Starch-Based Flocculant Composition for Fracturing Flowback Treatment

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Solution Overview

Problem

Current treatments for fracturing flowback fluid, particularly using polyaluminum chloride and polyacrylamide, are inefficient and environmentally harmful due to poor flocculation effects and slow biodegradation of polyacrylamide, leading to challenges in managing the high viscosity, salt content, and emulsification of this waste fluid.

Innovation Solution

A flocculant prepared by dissolving gelatinized starch with unsaturated polyethylene glycol, unsaturated short-chain carboxylic acid, and hydroxyethyl methacrylate phosphate under a nitrogen atmosphere, followed by reaction and purification, which enhances flocculation and biodegradability.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If polyacrylamide is used as flocculant, then flocculation effect is improved, but biodegradation rate deteriorates

Engineering Contradiction:
Improveflocculation effectVSAvoidbiodegradation rate
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent uses composite materials by combining gelatinized starch (natural polymer) with grafted acrylamide and acrylic acid units. This creates a semi-synthetic flocculant that maintains the biodegradability of starch while incorporating the effective flocculation properties of acrylamide-based polymers. The starch backbone provides biodegradability pathways while the grafted chains deliver flocculation performance.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent changes the molecular structure parameters by controlling the grafting degree and molecular weight of the flocculant. By optimizing these parameters, the flocculant achieves effective flocculation performance while maintaining a molecular structure that is more amenable to biodegradation compared to conventional high molecular weight polyacrylamide.

Inventive Principle:
Principle #35Parameter changes

2Ease of manufacture

If polyaluminum chloride is used as flocculant, then preparation simplicity is improved, but flocculation effect deteriorates

Engineering Contradiction:
Improvepreparation simplicityVSAvoidflocculation effect
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent changes the chemical composition parameters by using natural starch as the base polymer and grafting acrylamide and acrylic acid onto it. This approach maintains relative simplicity in raw material acquisition while achieving superior flocculation performance through controlled chemical modification, producing a semi-synthetic polymer with optimized properties.

Inventive Principle:
Principle #35Parameter changes

3Object-generated harmful factors

If conventional starch-based flocculant is used, then biodegradability is improved, but solubility and dissolution rate deteriorate

Engineering Contradiction:
ImprovebiodegradabilityVSAvoidsolubility and dissolution rate
Core Design Contradiction:
Object-generated harmful factorsVSEase of manufacture

Solution Approach 1:

The patent changes the physical and chemical parameters of starch by gelatinization (heating to 60-80°C for 30-120 minutes) and chemical grafting. These modifications improve solubility and dissolution rate while maintaining the starch backbone that ensures biodegradability. The gelatinization process opens the starch structure, and grafting introduces hydrophilic groups that enhance water solubility.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The flocculant effectively reduces turbidity, color, suspended matters, COD, and total iron in fracturing flowback fluid while minimizing environmental impact through biodegradability and simple preparation.

Implementation Method 1

adding starch into water, uniformly stirring, heating to a gelatinization temperature (usually 60-80° C.), keeping the temperature for 30-120 min

Methodology Applied
Scientific EffectGelatinization: Gel

Implementation Method 2

adding unsaturated polyethylene glycol, unsaturated short-chain carboxylic acid, hydroxyethyl methacrylate phosphate and an initiator under a nitrogen atmosphere for reaction

Methodology Applied
Scientific EffectPolymerization: Chemical Bonding

Implementation Method 3

The flocculant effectively reduces turbidity, color, suspended matters, COD, and total iron in fracturing flowback fluid

Methodology Applied
Scientific EffectFlocculation: Flocculation

Data Source

PatentUS20250346509A1Flocculant for treating fracturing flowback fluid and preparation method therefor
Publication Date: 2025.11.13 SHINEON ENVIRONMENTS TECHNOLOGY SERVICES CO LTD

AI summary

Disclosed are a flocculant for treating fracturing flowback fluid and a preparation method therefor, which relate to oilfield sewage treatment. The method includes: in parts by weight, dissolving gelatinized starch in water, adding unsaturated polyethylene glycol, unsaturated short-chain carboxylic acid, hydroxyethyl methacrylate phosphate and an initiator under a nitrogen atmosphere for reaction for 3-8 h, and after the reaction is completed, separating and purifying to obtain a product. The flocculant for treating fracturing flowback fluid is prepared by a one-pot method, and the solvent is water, so that the preparation method is simple and has better environmental protection performance; meanwhile, the flocculant not only can reduce turbidity, color and suspended matters of the flowback fluid, but also can effectively reduce COD and total iron of the flowback fluid, and also can reduce the mineralization to a certain degree. The flocculant has good biodegradability and has less impact on the environment.