Spherical Iron Powder via Oxidation-Reduction Cycle

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Solution Overview

Problem

Current methods for producing spherical iron powder are either expensive, toxic, or limited in producing fine particle sizes, with existing techniques like inert gas atomization being costly and introducing impurities, while reduction methods result in irregular shapes.

Innovation Solution

A method involving spray roasted iron oxide reduction in a carbon monoxide or hydrogen-rich gas environment, followed by oxidation and subsequent reduction to produce spherical iron powder with high purity and fine particle sizes, utilizing a multi-step process including heating, cooling, crushing, and screening to achieve dense spherical morphology.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Shape

If inert gas atomization is used to produce spherical iron powder, then spherical shape is achieved, but production cost increases significantly and particle size is limited

Engineering Contradiction:
Improvespherical shapeVSAvoidproduction cost
Core Design Contradiction:
ShapeVSEase of manufacture

Solution Approach 1:

The invention changes the fundamental parameters of the process by using liquid iron drop oxidation followed by hydrogen reduction, replacing the conventional inert gas atomization method. This parameter change enables spherical powder production without the high costs and size limitations of atomization techniques

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention replaces the mechanical atomization system with a chemical-thermal system involving controlled oxidation and reduction reactions. This substitution eliminates the need for high-pressure inert gas systems while achieving spherical morphology through controlled phase changes and surface tension effects during droplet formation

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

2Manufacturing precision

If carbonyl process is used to produce fine spherical iron powder, then fine particle size is achieved, but toxicity increases due to hazardous gases

Engineering Contradiction:
Improvefine particle sizeVSAvoidtoxicity
Core Design Contradiction:
Manufacturing precisionVSObject-affected harmful factors

Solution Approach 1:

The invention changes the chemical parameters by replacing carbonyl chemistry with oxidation-reduction chemistry using hydrogen and oxygen. This parameter change maintains fine particle size control through droplet-based processing while eliminating toxic carbon monoxide and carbonyl compounds from the process

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention converts the potentially harmful oxidation of iron into a beneficial step by controlling the oxidation to form spherical iron oxide droplets, which are then reduced to pure iron. The controlled oxidation that could be harmful is instead used to define the spherical morphology before final reduction

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

3Ease of manufacture

If reduction techniques are used to produce iron powder, then production cost is reduced, but particle shape becomes irregular

Engineering Contradiction:
Improveproduction costVSAvoidparticle shape
Core Design Contradiction:
Ease of manufactureVSShape

Solution Approach 1:

The invention performs preliminary oxidation of liquid iron droplets to form spherical iron oxide particles before the final reduction step. This preliminary action establishes the spherical morphology early in the process, which is then preserved through the reduction step, ensuring spherical shape in the final product while maintaining cost-effectiveness

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The invention utilizes phase transitions of iron through multiple states: liquid iron → oxidized liquid/solid iron oxide → reduced solid iron powder. These controlled phase transitions, particularly the liquid-to-solid transition during droplet cooling, naturally form spherical shapes that are maintained through subsequent processing steps

Inventive Principle:
Principle #36Phase transitions

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method effectively produces spherical iron powder with at least 98% metallic iron and a dense spherical morphology, achieving high purity and fine particle sizes in a cost-effective and non-toxic manner, suitable for various industrial applications.

Implementation Method 1

heating the spherical iron oxide in a reduction furnace to a temperature of about 500°C to 1200°C and reducing the spherical iron oxide in presence of a carbon monoxide rich gas or a hydrogen rich gas or a solid carbonaceous reducing agent

Methodology Applied
Scientific EffectChemical reduction: Reduction

Implementation Method 2

burning the irregular iron powder in the presence of oxygen rich gas to generate exothermic heat to melt and convert the irregular iron particles of the irregular iron powder into the spherical iron oxide particles

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 3

burning the irregular iron powder in the presence of oxygen rich gas to generate exothermic heat

Methodology Applied
Scientific EffectCombustion: Combustion

Implementation Method 4

heating the iron oxide (raw material) in a reduction furnace to a temperature of about 500°C to 1200°C

Methodology Applied
Scientific EffectThermal heating: Heating

Data Source

PatentEP3883713B1A method of producing spherical iron powder
Publication Date: 2024.07.03 TATA STEEL LTD
  • EP3883713B1 patent drawingFigure 1~2
  • EP3883713B1 patent drawingFigure 3
  • EP3883713B1 patent drawingFigure 4

AI summary

The present disclosure relates to a simple, economical, non-toxic and efficient method of producing spherical iron powder from iron oxide. The method comprises reacting iron oxide with a reducing agent to produce irregular iron powder, burning the obtained irregular iron powder in presence of oxygen to produce spherical iron oxide particles, and thereafter reacting the spherical iron oxide with a reducing agent to obtain the final spherical iron powder. The obtained spherical iron powder is characterized by a spherical morphology, high purity, finer particle size range and a porous structure across the surface of iron powder.