SOEC/SOFC Stack Interconnector Welding for Stable Gas Distribution

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Solution Overview

Problem

Existing high-temperature solid oxide electrolyzer (SOEC) and fuel cell (SOFC) stacks face challenges in achieving stable electrical contact, proper gas distribution, and efficient gas compartment separation, leading to inefficiencies and potential damage from hot spots and gas recombination.

Innovation Solution

A method involving spot welding a metallic coating layer, such as a nickel grid, onto interconnectors with a specific adhesive composition to secure electrochemical cells, combined with ceramic contact layers, ensures stable assembly and rigid structure, enhancing electrical contact and gas distribution.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If a metallic coating layer is spot-welded onto the interconnector to form a contact layer, then electrical contact stability is improved, but the assembly complexity and manufacturing difficulty increase

Engineering Contradiction:
Improveelectrical contact stabilityVSAvoidassembly complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The metallic coating layer is applied to the interconnector surface before assembly, and spot-welding is performed during the manufacturing process to pre-establish reliable electrical contacts. This preliminary action ensures that electrical contact stability is achieved before the stack operates, preventing contact failures during service.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The metallic coating layer acts as an intermediary between the interconnector and the electrochemical cell, providing a dedicated contact interface that ensures stable electrical connection while isolating the bulk interconnector material from direct contact requirements.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Stability of the object's composition

If an adhesive is used to fix the electrochemical cell to the interconnector, then cell stability and position fixation are improved, but residue formation and potential degradation increase

Engineering Contradiction:
Improvecell stabilityVSAvoidresidue formation
Core Design Contradiction:
Stability of the object's compositionVSObject-generated harmful factors

Solution Approach 1:

The adhesive composition is specifically formulated with controlled parameters including polyvinyl butyral content (5-50% by mass), terpineol content (5-50% by mass), and ethanol content (5-95% by mass). These parameter optimizations ensure the adhesive provides sufficient bonding strength while minimizing residue formation that could cause degradation.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The adhesive is a composite material combining polyvinyl butyral (providing bonding strength), terpineol (acting as a plasticizer and solvent), and ethanol (serving as a volatile carrier). This composite formulation achieves the desired balance between cell stability and residue minimization.

Inventive Principle:
Principle #40Composite materials

3Reliability

If the adhesive is deposited around the periphery of the coating layer outside the active area, then gas distribution is improved by avoiding active zone contamination, but the bonding area and attachment strength are reduced

Engineering Contradiction:
Improvegas distributionVSAvoidattachment strength
Core Design Contradiction:
ReliabilityVSStrength

Solution Approach 1:

The adhesive is applied with spatially varying properties: it is deposited around the periphery of the coating layer outside the active area, creating a localized bonding zone that does not interfere with gas distribution channels while still providing sufficient attachment strength through optimized peripheral bonding.

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The interconnector design incorporates contact ribs that replicate the gas distribution channel pattern, allowing the adhesive to be positioned in non-active peripheral zones while maintaining proper gas flow paths through the replicated rib structure.

Inventive Principle:
Principle #26Copying

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method improves the stability and efficiency of SOEC/SOFC stacks by preventing cell movement and residue formation, ensuring optimal electrical contact and gas distribution, thereby increasing production efficiency and reducing degradation.

Implementation Method 1

spot welding the metallic coating layer on the first face of the interconnector to allow its fixing

Methodology Applied
Scientific EffectSpot welding: Welding

Implementation Method 2

depositing an adhesive around the periphery of the coating layer (GN), outside the active area and away from the gas supplies, intended to fix the electrochemical cell (1)

Methodology Applied
Scientific EffectAdhesion: Adhesive

Implementation Method 3

each interconnector having two main flat faces, a second face of the two main flat faces comprising a thick ceramic coating layer, forming a contact layer with an electrochemical cell

Methodology Applied
Scientific EffectThermal contact: Conduction (thermal)

Data Source

PatentEP4315462B1Method of manufacturing a stack of solid oxides of the type soec/sofc and related stack
Publication Date: 2026.03.11 COMMISSARIAT A LENERGIE ATOMIQUE ET AUX ENERGIES ALTERNATIVES
  • EP4315462B1 patent drawingFigure 1~2
  • EP4315462B1 patent drawingFigure 3
  • EP4315462B1 patent drawingFigure 4~5

AI summary

The invention relates mainly to a method for producing a SOEC/SOFC-type solid oxide stack operating at high temperature, comprising a plurality of electrochemical cells each formed by a cathode, an anode and an electrolyte inserted between the cathode and the anode, and a plurality of metal interconnectors each arranged between two adjacent electrochemical cells, each interconnector having two main flat faces, a first face (P1) of the two main flat faces comprising a metal coating layer (GN) in the form of a grid forming a contact layer with an electrochemical cell, the method comprising the step of spot-welding (S) the metal coating layer (GN) onto the first face (P1) of the interconnector in order to allow the attachment thereof.