Spark Plug Electrode Material With Ni Oxide Oxidation Barrier

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Solution Overview

Problem

Iridium (Ir) alloy spark plug electrodes face challenges with high-temperature oxidation resistance due to the volatility of Ir oxides, leading to shorter lifespan compared to platinum plugs, especially in harsh engine environments with lean combustion, high EGR systems, and high power/rotation speed/compression ratio designs.

Innovation Solution

A spark plug electrode material featuring a substrate of Ir or Ir alloy with a Ni oxide antioxidant film, where the Ni film is converted to Ni oxide through heat treatment, providing a thickness of 3.0 µm to 8.0 µm to suppress oxidation and volatilization, and an underlying Au layer for adhesion and protection.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If Ir or Ir alloy is used as electrode material to achieve thinner electrode shape and good ignition efficiency, then ignition/combustion efficiency is improved, but high-temperature oxidation resistance deteriorates due to volatility of Ir oxides

Engineering Contradiction:
Improveignition efficiencyVSAvoidhigh-temperature oxidation resistance
Core Design Contradiction:
ProductivityVSReliability

Solution Approach 1:

A Ni film is introduced as an intermediary protective layer between the Ir electrode material and the oxidizing environment. The Ni film oxidizes preferentially to form NiO, which acts as a barrier preventing oxygen from reaching and oxidizing the Ir substrate, thereby protecting the electrode while maintaining its ignition functionality

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The invention creates a composite structure consisting of the Ir electrode material combined with a Ni protective film layer. This composite material leverages the excellent electrical and ignition properties of Ir while adding the oxidation protection capabilities of Ni/NiO, resolving the contradiction between ignition efficiency and oxidation resistance

Inventive Principle:
Principle #40Composite materials

2Reliability

If alloy composition is optimized by adding precious metals like Pt or Rh to improve high-temperature oxidation resistance, then oxidation resistance is improved, but manufacturing cost increases

Engineering Contradiction:
Improvehigh-temperature oxidation resistanceVSAvoidmanufacturing cost
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

Instead of using expensive precious metals for alloying, the invention employs a Ni film that serves as a sacrificial protective layer. The Ni film is relatively inexpensive and can be applied through cost-effective plating processes, providing oxidation protection without the high material costs associated with Pt or Rh alloys

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The invention changes the approach from modifying the bulk alloy composition to applying a surface coating with specific thickness parameters (3.0 μm to 8.0 μm). This parameter-based solution allows control of oxidation resistance through film thickness rather than expensive alloying, reducing manufacturing costs while maintaining reliability

Inventive Principle:
Principle #35Parameter changes

3Reliability

If Ni film thickness is increased to enhance oxidation protection, then high-temperature oxidation resistance is improved, but manufacturing complexity and cost increase

Engineering Contradiction:
Improveoxidation protectionVSAvoidfilm thickness control
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The invention establishes specific parameter ranges for the Ni film thickness (3.0 μm to 8.0 μm) that optimize both protection effectiveness and manufacturability. Within this range, the film provides sufficient oxidation barrier properties without requiring excessive thickness control precision or adding unnecessary manufacturing complexity

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The Ni film thickness is designed to be sufficient but not excessive (3.0-8.0 μm range). This partial action approach provides adequate oxidation protection without the diminishing returns and increased complexity associated with much thicker films, balancing effectiveness with manufacturability

Inventive Principle:
Principle #16Partial or excessive action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The Ni oxide film significantly enhances high-temperature oxidation resistance, reducing Ir consumption and extending the lifespan of spark plug electrodes by inhibiting oxygen diffusion and maintaining effectiveness even in extreme conditions.

Implementation Method 1

an antioxidant film being a Ni film having a thickness of 3.0 μm or more and 8.0 μm or less... the antioxidant film may be Ni oxide

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 2

the Ni film is converted to Ni oxide through heat treatment

Methodology Applied
Scientific EffectHeat treatment: Heat Treatment

Implementation Method 3

providing a thickness of 3.0 µm to 8.0 µm to suppress oxidation and volatilization... by inhibiting oxygen diffusion

Methodology Applied
Scientific EffectDiffusion barrier: Diffusion Barrier

Data Source

PatentEP3849032B1Material for spark plug electrodes and method for producing same
Publication Date: 2023.12.27 TANAKA KIKINZOKU KOGYO KK
  • EP3849032B1 patent drawingFigure 1

AI summary

The present invention discloses a spark plug electrode material including a substrate formed of Ir or Ir alloy, and an antioxidant film covering a surface of the substrate. Here, an underlying layer formed of Au is formed on a surface of the substrate formed of Ir or Ir alloy, and on the underlying layer, a Ni film having a thickness of 3.0 µm or more and 8.0 µm or less is formed as an antioxidant film. The Ni film turns into an antioxidant film formed of Ni oxide in an oxidizing atmosphere at 500°C or higher. Owing to the antioxidant film, the spark plug electrode material of the present invention has an excellent high-temperature oxidation property.