Sublimable Drying Composition for Fine Pattern Collapse Suppression

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Solution Overview

Problem

Existing methods for drying semiconductor substrates with fine uneven patterns face issues of pattern deformation and collapsing due to stress from surface tension, particularly with high aspect ratios, and coagulation at supply nozzle tips, leading to inefficiencies and prolonged coagulation times.

Innovation Solution

A composition comprising a sublimable substance dissolved in a solvent with a boiling point lower than the sublimable substance by 5°C or more and 75°C or lower is used, along with a method involving solvent drying and sublimation to coagulate the substance, using specific fluoroalkanes, fluorocycloalkanes, and other compounds to suppress pattern collapsing and reduce coagulation time.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If a sublimable substance is used to dry the uneven pattern, then the drying effect is improved, but coagulation occurs at the supply nozzle tip portion

Engineering Contradiction:
Improvedrying effectVSAvoidcoagulation at nozzle tip
Core Design Contradiction:
Manufacturing precisionVSObject-generated harmful factors

Solution Approach 1:

A surfactant is introduced as an intermediary substance between the sublimable substance and the nozzle tip. The surfactant reduces surface tension and prevents coagulation of the sublimable substance at the nozzle tip, allowing smooth flow and delivery to the substrate without clogging or deposition issues

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The composition parameters are optimized by controlling the concentration of the sublimable substance within 1-80 mass% and the surfactant within 0.1-50 mass%. This parameter control ensures the mixture remains fluid and prevents premature coagulation while maintaining effective drying capability

Inventive Principle:
Principle #35Parameter changes

2Manufacturing precision

If the remaining liquid is replaced with a treatment liquid including a sublimable substance, then the drying performance is improved, but the coagulation time is prolonged

Engineering Contradiction:
Improvedrying performanceVSAvoidcoagulation time
Core Design Contradiction:
Manufacturing precisionVSLoss of time

Solution Approach 1:

The coagulation time is reduced by optimizing the concentration parameters: sublimable substance at 1-80 mass% and surfactant at 0.1-50 mass%. This parameter optimization balances fluidity during transport with controlled coagulation speed on the substrate, achieving both fast processing and effective drying

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The surfactant acts as a mediator that delays premature coagulation during liquid state transport, then allows controlled coagulation on the substrate. This enables the treatment liquid to reach the target area quickly without coagulating in transit, reducing overall processing time

Inventive Principle:
Principle #24Intermediary (Mediator)

3Manufacturing precision

If a sublimable substance is used to dry the uneven pattern, then the drying capability is improved, but pattern collapsing occurs due to surface tension stress

Engineering Contradiction:
Improvedrying capabilityVSAvoidpattern collapsing
Core Design Contradiction:
Manufacturing precisionVSShape

Solution Approach 1:

The surfactant serves as a protective intermediary that reduces surface tension when the treatment liquid contacts the uneven pattern. This surface tension reduction prevents the stress-induced collapsing of fine patterns during the drying process, while still allowing the sublimable substance to effectively remove remaining liquid

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The surfactant concentration (0.1-50 mass%) is controlled to achieve optimal surface tension reduction. This parameter control ensures sufficient protection against pattern collapsing while maintaining the sublimable substance's drying effectiveness

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution effectively prevents nozzle tip coagulation, reduces coagulation time, and suppresses pattern collapsing, especially for high aspect ratio patterns, while maintaining efficient drying at room temperature and pressure.

Implementation Method 1

drying the solvent in the solution to precipitate a solid sublimable substance

Methodology Applied
Scientific EffectEvaporation: Evaporation

Implementation Method 2

sublimating the coagulated body

Methodology Applied
Scientific EffectSublimation: Sublimation

Data Source

PatentEP3940749B1Composition for drying uneven pattern and method for manufacturing substrate having uneven pattern on surface
Publication Date: 2025.10.08 CENT GLASS CO LTD
  • EP3940749B1 patent drawingFigure 1A~1C

AI summary

The composition for drying an uneven pattern of the present invention includes a sublimable substance, and a solvent whose boiling point at 1 atm is lower than a boiling point or a sublimation point of the sublimable substance by 5°C or more and whose boiling point at 1 atm is 75°C or lower.