particle size distributions that inherently resist deactivation, allowing the catalyst to maintain activity for extended periods without requiring replacement, thus avoiding production interruptions

Inventive Principle:
Principle #10Preliminary action

3Loss of time

If only a portion of the fixed catalyst bed is replaced instead of complete replacement, then the production interruption is reduced, but the process complexity increases

Engineering Contradiction:
Improveproduction interruption timeVSAvoidcatalyst replacement process complexity
Core Design Contradiction:
Loss of timeVSDevice complexity

Solution Approach 1:

The patent applies preliminary action by designing a catalyst with optimized composition and structure that maintains high activity over extended periods, eliminating the need for partial replacement operations and their associated complexity

Inventive Principle:
Principle #10Preliminary action

4Reliability

If the working pressure is increased to counteract catalyst deactivation, then the catalytic activity is maintained, but the compression performance requirement increases

Engineering Contradiction:
Improvecatalyst activityVSAvoidworking pressure
Core Design Contradiction:
ReliabilityVSStress or pressure

Solution Approach 1:

The patent applies parameter changes by modifying the catalyst's chemical composition (Mo-V-W oxide ratios) and physical structure (particle size) to maintain activity without requiring pressure increases, thereby avoiding additional compression requirements

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The shell catalyst significantly extends the service life of the catalyst bed by maintaining high acrolein conversion rates and reducing the need for frequent replacements or temperature adjustments, thereby improving process efficiency and reducing operational costs.

Implementation Method 1

catalysts are particularly suitable for catalyzing the heterogeneously catalyzed partial gas phase oxidation of acrolein to acrylic acid

Methodology Applied
Scientific EffectHeterogeneous catalysis: Catalysis

Implementation Method 2

the active mass is adhered to the surface of the carrier body with the aid of a binder

Methodology Applied
Scientific EffectAdhesion: Adhesive

Data Source

PatentEP2134465B1Method for producing a catalyst consisting of a carrier body and a catalytically active mass applied to the surface of the carrier body
Publication Date: 2018.06.13 BASF SE
  • EP2134465B1 patent drawingFigure 1
  • EP2134465B1 patent drawingFigure 2
  • EP2134465B1 patent drawingFigure 3

AI summary

The invention relates to a method for producing a shell catalyst, according to which a fine-particle mixture consisting of a multi-element oxide containing the elements Mo and V, and a molybdenum oxide or a molybdenum oxide forming agent, is applied to the surface of a carrier body as an active substance.