Solid-State High Harmonic CEP Measurement for Mid-IR Femtosecond Pulses

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Solution Overview

Problem

Existing methods for measuring carrier-to-envelope phase (CEP) fluctuations of femtosecond laser pulses face challenges such as the generation of stable supercontinuum spectra, weak interference signals, and limited availability of high-resolution spectrometers, particularly in the mid-infrared range, which hinder precise CEP measurement.

Innovation Solution

A method involving high harmonic generation in solids, where femtosecond laser pulses are focused in a solid-state material to generate high harmonics, and the relative phase is inferred from the high harmonic spectrum, allowing for single-shot CEP measurement by comparing individual harmonic spectra to a reference spectrogram.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Measurement precision

If f-to-2f spectral interferometry is used to measure CEP fluctuations, then CEP measurement capability is achieved, but measurement precision is limited by weak interference signals and availability of high-resolution spectrometers

Engineering Contradiction:
ImproveCEP measurement precisionVSAvoiddifficulty in detecting weak interference signals
Core Design Contradiction:
Measurement precisionVSDifficulty of detecting and measuring

Solution Approach 1:

The patent transforms the measurement approach by changing the physical parameter being measured from direct spectral interference to high harmonic generation intensity. By measuring the intensity of high harmonics (which strongly depends on CEP) rather than relying on weak spectral interference patterns, the measurement precision is significantly improved while avoiding the limitations of spectrometer resolution and signal weakness.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent replaces the optical interference-based measurement system with a high harmonic generation-based system. Instead of using spectral interferometry requiring complex optical paths and high-resolution spectrometers, the invention uses the nonlinear optical process of high harmonic generation in gases, where the harmonic intensity directly encodes CEP information, simplifying the measurement system while improving precision.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

2Adaptability or versatility

If supercontinuum generation is used in f-to-2f interferometry, then spectral broadening is achieved, but generation of stable supercontinuum spectra becomes difficult

Engineering Contradiction:
Improvespectral broadening capabilityVSAvoidstability of supercontinuum spectrum
Core Design Contradiction:
Adaptability or versatilityVSReliability

Solution Approach 1:

The patent extracts only the essential function of spectral broadening needed for CEP measurement, discarding the problematic supercontinuum generation step. By using high harmonic generation directly on the fundamental laser frequency, the method achieves the necessary spectral extension to the ultraviolet range without requiring stable supercontinuum spectra, thus eliminating the reliability issue while maintaining spectral versatility.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

Instead of broadening the spectrum first and then measuring interference (the conventional f-to-2f approach), the patent inverts the sequence by generating high harmonics directly from the fundamental frequency. This reversal eliminates the need for stable supercontinuum generation while achieving the same goal of accessing ultraviolet frequencies for CEP measurement.

Inventive Principle:
Principle #13The other way round (Inversion)

3Measurement precision

If high-resolution spectrometers are used for spectral interferometry, then measurement accuracy improves, but device complexity and cost increase

Engineering Contradiction:
ImproveCEP measurement accuracyVSAvoidcomplexity of spectrometer system
Core Design Contradiction:
Measurement precisionVSDevice complexity

Solution Approach 1:

The patent replaces the complex mechanical and optical system of high-resolution spectrometers with a simpler detection scheme. By measuring the intensity of high harmonic frequencies generated in a gas medium, the system uses standard photodetectors or photodiodes instead of complex spectrometers, significantly reducing device complexity while maintaining high measurement accuracy through the CEP-sensitive nature of high harmonic generation.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Solution Approach 2:

The patent substitutes expensive, complex high-resolution spectrometers with simpler, more affordable detection devices. The use of standard photodetectors to measure high harmonic intensity replaces the need for costly spectrometric equipment, making the CEP measurement system more accessible and less complex while achieving comparable or superior measurement accuracy.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

Enables precise measurement of CEP fluctuations in femtosecond laser pulses, even in the mid-infrared range, by leveraging the sensitivity of high harmonic generation to CEP variations, providing accurate and efficient CEP stability assessment.

Implementation Method 1

focusing laser pulses in a solid-state material for high harmonic generation, collecting a resulting high harmonic spectrum

Methodology Applied
Scientific EffectHigh harmonic generation:

Data Source

PatentUS12512644B2Method and system for measuring carrier-to-envelope phase fluctuations of a femtosecond laser pulse
Publication Date: 2025.12.30 INSTITUT NATIONAL DE LA RECHERCHE SCIENTIFIQUE
  • US12512644B2 patent drawing
  • US12512644B2 patent drawing
  • US12512644B2 patent drawing

AI summary

A method and a system for measuring carrier-to-envelope phase fluctuations (CEP) fluctuations of a laser field, the method comprising focusing laser pulses in a solid-state material for high harmonic generation, collecting a resulting high harmonic spectrum, and inferring a relative phase of the driving field from the high harmonic spectrum. The system comprises a source of CEP stable mid-infrared laser pulses; a CEP variation unit; a solid state medium; a detector; and first focusing optics focusing pulses generated by the source into the solid state medium and second focusing optics collecting resulting harmonics generated in the solid state medium into the detector.