Silicon Planarizing Film Composition for Thick Crack-Resistant Coatings

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Solution Overview

Problem

Advanced semiconductor manufacturing requires dielectric materials that can planarize deep trenches, be crack-resistant at thicknesses exceeding 6 µm, and maintain high optical transmittance and thermal stability at temperatures above 400°C.

Innovation Solution

A composition comprising a silicon-based material, a polysiloxane resin formed from monomers like methyltriethoxysilane and phenyl triethoxysilane, a cross-linker with a siloxane compound, and a catalyst, which is applied via spin-coating or slot coating to form a planarizing film that is thermally stable and crack-resistant.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Length of stationary object

If dielectric material thickness is increased to fill deep trenches (6 µm or deeper), then planarization capability is improved, but crack resistance deteriorates

Engineering Contradiction:
Improvefilm thicknessVSAvoidcrack resistance
Core Design Contradiction:
Length of stationary objectVSReliability

Solution Approach 1:

The patent employs a composite dielectric material system comprising siloxane polymer composition with specific cross-linking agents and fillers. This composite structure combines multiple materials with complementary properties: the siloxane base provides flexibility and adhesion, cross-linking agents enhance mechanical strength and thermal stability, and fillers improve crack resistance. The synergistic combination allows the film to maintain integrity at thicknesses of 6 µm or deeper without cracking.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent optimizes chemical composition parameters including the ratio of cross-linking agents to base polymers, filler content and distribution, and molecular weight of polymer chains. By adjusting these parameters, the material achieves optimal balance between flexibility (for thick film application) and strength (for crack resistance). The cross-linking density and filler dispersion are controlled to prevent stress concentration that would lead to cracking in thick films.

Inventive Principle:
Principle #35Parameter changes

2Length of stationary object

If dielectric material thickness is increased to fill deep trenches, then planarization capability is improved, but thermal stability deteriorates at temperatures exceeding 400°C

Engineering Contradiction:
Improvefilm thicknessVSAvoidthermal stability
Core Design Contradiction:
Length of stationary objectVSStability of the object's composition

Solution Approach 1:

The composite dielectric material incorporates thermally stable components including metal oxide fillers (such as silica, alumina) and thermally resistant cross-linking agents. These materials maintain their structural integrity and chemical stability at temperatures exceeding 400°C, preventing degradation, outgassing, or phase separation that would compromise the thick film's performance during semiconductor manufacturing processes.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent selects and optimizes materials with high glass transition temperatures and stable molecular structures that resist thermal degradation. The cross-linking architecture is designed to create thermally stable three-dimensional networks that prevent polymer chain mobility and decomposition at elevated temperatures, ensuring the thick dielectric film maintains its mechanical and electrical properties during subsequent processing steps.

Inventive Principle:
Principle #35Parameter changes

3Reliability

If dielectric material is optimized for crack resistance, then reliability is improved, but optical transmittance deteriorates

Engineering Contradiction:
Improvecrack resistanceVSAvoidoptical transmittance
Core Design Contradiction:
ReliabilityVSIllumination intensity

Solution Approach 1:

The patent employs filler materials with controlled size distribution and refractive index matching to the polymer matrix. By optimizing the local optical properties through proper filler selection and dispersion, the material achieves high optical transmittance in the visible spectrum while maintaining crack resistance. The filler size and spacing are controlled to minimize light scattering, allowing the thick film to remain optically clear for optoelectronic applications.

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution provides a planarizing film with excellent crack-resistance and high optical transmittance, maintaining strength and thermal stability even at thicknesses greater than 6 µm and temperatures exceeding 400°C, suitable for advanced semiconductor devices.

Implementation Method 1

a cross-linker including a siloxane compound according to the general formula: wherein R is an aliphatic comprising group and R 1, R 2, R 3, R 4, R 5, and R 6 are each independently selected from the group consisting of: H or an alkyl group with substituted or unsubstituted carbons

Methodology Applied
Scientific EffectCross-linking: Chemical Bonding

Implementation Method 2

a polysiloxane resin, wherein said polysiloxane resin is formed from monomers consisting of methyltriethoxysilane, dimethyldiethoxysilane and phenyl triethoxysilane

Methodology Applied
Scientific EffectPolymerization: Chemical Bonding

Implementation Method 3

there is a need for dielectric materials which can be spin-coated onto a surface of a device

Methodology Applied
Scientific EffectSpin coating: Spin Coating

Data Source

PatentEP3729497B1Crack-resistant silicon-based planarizing compositions, methods and films
Publication Date: 2024.01.31 HONEYWELL INTERNATIONAL INC
  • EP3729497B1 patent drawingFigure 1
  • EP3729497B1 patent drawingFigure 2
  • EP3729497B1 patent drawing

AI summary

A composition for planarizing a surface of a semiconductor device includes a silicon-based material including a siloxane, a silsesquioxane, a polysiloxane, a polysilsesquioxane, and/or a polysiloxane resin, together with at least one solvent, a catalyst, and a cross-linker including a siloxane compound.