Starch-Based Adhesive Fast Curing via Binary Crosslinking

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Solution Overview

Problem

Starch-based adhesives for particleboards have long curing times and low curing efficiency, making them unsuitable for modern particleboard production due to high viscosity and lack of thermosetting properties, which hinders their application in high-temperature hot-pressing processes.

Innovation Solution

A high-temperature fast-curing starch-based adhesive is developed by using a crosslinking monomer that does not self-crosslink at room temperature, combined with a binary crosslinking agent, to ensure rapid curing and improved thermosetting and water resistance, with specific control over acid hydrolysis time, initiator addition, crosslinking monomer amount, and reaction temperature to achieve low viscosity and efficient bonding.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If traditional starch-based adhesive is used, then it is environmentally friendly and low-cost, but it has high viscosity, cannot bear high temperature, lacks thermosetting property, and is poor in water resistance

Engineering Contradiction:
Improveenvironmental friendliness and costVSAvoidwater resistance and thermosetting property
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent combines starch with acrylic acid and crosslinking agents to create a composite adhesive system. The starch provides environmental friendliness and cost-effectiveness, while the acrylic acid and crosslinking agents contribute thermosetting properties and improved water resistance, resolving the contradiction between eco-friendliness and performance reliability.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent modifies the chemical parameters of starch through acid hydrolysis and grafting reactions. By controlling the degree of substitution and molecular weight distribution, the adhesive achieves both low viscosity for easy application and high crosslinking density for superior water resistance and thermosetting properties.

Inventive Principle:
Principle #35Parameter changes

2Ease of operation

If traditional starch-based adhesive is used, then it maintains low viscosity, but it has long curing time and low curing efficiency

Engineering Contradiction:
Improvelow viscosityVSAvoidcuring efficiency
Core Design Contradiction:
Ease of operationVSProductivity

Solution Approach 1:

The patent introduces crosslinking agents as intermediaries that facilitate rapid curing. These agents act as catalysts that accelerate the crosslinking reaction between starch and acrylic acid groups, enabling the adhesive to maintain low viscosity during application while achieving fast curing and high productivity during the bonding process.

Inventive Principle:
Principle #24Intermediary (Mediator)

3Ease of operation

If acid hydrolysis time is extended to reduce viscosity, then viscosity decreases, but excessive starch disintegration occurs leading to low monomer grafting efficiency

Engineering Contradiction:
ImproveviscosityVSAvoidmonomer grafting efficiency
Core Design Contradiction:
Ease of operationVSManufacturing precision

Solution Approach 1:

The patent performs preliminary acid hydrolysis of starch to control the molecular weight and reduce viscosity before the grafting reaction with acrylic acid. By optimizing the hydrolysis time and acid concentration, the starch achieves suitable viscosity while maintaining sufficient structural integrity for efficient monomer grafting, preventing both excessive viscosity and starch disintegration.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The adhesive achieves a curing time of 70 seconds or less, significantly improving production efficiency while meeting the performance requirements for P2 type particleboards, including excellent water resistance and bonding strength, as demonstrated by thickness swelling rates and adhesive curing time tests.

Implementation Method 1

a binary crosslinking agent matched with the crosslinking monomer is added before use to be quickly crosslinked with the crosslinking monomer at high temperature

Methodology Applied
Scientific EffectCrosslinking: Chemical Bonding

Implementation Method 2

ensure better thermosetting property and water resistance as well as faster curing speed

Methodology Applied
Scientific EffectThermosetting: Chemical Bonding

Implementation Method 3

the control of acid hydrolysis time, initiator addition amount, crosslinking monomer addition amount, and reaction temperature in three key steps

Methodology Applied
Scientific EffectAcid hydrolysis: Hydrolysis

Data Source

PatentUS11981834B2High-temperature fast-curing starch-based adhesive for particleboards and preparation method thereof
Publication Date: 2024.05.14 JIANGNAN UNIV

AI summary

The present disclosure discloses a high-temperature fast-curing starch-based adhesive for particleboards and a preparation method thereof, belonging to the technical field of adhesive preparation. The low viscosity of the starch-based adhesive is ensured by selecting a crosslinking monomer which does not self-crosslink in a reaction process in the present disclosure, and a binary crosslinking agent matched with the crosslinking monomer is added before use to be quickly crosslinked with the crosslinking monomer at high temperature so as to ensure better thermosetting property and water resistance as well as faster curing speed of the starch-based adhesive at the same time, which meets the requirements of the particleboards for the adhesive, solves the problem of long curing time of the existing starch-based adhesives at high temperatures, further shortens the curing time of the starch-based adhesives to about 60 s, and improves the production efficiency of the particleboards.