Superabsorbent Polymer Epoxy Crosslinking Rewetting

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Solution Overview

Problem

Superabsorbent polymers used in hygiene products face issues with rewetting and urine leakage phenomena due to pressure, which existing methods have not effectively addressed.

Innovation Solution

A method of preparing a superabsorbent polymer involving the crosslinking of acrylic acid-based monomers with a combination of first and second epoxy crosslinking agents, followed by surface modification, to enhance absorption properties and prevent rewetting.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If a superabsorbent polymer absorbs liquid, then absorption capacity is improved, but rewetting phenomenon occurs under pressure

Engineering Contradiction:
Improveabsorption capacityVSAvoidrewetting phenomenon
Core Design Contradiction:
Quantity of substanceVSObject-generated harmful factors

Solution Approach 1:

The patent changes the chemical parameters of the polymer by using specific epoxy equivalent weights (100-130 g/eq for first crosslinking agent, 130 g/eq or more for second crosslinking agent) and controlling the degree of neutralization of acrylic acid groups. These parameter changes create a polymer network that maintains absorption capacity while preventing rewetting under pressure.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite crosslinking system combining two different epoxy crosslinking agents with distinct molecular weight characteristics. This composite approach generates a dual-network structure that simultaneously provides high absorption capacity and resistance to pressure-induced rewetting, resolving the contradiction between these two properties.

Inventive Principle:
Principle #40Composite materials

2Object-generated harmful factors

If crosslinking density is increased to suppress rewetting, then rewetting resistance is improved, but liquid permeability deteriorates

Engineering Contradiction:
Improverewetting resistanceVSAvoidliquid permeability
Core Design Contradiction:
Object-generated harmful factorsVSDifficulty of detecting and measuring

Solution Approach 1:

The patent applies local quality by creating regions with different crosslinking densities through the use of two epoxy crosslinking agents with different molecular weights. The first crosslinking agent (100-130 g/eq) creates local networks that maintain permeability, while the second crosslinking agent (130 g/eq or more) creates regions that provide rewetting resistance, achieving both properties simultaneously.

Inventive Principle:
Principle #3Local quality

3Quantity of substance

If polymer volume is expanded by absorbing water, then absorption capacity is improved, but shape retention deteriorates

Engineering Contradiction:
Improveabsorption capacityVSAvoidshape retention
Core Design Contradiction:
Quantity of substanceVSShape

Solution Approach 1:

The patent performs preliminary crosslinking action before the polymer absorbs water and expands. By pre-establishing a robust crosslinked network structure using the two epoxy agents, the polymer is prepared to maintain its shape even when volume expands during water absorption, preventing collapse or deformation.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The resulting superabsorbent polymer exhibits improved water retention, liquid permeability, and reduced rewetting and urine leakage, maintaining a dry state even under pressure.

Implementation Method 1

an acrylic acid-based monomer having acidic groups which are at least partially neutralized and an internal crosslinking agent are crosslinked

Methodology Applied
Scientific EffectCrosslinking: Chemical Bonding

Implementation Method 2

the internal crosslinking agent includes a first epoxy crosslinking agent having an epoxy equivalent weight of 100 g/eq or more to less than 130 g/eq, and a second epoxy crosslinking agent having an epoxy equivalent weight of 130 g/eq or more

Methodology Applied
Scientific EffectEpoxy reaction: Chemical Bonding

Implementation Method 3

heating the base resin in the presence of a surface crosslinking agent to carry out surface modification of the base resin

Methodology Applied
Scientific EffectSurface crosslinking: Chemical Bonding

Implementation Method 4

heating the base resin in the presence of a surface crosslinking agent

Methodology Applied
Scientific EffectThermal heating: Heating

Implementation Method 5

A superabsorbent polymer (SAP) is a synthetic polymeric material capable of absorbing moisture from 500 to 1000 times its own weight

Methodology Applied
Scientific EffectAbsorption: Absorption (physical)

Implementation Method 6

superabsorbent polymers are required to exhibit high absorbency with respect to water, etc., and not to release the absorbed water even under an external pressure

Methodology Applied
Scientific EffectOsmosis: Osmosis

Data Source

PatentUS12257568B2Superabsorbent polymer and preparation method for the same
Publication Date: 2025.03.25 LG CHEM LTD

AI summary

A method of preparing a superabsorbent polymer includes preparing a base resin in which an acrylic acid-based monomer having acidic groups which are at least partially neutralized and an internal crosslinking agent are crosslinked; and heating the base resin in the presence of a surface crosslinking agent to carry out surface modification of the base resin, wherein the internal crosslinking agent includes a first epoxy crosslinking agent having an epoxy equivalent weight of 100 g/eq or more to less than 130 g/eq, and a second epoxy crosslinking agent having an epoxy equivalent weight of 130 g/eq or more. A superabsorbent polymer having improved rewetting property liquid permeability is also provided.