Two-Stage Distillation for Styrene Depolymerization Feedstock Purity

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Existing styrene purification processes from styrenic compound depolymerization are complex and energy-intensive due to the high content of 'heavy' compounds and low ethylbenzene content in the feedstock, requiring rapid cooling and specific column designs to manage viscosity and polymerization.

Innovation Solution

A two-step distillation process involving a distillation column with direct feed at the bottom and subsequent separation into styrene-rich, ethylbenzene-rich, and heavy compound streams, utilizing internal walls and controlled reflux ratios to minimize polymerization and fouling, with integrated cooling to optimize energy use.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional distillation processes are used for styrene purification from depolymerization feedstock, then separation of heavy compounds is achieved, but energy consumption increases and process complexity increases

Engineering Contradiction:
Improvestyrene purityVSAvoidenergy consumption
Core Design Contradiction:
Manufacturing precisionVSUse of energy by stationary object

Solution Approach 1:

The distillation process is divided into two separate columns: a first distillation column that separates heavy compounds from styrene-rich feedstock, and a second distillation column that purifies styrene from ethylbenzene and other light compounds. This segmentation allows each column to be optimized for its specific separation task, reducing overall energy consumption compared to a single complex multi-column system.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The first distillation column performs preliminary separation by removing heavy compounds before the styrene enters the second purification column. This preliminary action prevents heavy compounds from interfering with the subsequent styrene-ethylbenzene separation, simplifying the overall process and reducing energy requirements for the critical purification step.

Inventive Principle:
Principle #10Preliminary action

2Manufacturing precision

If conventional distillation processes are used for styrene purification from depolymerization feedstock, then separation of heavy compounds is achieved, but the number of process steps increases

Engineering Contradiction:
Improvestyrene purityVSAvoidprocess complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The purification process is segmented into two functional columns: the first column handles heavy compound removal with a reboiler designed for high-temperature operation, while the second column handles styrene-ethylbenzene separation with a reboiler optimized for lower temperatures. This functional segmentation reduces process complexity by assigning specific tasks to dedicated units rather than using a single complex multi-column system.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The process utilizes parameter changes by operating the first distillation column at higher temperatures to vaporize and remove heavy compounds, then operating the second column at lower temperatures for gentle styrene-ethylbenzene separation. This parameter optimization reduces the need for additional process steps and equipment while achieving the required purity levels.

Inventive Principle:
Principle #35Parameter changes

3Reliability

If rapid cooling is applied to prevent styrene polymerization, then polymerization is inhibited, but process complexity increases

Engineering Contradiction:
Improvepolymerization preventionVSAvoidprocess complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The first distillation column performs preliminary separation of heavy compounds that would otherwise require rapid cooling to prevent polymerization. By removing these problematic compounds first through controlled distillation, the need for rapid cooling downstream is reduced, simplifying the overall process while maintaining polymerization prevention.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The process controls temperature parameters in the first distillation column to selectively vaporize heavy compounds while maintaining conditions that prevent styrene polymerization. This parameter optimization allows controlled separation without requiring additional rapid cooling equipment or steps.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process achieves high-purity styrene (>99.5%) with reduced energy consumption and minimized fouling, improving process efficiency and life cycle analysis.

Implementation Method 1

a separation step employing a distillation column fed at the bottom of the column by the purification process feed and producing at the top of the column an extract rich in light compounds, at the bottom a raffinate rich in heavy compounds

Methodology Applied
Scientific EffectDistillation: Distillation

Implementation Method 2

A separation step of the styrene-rich stream into at least one stream comprising mainly ethylbenzene, one stream comprising mainly styrene and one stream of heavy compounds

Methodology Applied
Scientific EffectDistillation: Distillation

Data Source

PatentEP4402117B1Method for purifying a feedstock resulting from a method for depolymerising styrene compounds
Publication Date: 2025.10.29 MICHELIN & CO (CIE GEN DES ESTAB MICHELIN)
  • EP4402117B1 patent drawingFigure 1~2
  • EP4402117B1 patent drawingFigure 3~4

AI summary

The invention relates to a method for purifying a feedstock resulting from a method for depolymerising styrene compounds, referred to as purification method feedstock, comprising at least one step of separation which produces an extract rich in light compounds, a raffinate rich in heavy compounds, and a styrene-rich stream, and a step of separation of the styrene-rich stream into at least a stream predominantly comprising ethylbenzene, a stream predominantly comprising styrene and a stream of heavy compounds.