Stretchable Conductive Paste for Wearable Electronics

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Solution Overview

Problem

Conductive pastes used in stretchable electronic devices face issues with resistance increase and durability when subjected to repeated stretching, particularly with narrow wiring widths, due to insufficient crosslinking and heat resistance limitations in existing binder materials.

Innovation Solution

A conductive paste composition incorporating a polyurethane elastomer with a specific urethane group concentration and glass transition temperature, combined with silver particles and carbon materials, which allows for high repeated stretchability without the need for crosslinking agents and maintains conductivity even after extensive elongation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If a metal wire or metal foil is used to form an electrical wiring line, then the conductivity is high, but the stretchability is insufficient

Engineering Contradiction:
ImproveconductivityVSAvoidstretchability
Core Design Contradiction:
ReliabilityVSAdaptability or versatility

Solution Approach 1:

The patent changes the physical state and composition parameters by replacing traditional metal conductors with a conductive paste containing conductive particles (silver, carbon, etc.) dispersed in a specific binder resin system. This transformation enables the wiring line to achieve both high conductivity and stretchability by allowing the conductive particles to maintain electrical contact while the binder accommodates deformation.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite material system consisting of conductive particles (silver powder, carbon black, or carbon nanotubes) combined with a specially formulated binder resin (polyurethane or silicone rubber with specific molecular weight and glass transition temperature). This composite structure combines the electrical conductivity of metal particles with the elasticity of polymer binders, resolving the contradiction between conductivity and stretchability.

Inventive Principle:
Principle #40Composite materials

2Adaptability or versatility

If a corrugated wiring line is formed by placing metal wire or metal foil in a corrugated shape, then pseudo stretchability is achieved, but permanent plastic deformation occurs under excessive deformation

Engineering Contradiction:
ImprovestretchabilityVSAvoiddurability
Core Design Contradiction:
Adaptability or versatilityVSReliability

Solution Approach 1:

The patent changes the structural parameters by abandoning the corrugated geometry in favor of a smooth wiring line formed from conductive paste. The key parameter change is in the material composition - using a binder resin with specific glass transition temperature and molecular weight that provides inherent elasticity, allowing the wiring to stretch and recover without permanent deformation.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent replaces the durable but non-stretchable metal foil with a consumable conductive paste formulation that can be printed and cured to form a stretchable wiring line. This approach sacrifices the indefinite durability of metal but gains stretchability and durability under repeated deformation through the optimized polymer matrix.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Productivity

If the wiring width is reduced to 5 mm or less for device miniaturization, then the device size is reduced, but the resistance increase becomes significant during repeated stretching

Engineering Contradiction:
Improvedevice miniaturizationVSAvoidresistance stability
Core Design Contradiction:
ProductivityVSReliability

Solution Approach 1:

The patent optimizes multiple parameters including the binder resin molecular weight (10,000-1,000,000), glass transition temperature (-60°C to 0°C), and conductive particle concentration to achieve narrow wiring widths (5 mm or less) while maintaining stable resistance. The specific parameter range of the binder resin ensures sufficient elasticity and particle contact maintenance even in narrow wiring configurations.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies local quality optimization by ensuring uniform distribution of conductive particles within the binder resin matrix, creating consistent electrical properties throughout the narrow wiring line. The localized interaction between conductive particles and binder resin molecules ensures stable electrical contact at each point along the narrow wiring path.

Inventive Principle:
Principle #3Local quality

4Adaptability or versatility

If existing conductive paste compositions are used, then the wiring line has stretchability, but the resistance increases significantly after repeated stretching due to insufficient crosslinking

Engineering Contradiction:
ImprovestretchabilityVSAvoidrepeated durability
Core Design Contradiction:
Adaptability or versatilityVSReliability

Solution Approach 1:

The patent optimizes the chemical composition parameters of the binder resin, specifically selecting polyurethane or silicone rubber with controlled molecular weight (10,000-1,000,000) and glass transition temperature (-60°C to 0°C). These parameter specifications ensure sufficient crosslinking density and molecular chain flexibility, maintaining both stretchability and resistance stability after repeated deformation cycles.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates an optimized composite material system where the binder resin (polyurethane or silicone rubber) forms a crosslinked network that entraps conductive particles. This composite structure provides both the elasticity needed for stretching and the structural integrity to maintain particle contact and conductivity during repeated deformation, resolving the durability issue of existing formulations.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution enables the formation of stretchable conductive lines with reduced resistance increase and improved durability, suitable for wearable devices, by maintaining strong interactions between silver particles and the binder while allowing for fine line printing and high repeated stretchability without crosslinking, thus enhancing the usability of stretchable electronic components.

Implementation Method 1

maintaining strong interactions between silver particles and the binder

Methodology Applied
Scientific EffectAdhesion: Adhesive

Implementation Method 2

a stretchable conductor capable of forming an electric conductor having stretchability... elastomers such as stretchable urethane resin, natural rubber, synthetic rubber

Methodology Applied
Scientific EffectElasticity: Elasticity

Data Source

PatentUS11469010B2Conductive paste, stretchable conductor and electronic component using same, and clothes-type electronic device
Publication Date: 2022.10.11 TOYOBO CO LTD

AI summary

A stretchable conductor forming paste containing a conductive filler, a polyurethane elastomer having a glass transition temperature (Tg) of −60° C. to −10° C. and a urethane group concentration of 3000 to 4500 m equivalent/kg, and an organic solvent. Preferably, a total amount of components excluding the solvent is 100 parts by mass, a total of the conductive filler is 70 to 95 parts by mass, and an amount of the polyurethane elastomer is 5 to 30 parts by mass. The obtained paste is printed or coated and then dried to obtain a stretchable conductor, capable of forming a wiring line having good repeated stretchability.