Silane Production in Baffled Bubble Column Reactor

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Solution Overview

Problem

Current methods for producing silane are economically challenged due to high starting material costs and require improvements in reactor productivity and conversion efficiency.

Innovation Solution

A process involving a reaction vessel with baffles creating multiple zones, where a halosilane and a hydride react to produce silane, with the reaction mixture being agitated and the upper zone cooled, allowing for counter-current flow of reactants and products to enhance conversion without direct measurement of concentrations, using a baffle-defined lower and upper reaction zone.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If a single reaction zone is used, then the reactor structure is simple, but conversion efficiency and productivity are limited

Engineering Contradiction:
Improvereactor productivityVSAvoidreactor structure
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The reaction vessel is divided into multiple reaction zones (first, second, and third zones) separated by baffles, allowing the reaction process to occur in stages. This segmentation enables improved conversion efficiency and productivity while maintaining a relatively simple overall structure using standard baffle components.

Inventive Principle:
Principle #1Segmentation

2Productivity

If high conversion efficiency is achieved through complex temperature control, then reactant conversion improves, but system complexity and cost increase

Engineering Contradiction:
Improveconversion efficiencyVSAvoidtemperature control system
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

Different temperature conditions are applied to different reaction zones: the first zone operates at a first temperature, the second zone at a second temperature, and the third zone at a third temperature. This local differentiation of temperature conditions optimizes conversion efficiency in each zone without requiring a complex centralized control system.

Inventive Principle:
Principle #3Local quality

3Ease of manufacture

If starting material costs are reduced, then production cost decreases, but conversion efficiency may be affected

Engineering Contradiction:
Improveproduction costVSAvoidconversion efficiency
Core Design Contradiction:
Ease of manufactureVSProductivity

Solution Approach 1:

The process utilizes specific parameter ranges including temperature (20-100°C), pressure (1-10 atm), and reaction time (1-24 hours) to optimize the reaction between silicon tetrafluoride and aluminum tetrahydride. These parameter optimizations enable high conversion efficiency with cost-effective starting materials.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method increases conversion efficiency of reactants, reduces costs by optimizing temperature control and flow rates, and produces high-purity silane with minimal need for specialized personnel or equipment for concentration measurements.

Implementation Method 1

A feed gas comprising a halosilane is introduced into the reaction vessel to bubble the feed gas through the reaction mixture

Methodology Applied
Scientific EffectBubbling: Bubble

Implementation Method 2

the upper reaction zone being cooled

Methodology Applied
Scientific EffectCooling: Cooling

Implementation Method 3

The reaction mixture is agitated

Methodology Applied
Scientific EffectAgitation: Stirring

Implementation Method 4

The hydride reacts with the halosilane to produce silane and a halide salt

Methodology Applied
Scientific EffectChemical reaction: Chemical Bonding

Data Source

PatentEP2726410B1Processes for producing silane in a bubble column
Publication Date: 2016.05.11 SUNEDISON INC
  • EP2726410B1 patent drawingFigure 1
  • EP2726410B1 patent drawingFigure 2
  • EP2726410B1 patent drawingFigure 3

AI summary

Methods for producing silane by reacting a hydride and a halosilane are disclosed. Some embodiments involve use of a column which is not mechanically agitated and in which reactants may be introduced in a counter-current arrangement. Some embodiments involve use of a baffled column which has multiple reaction zones.