SrGa2S4:Eu Green Phosphor Crystallinity Control

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Solution Overview

Problem

Conventional green phosphors excited by blue LEDs have insufficient conversion efficiency, necessitating a higher efficiency phosphor for effective light emission.

Innovation Solution

A green phosphor with the composition formula (Sr1-yCay)1-xGa2S4:Eu x (0.03 ≤ x ≤ 0.20 and 0 < y ≤ 1) is developed, where the full width at half maximum of the diffraction peak corresponding to the (422) plane in the XRD pattern is less than 0.18, enhancing crystallinity and conversion efficiency.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Loss of energy

If conventional green phosphors are used, then the phosphor can be excited by blue LED, but the conversion efficiency is insufficient

Engineering Contradiction:
Improveconversion efficiencyVSAvoidlight emission effectiveness
Core Design Contradiction:
Loss of energyVSReliability

Solution Approach 1:

The patent applies parameter changes by precisely controlling the full width at half maximum (FWHM) of the diffraction peak corresponding to the (422) plane in the XRD pattern to be less than 0.18 degrees. This specific parameter control optimizes the crystallinity and phase purity of the SrGa2S4:Eu phosphor, thereby improving its conversion efficiency from blue LED excitation to green light emission. The narrow FWHM indicates high crystallinity which directly enhances the phosphor's optical performance and energy conversion efficiency.

Inventive Principle:
Principle #35Parameter changes

2Stability of the object's composition

If the full width at half maximum of the diffraction peak is reduced, then crystallinity is improved, but manufacturing precision requirements increase

Engineering Contradiction:
ImprovecrystallinityVSAvoiddiffraction peak width control
Core Design Contradiction:
Stability of the object's compositionVSManufacturing precision

Solution Approach 1:

The patent establishes a specific parameter range for the FWHM of the (422) diffraction peak (less than 0.18 degrees) as a critical quality indicator. By setting this precise parameter threshold, the patent enables manufacturers to control crystallinity through measurable and controllable parameters during the firing process, transforming the abstract concept of crystallinity into a quantifiable manufacturing specification.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent implements a feedback mechanism by using XRD pattern analysis, specifically the FWHM of the (422) peak, as a quality control metric. Manufacturers can measure the diffraction peak width and adjust firing conditions accordingly to achieve the target FWHM value, creating a closed-loop control system that ensures consistent high crystallinity while managing manufacturing precision requirements.

Inventive Principle:
Principle #23Feedback

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The phosphor achieves high conversion efficiency, with absorptance, internal quantum efficiency, and external quantum efficiency improved, producing green light with high color purity and a wide color gamut when used in illumination devices.

Implementation Method 1

A SrGa2S4:Eu (hereinafter, written as SGS) phosphor is attracting attention as a green light emitting phosphor to be excited by a blue LED

Methodology Applied
Scientific EffectPhotoluminescence: Photoluminescence

Implementation Method 2

when a full width at half maximum of a diffraction peak corresponding to a (422) plane in an XRD pattern is less than a predetermined value

Methodology Applied
Scientific EffectX-ray diffraction: X-Ray

Implementation Method 3

full width at half maximum of a diffraction peak corresponding to a (422) plane in an XRD pattern

Methodology Applied
Scientific EffectDiffraction: Diffraction

Data Source

PatentEP3048157B1Green phosphor and production method therefor, phosphor sheet, and illumination device
Publication Date: 2020.06.03 DEXERIALS CORP
  • EP3048157B1 patent drawingFigure 1
  • EP3048157B1 patent drawingFigure 2(A)~2(D)
  • EP3048157B1 patent drawingFigure 3~4

AI summary

Provided is a green phosphor having high conversion efficiency. The green phosphor is represented by the composition formula (Sr1-yCay)1-xGa2S4:Eux (0.03 ≤ x ≤ 0.20 and 0 &lt; y ≤ 1). A full width at half maximum of a diffraction peak corresponding to a (422) plane in an XRD pattern is less than 0.18.