SiAlON Phosphor Radiation Detector High-Temperature Stability

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Solution Overview

Problem

Current scintillator materials like ZnS:Ag,Cu are not suitable for high-temperature environments and suffer significant degradation under high-density radiation, leading to inaccurate dose measurements and frequent replacements in radiation measurement equipment used in nuclear power facilities and accelerator facilities.

Innovation Solution

A charged particle radiation measuring method and device utilizing a β-type SiAlON phosphor with the general formula Eu x Si 6-z Al z O z N 8-z, where 0.01 ≤ x ≤ 0.5 and 0 < z ≤ 4.2, which maintains luminescence efficiency even at high temperatures and under high-density radiation, combined with an optical component and a measuring portion to collect and read radiation-induced light.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Illumination intensity

If ZnS:Ag,Cu scintillator materials are used for radiation measurement, then luminous efficiency is improved, but the materials cannot withstand high-temperature environments (100°C or higher)

Engineering Contradiction:
Improveluminous efficiencyVSAvoidoperating temperature range
Core Design Contradiction:
Illumination intensityVSTemperature

Solution Approach 1:

The patent changes the material composition parameters by doping Sr2Si5N8:Eu with Al and O to create Sr2-zAlzSi5-zOzN8-x:Eu phosphor, which enables the scintillator to maintain stable luminescence properties at high temperatures up to 500°C while preserving luminous efficiency

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite phosphor material combining Sr2Si5N8 host lattice with Eu activator and Al/O dopants, forming a new composite scintillator material that simultaneously achieves high-temperature stability and maintained luminous efficiency

Inventive Principle:
Principle #40Composite materials

2Illumination intensity

If ZnS:Ag,Cu scintillator materials are used for radiation measurement, then initial luminous intensity is achieved, but luminous intensity degrades significantly under high-density radiation

Engineering Contradiction:
Improveluminous intensityVSAvoidradiation resistance
Core Design Contradiction:
Illumination intensityVSReliability

Solution Approach 1:

The patent modifies the material composition by introducing Al and O dopants into the Sr2Si5N8:Eu phosphor structure, which changes the crystal lattice parameters and electronic structure to resist radiation-induced damage, maintaining stable luminescence under high-density charged particle irradiation

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent replaces the short-lived ZnS:Ag,Cu scintillator material that degrades under radiation with a more stable Sr2-zAlzSi5-zOzN8-x:Eu phosphor that maintains reliability over extended periods under high-density radiation conditions

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Measurement precision

If existing scintillator materials are used in high-temperature environments, then initial measurements can be taken, but measurement precision deteriorates over time

Engineering Contradiction:
Improvedose measurement precisionVSAvoidmeasurement duration
Core Design Contradiction:
Measurement precisionVSDuration of action of stationary object

Solution Approach 1:

The patent changes the thermal stability parameters of the scintillator material by using Sr2-zAlzSi5-zOzN8-x:Eu phosphor with optimized doping concentrations, which maintains consistent luminescence response over extended periods at high temperatures, ensuring long-term measurement precision

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent provides more than sufficient thermal stability by designing the phosphor to remain stable up to 500°C, which far exceeds the 100°C operational requirement, ensuring measurement precision is maintained throughout the intended measurement duration

Inventive Principle:
Principle #16Partial or excessive action

4Measurement precision

If ZnS:Ag,Cu scintillator materials are used in accelerator facilities, then initial beam quality measurement is achieved, but work efficiency decreases due to frequent replacement

Engineering Contradiction:
Improvebeam quality measurementVSAvoidoperating efficiency
Core Design Contradiction:
Measurement precisionVSProductivity

Solution Approach 1:

The patent replaces the frequently degrading ZnS:Ag,Cu scintillator with a durable Sr2-zAlzSi5-zOzN8-x:Eu phosphor that resists high-density radiation damage, eliminating the need for frequent replacements and maintaining continuous operating efficiency in accelerator facilities

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent performs preliminary material design and optimization to create a radiation-resistant phosphor before deployment, ensuring the scintillator can withstand the full operational lifetime in accelerator facilities without requiring replacement, thus maintaining productivity

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method provides highly heat-resistant and radiation-resistant radiation measuring equipment capable of precise measurements over extended periods, even in high-temperature environments, with sustained luminescence intensity and prolonged equipment lifespan.

Implementation Method 1

scintillators are substances that generate light when radiation impinges thereon

Methodology Applied
Scientific EffectLuminescence: Luminescence

Implementation Method 2

an optical component that selectively collects light from the scintillator

Methodology Applied
Scientific EffectLight collection: Reflection

Implementation Method 3

a measuring portion that reads out light generated by radiation

Methodology Applied
Scientific EffectLight detection: Photoelectric Effect

Data Source

PatentEP3343248B1Charged particle radiation measuring method and charged particle radiation measuring device
Publication Date: 2020.02.26 NAT INST FOR QUANTUM & RADIOLOGICAL SCI & TECH
  • EP3343248B1 patent drawingFigure 1
  • EP3343248B1 patent drawingFigure 2~3
  • EP3343248B1 patent drawingFigure 4

AI summary

[Problem] To provide highly heat-resistant and radiation-resistant radiation measuring equipment. [Solution] Provided are a charged particle radiation measuring method and a charged particle radiation measuring device using a scintillator comprising a phosphor in which the main component is a SiAlON phosphor.