Sulfur Dioxide Electrolyte Lithium Cell Design

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Solution Overview

Problem

Conventional lithium-ion batteries face safety risks due to organic electrolytes, particularly in high-capacity applications, leading to increased costs, volume, and reduced energy density, and they are irreversibly damaged when discharged below 2.7 V, limiting their deep discharge capability.

Innovation Solution

A rechargeable lithium battery cell with a sulfur dioxide (SO2)-containing electrolyte and a porous positive electrode structure that allows lithium deposition, ensuring high ionic conductivity and preventing electronic short circuits, while using lithium tetrachloroaluminate as a conductive salt and incorporating a lithium dithionite layer to enhance safety and performance.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If organic electrolyte is used in lithium-ion cells, then ion mobility is achieved, but safety risks increase due to flammability

Engineering Contradiction:
ImprovesafetyVSAvoidflammability
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the chemical composition parameters of the electrolyte by replacing organic solvents with inorganic sulfur dioxide and using aluminum chloride-based conductive salts, fundamentally altering the electrolyte's physical and chemical properties to eliminate flammability while maintaining ionic conductivity

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates an inert chemical environment by using sulfur dioxide as the electrolyte solvent and aluminum chloride-based salts, which do not support combustion and are chemically stable, thereby eliminating the flammability hazard associated with organic electrolytes

Inventive Principle:
Principle #39Inert atmosphere (Inert environment)

2Reliability

If safety measures are added to reduce flammability risks, then safety is improved, but device complexity and costs increase

Engineering Contradiction:
ImprovesafetyVSAvoidsafety measures complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent converts the inherently safe chemical properties of inorganic sulfur dioxide and aluminum chloride into a beneficial electrolyte system that is non-flammable by design, eliminating the need for additional safety measures such as flame inhibitors, protective coatings, or complex monitoring systems required with organic electrolytes

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

3Ease of operation

If organic lithium-ion cells are discharged below 2.7 V, then deep discharge capability is achieved, but the cell is irreversibly damaged

Engineering Contradiction:
Improvedeep discharge capabilityVSAvoidcell durability
Core Design Contradiction:
Ease of operationVSReliability

Solution Approach 1:

The patent changes the electrochemical window and reaction mechanisms by using inorganic sulfur dioxide electrolyte with aluminum chloride-based salts, enabling the cell to withstand and reversibly operate at potentials below 2.7 V without the irreversible damage that occurs in organic electrolyte systems

Inventive Principle:
Principle #35Parameter changes

4Quantity of substance

If electrode thickness is increased to improve energy density, then energy density is improved, but ion transport efficiency decreases

Engineering Contradiction:
Improveenergy densityVSAvoidion transport speed
Core Design Contradiction:
Quantity of substanceVSSpeed

Solution Approach 1:

The patent changes the ionic conductivity parameter of the electrolyte by using inorganic sulfur dioxide with aluminum chloride-based conductive salts, which provide high ionic conductivity that enables efficient ion transport even through thicker electrodes, thereby allowing increased energy density without sacrificing ion transport efficiency

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The SO2-containing electrolyte and porous structure enable thicker electrodes, higher power density, improved safety, and deep discharge capability, achieving higher energy density and cycle life while maintaining cost-effectiveness.

Implementation Method 1

the mobility of the ions that cause the charge transport is at least partially due to the SO2

Methodology Applied
Scientific EffectIonic conduction: Conduction (electrical)

Implementation Method 2

the active cations, which react as a metal when charging the battery cell on the negative electrode by being incorporated into a host lattice or by alloying or by deposition

Methodology Applied
Scientific EffectElectrodeposition: Electrodeposition

Implementation Method 3

a porous positive electrode structure that allows lithium deposition

Methodology Applied
Scientific EffectAbsorption: Absorption (physical)

Data Source

PatentEP3069399B1Rechargeable electrochemical lithium cell with sulphur-dioxide containing electrolytes
Publication Date: 2021.03.24 FORTU NEW BATTERY TECH GMBH
  • EP3069399B1 patent drawingFigure 1~2

AI summary

The invention relates to a rechargeable, non-aqueous electrochemical battery cell which has a negative electrode, a positive electrode and a sulphur-dioxide containing electrolyte.