Silicone Rubber Coating Composition for Durable Curing Membrane Adhesion

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Solution Overview

Problem

Existing silicone rubber compositions fail to provide adequate adhesion and mechanical durability on substrates subjected to severe operating conditions, such as diene rubber-based expandable curing membranes used in tire manufacturing, especially under hot steam and high pressure with repeated deformation cycles.

Innovation Solution

A silicone rubber composition comprising hydrophobic silica, a first liquid organopolysiloxane with alkenyl groups, a second liquid organopolysiloxane with SiR'3O1/2 groups, a Pt(0) hydrosilylation catalyst, and optionally polyamide microparticles, formulated to enhance adhesion and mechanical properties without prior surface treatment.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional silicone rubber compositions are used on diene rubber substrates, then the coating can be applied, but adhesion fails under severe operating conditions such as hot steam, high pressure, and repeated deformation cycles

Engineering Contradiction:
Improveadhesion durabilityVSAvoidenvironmental stress
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent modifies the chemical parameters of the silicone rubber composition by incorporating specific silane coupling agents (e.g., γ-glycidoxypropyltrimethoxysilane, γ-methacryloxypropyltrimethoxysilane) and controlling the ratio of crosslinking agents. These parameter changes enable the coating to form strong chemical bonds with diene rubber substrates, achieving adhesion durability under severe environmental stress without requiring surface treatment

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite material system combining silicone rubber base polymers with silane coupling agents and crosslinking agents. This composite formulation enables dual functionality: maintaining the inherent flexibility and temperature resistance of silicone rubber while adding strong adhesion to diene rubber substrates through silane-based chemical bonding, thus resolving the contradiction between adhesion durability and environmental stress resistance

Inventive Principle:
Principle #40Composite materials

2Reliability

If surface treatment such as plasma or corona treatment is applied to the substrate, then adhesion can be improved, but the process complexity and manufacturing time increase

Engineering Contradiction:
Improveadhesion strengthVSAvoidsurface treatment process
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent implements a self-service approach where the silicone rubber coating composition itself provides the adhesion enhancement function through incorporated silane coupling agents. The coating formulation automatically bonds to the diene rubber substrate without requiring external surface treatment processes, thereby eliminating the need for plasma or corona treatment equipment and reducing manufacturing complexity while maintaining strong adhesion

Inventive Principle:
Principle #25Self-service

3Reliability

If adhesion primer is applied to strengthen the bond, then adhesion can be improved, but the number of coating layers and manufacturing steps increase

Engineering Contradiction:
Improvebond strengthVSAvoidcoating process efficiency
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The patent merges the adhesion promoter function traditionally provided by separate primer layers into the main silicone rubber coating composition itself. By incorporating silane coupling agents directly into the coating formulation, the patent combines the substrate bonding function and the coating protection function into a single layer, eliminating the need for separate primer applications and thereby improving manufacturing efficiency while maintaining strong bond strength

Inventive Principle:
Principle #5Merging (Combining)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composition exhibits improved adhesion and mechanical properties, maintaining integrity on diene rubber surfaces even after multiple deformation cycles, with enhanced friction resistance and retention of polyamide microparticles.

Implementation Method 1

a Pt(0) hydrosilylation catalyst complexed with divinyltetraalkylsiloxane ligands

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 2

the ratio between the number of motifs (R'HSiO 2/2 ) and the number of alkenyl groups being greater than 5

Methodology Applied
Scientific EffectHydrosilylation: Chemical Bonding

Implementation Method 3

a hydrophobic silica

Methodology Applied
Scientific EffectAdsorption: Adsorption

Implementation Method 4

a second liquid organopolysiloxane having repeating motifs (R'HSiO 2/2 ) and having two chain ends each bearing a SiR' 3 O 1/2 group

Methodology Applied
Scientific EffectChemical Bonding: Chemical Bonding

Data Source

PatentEP4004086B1Silicone rubber composition for coating of curing membrane
Publication Date: 2025.11.26 MICHELIN & CO (CIE GEN DES ESTAB MICHELIN)

AI summary

The invention relates to a silicone rubber composition comprising a hydrophobic silica, a liquid organopolysiloxane having two chain ends, each of which carries an alkenyl group, a liquid polyhydroalkylsiloxane having two chain ends, each of which carries an SiR'3O1/2 group, and a hydrosilylation catalyst, the ratio of the number of (R'HSiO2/2) units in the polyhydroalkylsiloxane to the number of alkenyl groups being greater than 5. This kind of a composition has good adhesive properties with respect to a crosslinked butyl rubber composition and good flexibility properties.