Silicon Dioxide Wet Etch Composition Selectivity

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Solution Overview

Problem

Conventional wet etchants for silicon dioxide, such as BOE, face issues with Solid Phase Segregation of ammonium fluoride, leading to stability and contamination problems, limiting the etch selectivity to silicon nitride films, and reducing productivity in semiconductor processing.

Innovation Solution

A composition comprising 1 to 40 wt % hydrogen fluoride, 5 to 40 wt % ammonium hydrogen fluoride, water, and optional anionic surfactants and silicon dioxide etching accelerators, which achieves an etch selectivity of 150 or higher for silicon dioxide to silicon nitride films and an etch rate of 10000 Å/min or higher, addressing the limitations of conventional etchants.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Speed

If the concentration of hydrogen fluoride and ammonium fluoride is increased to improve etch rate, then the etch rate of silicon dioxide increases, but Solid Phase Segregation of ammonium fluoride occurs causing stability and contamination problems

Engineering Contradiction:
Improveetch rateVSAvoidstability
Core Design Contradiction:
SpeedVSReliability

Solution Approach 1:

The patent changes the chemical composition parameters by replacing conventional ammonium fluoride with ammonium hydrogen fluoride and adjusting the HF concentration range (5-40 wt%), achieving both high etch rate and stability without Solid Phase Segregation

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite etchant system combining hydrogen fluoride (5-40 wt%) and ammonium hydrogen fluoride (40-80 wt%) with specific concentration ratios, achieving synergistic effects that resolve the contradiction between etch rate and stability

Inventive Principle:
Principle #40Composite materials

2Speed

If the concentration of hydrogen fluoride and ammonium fluoride is increased to improve etch rate, then the etch rate of silicon dioxide increases, but the etch selectivity to silicon nitride film decreases

Engineering Contradiction:
Improveetch rateVSAvoidetch selectivity
Core Design Contradiction:
SpeedVSManufacturing precision

Solution Approach 1:

The patent optimizes the concentration parameters of HF (5-40 wt%) and NH4HF2 (40-80 wt%) to achieve the optimal balance point where etch rate is maximized while etch selectivity is maintained at 150 or higher

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent introduces ammonium hydrogen fluoride as an intermediary substance that mediates between the etching action of HF and the protection of silicon nitride, enabling high etch rate with maintained selectivity

Inventive Principle:
Principle #24Intermediary (Mediator)

3Manufacturing precision

If conventional BOE is used to achieve high etch selectivity, then selectivity to silicon nitride film is maintained, but productivity is reduced due to long process time required

Engineering Contradiction:
Improveetch selectivityVSAvoidproductivity
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The patent changes the etchant composition parameters to achieve both high etch rate (10000 Å/min or higher) and high etch selectivity (150 or higher), resolving the contradiction between processing speed and selectivity maintenance

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent enables continuous high-rate etching throughout the process by preventing Solid Phase Segregation and maintaining chemical stability, maximizing productivity without sacrificing selectivity

Inventive Principle:
Principle #20Continuity of useful action

4Ease of manufacture

If ammonium fluoride is used in conventional BOE, then etching capability is achieved, but contamination occurs due to sublimation property of ammonium fluoride in spray nozzle

Engineering Contradiction:
Improveetching capabilityVSAvoidcontamination
Core Design Contradiction:
Ease of manufactureVSObject-generated harmful factors

Solution Approach 1:

The patent extracts ammonium fluoride from the etchant composition and replaces it with ammonium hydrogen fluoride, eliminating the sublimation-related contamination problem while preserving etching capability

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent uses a composition that avoids materials with sublimation properties, preventing contamination of equipment and particles without requiring complex contamination control measures

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composition significantly increases etch selectivity and rate, reducing process time and improving productivity in single-type semiconductor processing by maintaining high etch rates and selectivity, while avoiding the stability and contamination issues of conventional etchants.

Implementation Method 1

a composition for wet etching of silicon dioxide includes 1 to 40 wt % of hydrogen fluoride (HF), 5 to 40 wt % of ammonium hydrogen fluoride (NH4HF2)

Methodology Applied
Scientific EffectWet etching: Chemical Bonding

Data Source

PatentUS8465662B2Composition for wet etching of silicon dioxide
Publication Date: 2013.06.18 TECHNO SEMICHEM

AI summary

Provided is an etching composition for electively removing silicon dioxide at a high etch rate, more particularly, a composition for wet etching of silicon dioxide, including 1 to 40 wt % of hydrogen fluoride (HF); 5 to 40 wt % of ammonium hydrogen fluoride (NH4HF2); and water, and further including a surfactant to improve selectivity of the silicon dioxide and a silicon nitride film. Since the composition for wet etching of silicon dioxide has the high etch selectivity of the silicon dioxide to the silicon nitride film, it is useful for selectively removing silicon dioxide.