Acylation Process for Starch Viscosity Control

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

The physical properties of acylated polymer compositions, such as acylated starch, are difficult to control in the acylation process, making it challenging to produce acylated polymer compositions with superior properties for applications like inks, varnishes, and pharmaceutical excipients.

Innovation Solution

A process involving pre-treatment of amylose and/or amylopectin with an aqueous phase containing an acid with a pKa of 4.8 or less and an enzyme, followed by reaction with an acylating agent, and subsequent treatment with another acid in the presence of water to control viscosity and degree of substitution, achieving acylated polymer compositions with specific viscosity and ethanol tolerance.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional acylation process is used, then acylated polymer composition is produced, but physical properties are difficult to control

Engineering Contradiction:
Improvecontrol of physical propertiesVSAvoidprocess complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The starch is pre-treated with an aqueous phase containing acid and enzyme before acylation to modify its structure and properties. This preliminary action enables better control of physical properties (viscosity, ethanol tolerance) in the final acylated product by preparing the polymer in a more reactive and controllable state prior to the main acylation reaction.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The invention controls physical properties by adjusting multiple parameters including acid type and concentration, enzyme type and amount, reaction temperature, reaction time, and acylating agent conditions. These parameter changes allow precise control over viscosity and ethanol tolerance of the acylated starch product.

Inventive Principle:
Principle #35Parameter changes

2Manufacturing precision

If pre-treatment with acid and enzyme is applied, then physical properties are controlled, but process steps increase

Engineering Contradiction:
Improveviscosity controlVSAvoidnumber of process steps
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The pre-treatment step combines acid modification and enzymatic treatment in a single aqueous phase treatment process. This merging of multiple functions (swelling, partial hydrolysis, and enzymatic modification) into one step achieves viscosity control without proportionally increasing process complexity.

Inventive Principle:
Principle #5Merging (Combining)

3Manufacturing precision

If pre-treatment with acid and enzyme is applied, then physical properties are controlled, but production time increases

Engineering Contradiction:
Improveethanol tolerance controlVSAvoidproduction time
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The acylation process is conducted in periodic stages: pre-treatment phase (acid and enzyme application), main acylation phase, and post-treatment phase (acid treatment). This periodic action allows each stage to be optimized for its specific function while maintaining overall production efficiency and achieving precise ethanol tolerance control.

Inventive Principle:
Principle #19Periodic action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process effectively controls the physical properties of acylated polymer compositions, resulting in products with viscosity of 50 mPas or greater and ethanol tolerance of 60% or less, suitable for various industrial applications.

Implementation Method 1

The pre-treatment step in the process allows for efficient swelling of the polymer composition

Methodology Applied
Scientific EffectSwelling:

Implementation Method 2

treating the starch before acylation with an aqueous phase comprising one additive chosen from the group consisting of at least one acid A having a pKa of equal to or less than 4.8 at 25° C. and an enzyme

Methodology Applied
Scientific EffectEnzyme action: Enzyme

Implementation Method 3

reacting the pre-treated polymer composition with an acylating agent to provide an acylated polymer composition comprising amylose and/or amylopectin

Methodology Applied
Scientific EffectAcylation reaction: Chemical Bonding

Implementation Method 4

treating the acylated polymer with at least one acid A′ with a pKa of equal to or less than 4.8 at 25° C., in the presence of water

Methodology Applied
Scientific EffectAcid treatment:

Data Source

PatentUS11041024B2Acylation process
Publication Date: 2021.06.22 SOLVAY ACETOW GMBH(DE)

AI summary

A process for the manufacture of an acylated polymer composition including amylose and/or amylopectin, including a pre-treatment step in the presence of an acid and a hydroxycarboxylic acid, subsequent acylation and, preferably, a post-treatment step with an acid. The products obtained are useful as additives in inks, varnishes, lacquers, coatings, thickeners, adhesives or binders.