Silicon Oxide Etching Gas Chemistry for Uniform Surface Flatness

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Solution Overview

Problem

Existing etching methods for silicon oxide films on semiconductor wafers result in uneven surface flatness due to variations in reaction product formation and collision probabilities of etching gases, leading to convex or concave shapes that degrade semiconductor device performance.

Innovation Solution

An etching method using a combination of halogen-containing, ammonia, and amine gases, with controlled gas supply cycles and pressure conditions, to achieve uniform etching and high surface flatness of silicon oxide films.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Device complexity

If a single type of etching gas is supplied to the silicon oxide film, then the etching process is simple, but the surface flatness becomes uneven due to variations in reaction product formation and gas collision probabilities

Engineering Contradiction:
Improveetching process complexityVSAvoidsurface flatness
Core Design Contradiction:
Device complexityVSManufacturing precision

Solution Approach 1:

The patent combines multiple types of etching gases (halogen-containing gas, ammonia gas, and amine gas) into a single etching atmosphere to simultaneously achieve uniform etching across the silicon oxide film surface and maintain process simplicity. This merging approach allows different gases to complement each other's functions, with halogen-containing gases providing etching capability and ammonia/amine gases regulating reaction product formation, thereby resolving the contradiction between process simplicity and surface flatness uniformity.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The patent changes the compositional parameters of the etching gas mixture by introducing multiple gas types with different chemical properties. Specifically, it controls the ratios of halogen-containing gas, ammonia gas, and amine gas to optimize the etching uniformity and surface flatness. This parameter adjustment allows the system to achieve desired etching results while maintaining controlled reaction conditions throughout the etching process.

Inventive Principle:
Principle #35Parameter changes

2Productivity

If etching gases are supplied continuously, then the etching speed is high, but the reaction product formation becomes uneven leading to convex or concave shapes on the etched surface

Engineering Contradiction:
Improveetching speedVSAvoidsurface shape uniformity
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent implements periodic action by sequentially controlling the supply of different etching gases during the etching process. It alternates between supplying halogen-containing gas for etching and ammonia/amine gases for reaction product management, creating a cyclic etching pattern that prevents excessive reaction product accumulation and ensures uniform surface morphology while maintaining high etching speed.

Inventive Principle:
Principle #19Periodic action

Solution Approach 2:

The patent maintains continuous useful action by ensuring that etching and reaction product management occur simultaneously through the continuous supply of a multi-component gas mixture. The halogen-containing gas continuously provides etching capability while ammonia and amine gases continuously regulate reaction product formation, ensuring both high productivity and uniform surface shape throughout the etching process.

Inventive Principle:
Principle #20Continuity of useful action

3Productivity

If halogen-containing gas alone is used for etching, then the etching rate is high, but the surface flatness deteriorates due to excessive reaction product formation

Engineering Contradiction:
Improveetching rateVSAvoidsurface flatness
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent introduces ammonia gas and amine gas as intermediary substances that mediate between the halogen-containing gas and the silicon oxide film. These intermediary gases regulate the formation and removal of reaction products, preventing excessive accumulation that would otherwise degrade surface flatness. They act as buffers that maintain etching rate while ensuring uniform surface morphology.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent creates a composite etching atmosphere by combining halogen-containing gas, ammonia gas, and amine gas in specific ratios. This composite gas mixture synergistically combines the high etching rate capability of halogen-containing gases with the surface-flatness-preserving properties of ammonia and amine gases, achieving both high productivity and high manufacturing precision simultaneously.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method ensures a desired shape and high flatness of etched silicon oxide films, preventing performance degradation in semiconductor devices by balancing reaction product formation and gas collisions, thereby enhancing manufacturing quality.

Implementation Method 1

etching a silicon oxide film by supplying a halogen-containing gas, an ammonia gas, and an amine gas as etching gases

Methodology Applied
Scientific EffectChemical reaction: Chemical Bonding

Implementation Method 2

whereby the reaction products are made to sublime

Methodology Applied
Scientific EffectSublimation: Sublimation

Data Source

PatentEP4682940A1Etching method and etching device
Publication Date: 2026.01.21 TOKYO ELECTRON LTD
  • EP4682940A1 patent drawingFigure 1
  • EP4682940A1 patent drawingFigure 2A~2D
  • EP4682940A1 patent drawingFigure 3A~3B

AI summary

An etching method according to the present disclosure includes an etching step in which a halogen-containing gas, an ammonia gas, and an amine gas are supplied as etching gases to a substrate including a silicon oxide film formed on a surface of the substrate, and the silicon oxide film is etched.