Soft Elastomeric Films via Selective Hydrogenation

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Solution Overview

Problem

Soft elastomeric films used in personal hygiene articles, such as gloves and diapers, face challenges with thermal, oxidative, and UV degradation due to their unsaturated nature, limiting their stability and performance over time.

Innovation Solution

Development of selectively hydrogenated block copolymers with specific molecular weights and vinyl content, combined with coupling agents and hydrogenation processes, to create stable and soft elastomeric films that retain strength and elasticity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If unsaturated block copolymers (SIS) are used to produce soft elastomeric films, then softness and strength are achieved, but thermal, oxidative and UV stability deteriorate

Engineering Contradiction:
Improvefilm strengthVSAvoidoxidative and UV stability
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

The patent applies parameter changes by partially hydrogenating the unsaturated block copolymer to reduce double bond content from 100% (in SIS) to a controlled level (0-50% retention), thereby improving oxidative and UV stability while maintaining sufficient softness and strength for personal hygiene applications

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite material system by combining hydrogenated block copolymer with specific additives including antioxidants, UV absorbers, and processing aids, forming a stable elastomeric film composition that addresses multiple performance requirements simultaneously

Inventive Principle:
Principle #40Composite materials

2Reliability

If saturated block copolymers (SEBS) are used to improve stability, then thermal and oxidative stability improve, but softness and strength deteriorate

Engineering Contradiction:
Improvethermal stabilityVSAvoidfilm strength
Core Design Contradiction:
ReliabilityVSStrength

Solution Approach 1:

The patent applies partial action by performing partial hydrogenation rather than complete hydrogenation, retaining 0-50% of double bonds to maintain the elastomeric properties and softness characteristic of unsaturated polymers while gaining sufficient stability for commercial applications

Inventive Principle:
Principle #16Partial or excessive action

Solution Approach 2:

The patent modifies the saturation level parameter to an intermediate state (partially hydrogenated) that balances the conflicting requirements of stability and softness, avoiding the extremes of fully unsaturated (unstable) or fully saturated (too rigid) states

Inventive Principle:
Principle #35Parameter changes

3Productivity

If high temperatures are used during melt processing, then processing efficiency improves, but thermal degradation of unsaturated films worsens

Engineering Contradiction:
Improveprocessing efficiencyVSAvoidthermal degradation
Core Design Contradiction:
ProductivityVSObject-affected harmful factors

Solution Approach 1:

The patent applies preliminary action by pre-hydrogenating the block copolymer before processing, which stabilizes the material against thermal degradation during subsequent melt processing operations, allowing for more robust processing conditions

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent changes the chemical composition parameter (double bond content) to reduce susceptibility to thermal degradation, enabling processing at temperatures and shear rates that would otherwise cause degradation of fully unsaturated polymers

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The resulting films exhibit improved thermal, oxidative, and UV stability while maintaining softness and strength, suitable for prolonged use in personal hygiene applications.

Implementation Method 1

selectively hydrogenated block copolymers which has the softness of conventional SIS-based films but the stability inherent in saturated conjugated diene rubbers

Methodology Applied
Scientific EffectHydrogenation: Hydrogenation

Data Source

PatentEP2231767B1Soft elastomeric films
Publication Date: 2014.10.15 KRATON POLYMERS US LLC
  • EP2231767B1 patent drawingFigure 1
  • EP2231767B1 patent drawingFigure 2

AI summary

Elastomeric films which are both soft and thermally, UV and oxidatively stable are provided. The films are composed of coupled, selectively hydrogenated block copolymers having a relatively high molecular weight and high vinyl content. In addition to the block copolymer other components may be present in formulated films such as other block copolymers, hydrocarbon resins, polyolefins, metallocene polyolefins, homopolystyrene or mineral oils. The softness of the films is determined by the stress at 100% tensile elongation where the films with suitable softness have a 100% stress of about 100 psi or less. While soft, the films also are strong with tensile strengths of 1000 psi or more and suitable hysteresis properties. The elastomeric films are useful as integral components of personal hygiene articles such as gloves, diapers, incontinence products, disposable swimwear and disposable undergarments.