Subnanometer Carbon Coatings for Scratch-Resistant Infrared Glazing

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Solution Overview

Problem

Existing materials with infrared radiation-acting stacks suffer from insufficient mechanical strength, leading to defects such as corrosion, scratches, or tearing during processing, storage, and transportation, which affect aesthetics and optical performance, and conventional protective layers do not provide sufficient scratch resistance without altering optical properties.

Innovation Solution

A thin graphite-type carbon protective layer with less than 1 nm thickness, deposited by cathodic sputtering, is used to enhance scratch resistance without significantly changing optical properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional protective layers (titanium oxide, zinc-tin oxide) are used to protect the stack, then corrosion resistance is improved, but scratch resistance remains insufficient

Engineering Contradiction:
Improvecorrosion resistanceVSAvoidscratch resistance
Core Design Contradiction:
ReliabilityVSStrength

Solution Approach 1:

The patent combines multiple materials in a stack structure: a lower protective layer (titanium oxide, zinc-tin oxide) for corrosion protection, and an upper protective layer (amorphous carbon with sp2-sp3 hybridization) for scratch resistance. This composite approach allows each layer to fulfill its specific function, resolving the contradiction between corrosion resistance and scratch resistance.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

Different regions of the protective coating system are assigned different properties: the lower layer near the substrate provides chemical stability and corrosion resistance, while the upper exposed layer provides mechanical hardness and scratch resistance. This local differentiation of properties allows optimization for specific functions at different locations in the coating system.

Inventive Principle:
Principle #3Local quality

2Strength

If graphite carbon layers are used to improve scratch resistance, then mechanical strength is improved, but visible and infrared absorption increases significantly

Engineering Contradiction:
Improvescratch resistanceVSAvoidvisible and infrared absorption
Core Design Contradiction:
StrengthVSUse of energy by moving object

Solution Approach 1:

The patent changes the hybridization parameter of the carbon layer from pure sp2 (graphite, highly absorptive) to a mixture of sp2-sp3 (amorphous carbon, less absorptive). This parameter change reduces the absorption in visible and infrared ranges while maintaining scratch resistance, resolving the contradiction between mechanical strength and optical energy transmission.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The carbon layer is positioned specifically as the uppermost protective layer where scratch resistance is needed, while its amorphous sp2-sp3 structure ensures it does not significantly absorb visible and infrared radiation. This localized application with controlled properties resolves the contradiction between mechanical protection and optical performance.

Inventive Principle:
Principle #3Local quality

3Strength

If the carbon layer thickness is increased to improve protection, then scratch resistance is improved, but visible absorption increases

Engineering Contradiction:
Improvescratch resistanceVSAvoidvisible light transmission
Core Design Contradiction:
StrengthVSIllumination intensity

Solution Approach 1:

The patent optimizes the thickness parameter of the carbon layer to a specific range (0.5-5 nm) where it provides sufficient scratch resistance while maintaining high visible light transmission. This precise parameter control resolves the contradiction between mechanical protection and optical transparency.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The carbon layer thickness is kept minimal (just enough to provide scratch resistance) rather than thick, allowing visible light to pass through while still providing mechanical protection. This partial action approach resolves the contradiction by providing only the necessary amount of protection without excessive absorption.

Inventive Principle:
Principle #16Partial or excessive action

4Strength

If amorphous carbon layers (DLC) are used to improve scratch resistance, then mechanical strength is improved, but deposition complexity and cost increase due to requiring PECVD, laser ablation, or ion beam deposition

Engineering Contradiction:
Improvescratch resistanceVSAvoiddeposition process complexity
Core Design Contradiction:
StrengthVSDevice complexity

Solution Approach 1:

The patent extracts the essential property needed from complex DLC layers (amorphous carbon with sp2-sp3 hybridization) and achieves it through a simpler magnetron sputtering process. This extraction of the core functional property while removing the complex deposition requirements resolves the contradiction between scratch resistance and manufacturing simplicity.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent replaces complex deposition systems (PECVD, laser ablation, ion beam) with a simpler magnetron sputtering system to deposit the amorphous carbon layer. This substitution of the deposition mechanism maintains the protective properties while reducing equipment complexity and manufacturing cost.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The thin carbon layer significantly improves scratch resistance, maintaining low visible absorption and reducing friction, thus preventing defects during handling and processing, while being easy to deposit and cost-effective.

Implementation Method 1

The stack comprises, before treatment, a thin layer at least partially absorbing the laser radiation, which may be a carbon layer

Methodology Applied
Scientific EffectLaser radiation absorption: Absorption (EM radiation)

Implementation Method 2

deposited by cathodic sputtering

Methodology Applied
Scientific EffectCathodic sputtering: Sputtering

Data Source

PatentEP3237346B1Glazing comprising a carbon-based upper protective layer
Publication Date: 2025.10.15 SAINT GOBAIN VITRAGE SA

AI summary

The invention relates to a material comprising a transparent substrate coated with a stack of thin layers which act on infrared radiation, comprising at least one functional layer, characterised in that the stack comprises a carbon-based upper protective layer within which the carbon atoms are substantially in an sp2 hybridisation state, the protective layer being arranged above at least a portion of the functional layer and having a thickness less than 1 nm.