Spray Device Capillary Nozzle for Homogeneous Matrix Crystals

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Solution Overview

Problem

Current methods for coating tissue samples in MALDI imaging struggle with forming small, homogeneous matrix crystals, leading to limited resolution and inefficient use of expensive matrix solutions, especially when detecting larger molecules like peptides or proteins, due to large crystal sizes and excessive matrix consumption.

Innovation Solution

A method involving multiple thin layers of matrix solution application with increasing amounts per area, using a spray device with a capillary line and gas outlet configuration that produces fine droplets, allowing for precise control and homogeneous layer formation, resulting in crystal sizes as small as 130-140 nm.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If a large amount of matrix solution is applied to the sample, then extraction of large molecules is improved, but crystal size increases and resolution decreases

Engineering Contradiction:
Improvematrix solution amountVSAvoidcrystal size
Core Design Contradiction:
Quantity of substanceVSManufacturing precision

Solution Approach 1:

The coating process is divided into multiple sequential spray passes (at least two passes) with drying intervals between them. Each pass deposits a thin layer of matrix solution that dries to form a partial coating. This segmentation allows the total matrix amount to be accumulated in controlled increments, preventing excessive crystal growth that would occur with single-pass application of large amounts, while still achieving sufficient matrix quantity for large molecule extraction.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The first spray pass applies a preliminary layer of matrix solution that is allowed to dry completely before subsequent passes. This preliminary action creates a foundation layer that facilitates controlled crystal formation and prevents the formation of large crystals that would result from applying all matrix solution at once. The drying step between passes is a preliminary action that prepares the surface for controlled additional matrix deposition.

Inventive Principle:
Principle #10Preliminary action

2Area of stationary object

If matrix solution is applied to the entire area, then complete coverage is achieved, but matrix consumption increases

Engineering Contradiction:
Improvecoverage areaVSAvoidmatrix consumption
Core Design Contradiction:
Area of stationary objectVSLoss of substance

Solution Approach 1:

The spray device is configured to apply matrix solution selectively to the sample area with controlled distribution. The multi-pass spraying with drying intervals allows matrix solution to be concentrated where needed on the sample surface rather than uniformly covering the entire area. This local quality approach ensures complete sample coverage while minimizing matrix consumption by avoiding unnecessary application to surrounding areas.

Inventive Principle:
Principle #3Local quality

3Measurement precision

If crystal size is reduced to improve resolution, then detection precision improves, but matrix solution efficiency decreases

Engineering Contradiction:
Improvedetection resolutionVSAvoidmatrix solution efficiency
Core Design Contradiction:
Measurement precisionVSQuantity of substance

Solution Approach 1:

The coating process uses periodic spraying interspersed with drying periods. Each spray-dry cycle creates a generation of fine matrix crystals. By repeating this periodic action multiple times, fine crystals are formed and accumulated without the need to apply excessive matrix solution in a single pass. The periodic drying intervals are critical as they allow crystal formation to occur in a controlled manner, maintaining fine crystal size while building up sufficient matrix quantity for efficient large molecule extraction.

Inventive Principle:
Principle #19Periodic action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enables detailed, semi-quantitative or quantitative detection of molecules by achieving smaller matrix crystal sizes, improving resolution to match advanced laser technology, and optimizing matrix usage, suitable for analyzing tissues at a cellular level.

Implementation Method 1

the air flow entrains and finely distributes the liquid according to the ejector principle

Methodology Applied
Scientific EffectAir Entrainment: Entrainment

Implementation Method 2

the previously applied layer has dried

Methodology Applied
Scientific EffectEvaporation: Evaporation

Data Source

PatentEP3334537B1Method for coating samples
Publication Date: 2020.10.07 SUNCHROM WISS GERATE
  • EP3334537B1 patent drawingFigure 1
  • EP3334537B1 patent drawingFigure 2
  • EP3334537B1 patent drawingFigure 3

AI summary

The spraying device serves for spraying samples with a solution, wherein a liquid feed for the metered feeding of the solution and a gas feed are provided which are connected via supply lines to a nozzle head (10) which has a gas outlet (36) and a liquid outlet (16) in order to spray the solution. In order, after drying, to allow a formation of relatively small crystals of the matrix in a coating which is as homogeneous as possible, it is proposed that the liquid outlet (16) is provided at the end of a capillary line (14) which projects beyond the gas outlet (36).