Silicate-Chlorophyll Complex Precipitation for Protein Separation

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Solution Overview

Problem

Current methods for separating chlorophyll and soluble proteins, such as rubisco, from plant extracts are inefficient, often resulting in green-tasting products, high protein losses, and economic burdens due to harsh processing conditions that denature proteins and fail to achieve high yields and purity.

Innovation Solution

A method involving the addition of water-soluble silicates to an aqueous solution to form insoluble silicate-chlorophyll complexes, allowing for the separation of soluble proteins while maintaining their bioactivity, using pH adjustments within specific ranges to optimize the precipitation process.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional protein extraction methods are used, then proteins can be obtained from plant extracts, but the products become green-tasting and have poor quality due to inadequate chlorophyll removal

Engineering Contradiction:
Improveproduct qualityVSAvoidgreen color and taste
Core Design Contradiction:
Manufacturing precisionVSObject-generated harmful factors

Solution Approach 1:

The patent extracts and removes chlorophyll from the protein solution by forming insoluble silicate-chlorophyll complexes that precipitate out, separating the harmful green pigment from the desired protein product to achieve colorless, high-quality protein

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

Silicates act as an intermediary substance that selectively binds to chlorophyll molecules, forming insoluble complexes that can be removed from the solution without affecting the soluble proteins, thus enabling indirect separation of chlorophyll from proteins

Inventive Principle:
Principle #24Intermediary (Mediator)

2Manufacturing precision

If harsh processing conditions are applied to separate chlorophyll and proteins, then separation may be achieved, but proteins are denatured and losses increase

Engineering Contradiction:
Improveseparation efficiencyVSAvoidprotein bioactivity
Core Design Contradiction:
Manufacturing precisionVSReliability

Solution Approach 1:

The patent changes the chemical parameters of the solution by adjusting pH to specific ranges (pH 6-11) and adding silicates at controlled concentrations, creating conditions where chlorophyll selectively precipitates while proteins remain soluble and active, avoiding denaturation

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

Silicates serve as a gentle intermediary that enables separation through selective complex formation rather than harsh physical or chemical treatment, maintaining protein structure and function while achieving effective chlorophyll removal

Inventive Principle:
Principle #24Intermediary (Mediator)

3Object-generated harmful factors

If conventional separation methods are used, then some chlorophyll removal is achieved, but protein losses are high and yields are low

Engineering Contradiction:
Improvechlorophyll removalVSAvoidprotein loss
Core Design Contradiction:
Object-generated harmful factorsVSLoss of substance

Solution Approach 1:

Silicates act as a selective intermediary that binds specifically to chlorophyll molecules, forming insoluble complexes that precipitate and can be removed without co-precipitating proteins, thus achieving high chlorophyll removal with minimal protein loss

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent creates local chemical conditions (specific pH ranges, silicate concentrations) that are optimal for chlorophyll-silicate complex formation while maintaining protein solubility, enabling selective removal of chlorophyll without affecting protein integrity or yield

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method effectively separates chlorophyll and proteins into enriched fractions, retaining protein solubility and bioactivity, and can be scaled for commercial viability with reduced environmental impact and improved product quality.

Implementation Method 1

adding a water-soluble silicate to the solution of step a) such that the total concentration of silicon in the form of free or complexed silicates in the solution is in the range of 1-500 mM... allowing the silicate to form an insoluble precipitate comprising silicate-chlorophyll complexes

Methodology Applied
Scientific EffectPrecipitation: Precipitation

Data Source

PatentEP3849995B1Methods for separation of chlorophyll and soluble proteins
Publication Date: 2022.11.09 LIHME PROTEIN SOLUTIONS APS
  • EP3849995B1 patent drawingFigure 1
  • EP3849995B1 patent drawingFigure 2

AI summary

A method is provided for separating soluble proteins from chlorophyll using a water-soluble silicate. Various purified products and intermediates are also provided.