Multilayer Spider Silk Protein Films via Formic Acid Evaporation

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Solution Overview

Problem

There is no general method available for forming multilayer films from spider silk proteins, as existing methods require specific conditions such as oppositely charged layers, which limits their application and stability.

Innovation Solution

A method involving the use of spider silk protein solutions in formic acid, where the acid is evaporated to form a film layer, and this process is repeated to create multiple layers, allowing for stable multilayer films without the need for surface modification, enabling the combination of different silk proteins and other materials for tailored properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Stability of the object's composition

If existing methods using oppositely charged layers are used to form multilayer films, then film stability is improved, but the method complexity and requirement for surface modification increase

Engineering Contradiction:
Improvemultilayer film stabilityVSAvoidsurface modification requirement
Core Design Contradiction:
Stability of the object's compositionVSDevice complexity

Solution Approach 1:

The patent extracts and removes the requirement for surface modification and charged layers from the film formation process. By using formic acid as a solvent that evaporates completely, the method eliminates the need for complex surface treatments while maintaining film stability through the natural properties of silk proteins in formic acid solution.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent changes the chemical parameter of the solvent from water or buffered solutions to formic acid. This parameter change allows the silk proteins to self-assemble into stable multilayer films without requiring charged surfaces, as formic acid provides the right chemical environment for protein stabilization during film formation.

Inventive Principle:
Principle #35Parameter changes

2Ease of manufacture

If a general method for forming multilayer films from silk proteins is developed, then versatility and ease of manufacture are improved, but the need for specific conditions (such as charged layers) is reduced

Engineering Contradiction:
Improvefilm production simplicityVSAvoidapplication range
Core Design Contradiction:
Ease of manufactureVSAdaptability or versatility

Solution Approach 1:

The patent creates a universal method that can produce multilayer films from any silk protein source (spider, insect, or recombinant) using a single approach with formic acid. This universal solvent system replaces multiple specialized methods, allowing the same basic procedure to be applied across different protein types while maintaining film quality and stability.

Inventive Principle:
Principle #6Universality (Multi-functionality)

3Manufacturing precision

If multiple layers are formed by repeating the film formation process, then film thickness and composition control are improved, but the production time increases

Engineering Contradiction:
Improvefilm thickness controlVSAvoidproduction time
Core Design Contradiction:
Manufacturing precisionVSLoss of time

Solution Approach 1:

The patent prepares silk protein solutions in formic acid with predetermined concentrations and compositions before the film formation process. This preliminary preparation allows for precise control of film thickness and properties from the outset, reducing the need for iterative adjustments and speeding up the overall production process while maintaining manufacturing precision.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enables the production of stable and tailored multilayer spider silk protein films with controlled thickness and composition, allowing for various applications by combining different silk proteins and other materials, such as polystyrene or collagen, without the need for surface modification, enhancing their bio-functionality and structural properties.

Implementation Method 1

evaporating the formic acid, thereby forming a first spider silk protein film layer

Methodology Applied
Scientific EffectEvaporation: Evaporation

Data Source

PatentEP2013290B1Multilayer silk protein films
Publication Date: 2013.06.12 AMSILK
  • EP2013290B1 patent drawingFigure 1
  • EP2013290B1 patent drawingFigure 2
  • EP2013290B1 patent drawingFigure 3

AI summary

The present invention is directed to a method of forming multilayer silk protein films and a multilayer film obtained therefrom. The invention is further directed to various materials, products and compositions containing said multilayer film and to the use of Said multilayer film in several applications.