Solvothermal Lithium Extraction Using Polyol Solvents

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Solution Overview

Problem

Current lithium extraction methods from lithium-containing materials, such as lithium-ion batteries and ores, are economically and environmentally costly due to the use of hazardous chemicals, high energy requirements, and the need for multiple steps, especially in processes like hydrometallurgy and pyrometallurgy, which also result in the non-selective dissolution of other metals.

Innovation Solution

A solvothermal process using a polyol solvent and carbonate to selectively extract lithium from materials containing lithium and other metals, such as cobalt, nickel, and manganese, without the need for hazardous chemicals or additional waste treatment, involving steps like solvothermal treatment, separation, and optional isolation of lithium carbonate.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If hydrometallurgy or pyrometallurgy processes are used to extract lithium, then lithium can be extracted from the material, but hazardous chemicals are used and high energy requirements are incurred, resulting in environmental costs and economic costs

Engineering Contradiction:
Improvelithium extraction efficiencyVSAvoidhazardous chemical waste and energy consumption
Core Design Contradiction:
ProductivityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the chemical parameters by using a polyol solvent system instead of traditional strong acids, and controls temperature parameters through solvothermal conditions (typically 100-250°C) to achieve selective lithium extraction without hazardous chemicals and with reduced energy consumption compared to pyrometallurgy

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent introduces a polyol solvent as an intermediary substance that mediates the extraction process. The polyol forms soluble complexes with lithium at specific temperature ranges, enabling selective extraction without requiring hazardous strong acids or high-energy combustion conditions

Inventive Principle:
Principle #24Intermediary (Mediator)

2Productivity

If traditional leaching processes are used, then lithium can be extracted, but other metals are also dissolved non-selectively, requiring additional extraction and precipitation steps

Engineering Contradiction:
Improvelithium extraction rateVSAvoidnumber of processing steps
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The patent applies local quality by creating selective chemical environments through polyol solvents that specifically target lithium extraction. The polyol-Lithium complex formation occurs under controlled solvothermal conditions, allowing lithium to be selectively extracted while leaving other metals undissolved, thus eliminating the need for multiple separation steps

Inventive Principle:
Principle #3Local quality

3Productivity

If brine excavation is used for lithium production, then lithium can be extracted from natural sources, but production is limited to selected climates and regions and is dependent on weather conditions

Engineering Contradiction:
Improvelithium production volumeVSAvoidgeographic and climatic adaptability
Core Design Contradiction:
ProductivityVSAdaptability or versatility

Solution Approach 1:

The patent replaces the natural weather-dependent evaporation process of brine excavation with a controlled solvothermal chemical process. Instead of relying on solar evaporation in specific climates, the invention uses polyol solvents under controlled temperature and pressure conditions to extract lithium, making the process adaptable to any geographic location regardless of climate

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This process achieves efficient, selective, and environmentally friendly lithium extraction with reduced energy consumption and no hazardous chemical waste, making it economically viable and suitable for recycling lithium from various sources, including lithium-ion battery cathode materials and ores.

Implementation Method 1

Performing a solvothermal treatment of the reaction mixture obtained in step a) to obtain a solvothermally treated composition SP1

Methodology Applied
Scientific EffectSolvothermal treatment:

Implementation Method 2

Contacting said material with a polyol solvent and a carbonate to obtain a reaction mixture

Methodology Applied
Scientific EffectSolvation: Solvation

Implementation Method 3

Separating the liquid L1 containing lithium carbonate and the solid S1 forming the composition SP1 obtained in step b)

Methodology Applied
Scientific EffectLiquid-solid separation:

Data Source

PatentUS20230056619A1Process of extraction of lithium from a material comprising lithium and at least another metal
Publication Date: 2023.02.23 ECOLE NAT SUPERIEURE DINGS DE CAEN

AI summary

The present invention is in the field of the extraction of lithium from a material comprising lithium and at least another metal. In particular, the invention concerns a process of extraction of lithium at least, from a material comprising lithium and at least another metal.