Tackifier-Free UV-Crosslinked Acrylate Adhesive for Rough Surfaces

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Existing pressure-sensitive adhesive tapes face challenges in achieving effective adhesion to rough surfaces and low surface energy surfaces, and they often leave residue upon removal, due to the difficulty in incorporating tackifiers into crosslinked networks and the adverse effects of tackifiers absorbing actinic radiation.

Innovation Solution

A crosslinkable composition comprising two different (meth)acrylate polymers, each with a weight average molecular weight of 50,000 to 500,000 Daltons, where at least one polymer contains pendant aromatic ketone groups that crosslink upon ultraviolet radiation exposure, forming a crosslinked composition free of tackifiers, which can be used as pressure-sensitive adhesives for rough and low surface energy surfaces.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If tackifiers are added to improve adhesion to rough and low surface energy surfaces, then adhesion performance is improved, but the adhesive leaves residue upon removal and absorbs actinic radiation adversely affecting crosslinking

Engineering Contradiction:
Improveadhesion performanceVSAvoidresidue formation and radiation absorption
Core Design Contradiction:
StrengthVSObject-generated harmful factors

Solution Approach 1:

The invention extracts and eliminates tackifiers from the adhesive composition entirely. Instead of using tackifiers to achieve adhesion to rough and low surface energy surfaces, the patent employs a tackifier-free (meth)acrylate polymer formulation that crosslinks upon UV exposure, achieving strong adhesion without the harmful residue-forming and radiation-absorbing properties of traditional tackifiers.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The invention changes the chemical composition parameters by using specific (meth)acrylate polymers with controlled molecular weights (50,000 to 500,000 Daltons) and incorporating UV-crosslinkable functional groups. This parameter change enables the adhesive to achieve strong initial tack and maintained adhesion without requiring tackifiers, thereby eliminating residue formation and UV radiation absorption issues.

Inventive Principle:
Principle #35Parameter changes

2Strength

If crosslinking is implemented to improve cohesive strength and adhesion, then structural integrity is improved, but incorporating tackifiers into crosslinked networks is difficult

Engineering Contradiction:
Improvecohesive strengthVSAvoiddifficulty of incorporating tackifiers into crosslinked networks
Core Design Contradiction:
StrengthVSEase of manufacture

Solution Approach 1:

The invention removes tackifiers from the formulation entirely, eliminating the compatibility and incorporation difficulties associated with integrating tackifiers into crosslinked networks. The crosslinking is achieved through UV-curable functional groups inherent to the (meth)acrylate polymer structure.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The invention uses composite (meth)acrylate polymer formulations containing multiple polymer components with different molecular weights and UV-crosslinkable functional groups. This composite approach achieves both strong cohesive strength through crosslinking and ease of manufacture by avoiding the complex integration of tackifiers into the crosslinked network.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The crosslinked composition demonstrates enhanced adhesion to various surfaces, including rough surfaces and low surface energy surfaces, and can be cleanly removed without leaving residue, as it forms a robust network without the limitations of tackifiers.

Implementation Method 1

At least one of the (meth)acrylate polymers contains pendant aromatic ketone groups that upon exposure to ultraviolet radiation, result in the formation of crosslinks within the polymeric material

Methodology Applied
Scientific EffectPhotopolymerization: Photopolymerisation

Data Source

PatentUS11168164B2Crosslinkable and crosslinked compositions
Publication Date: 2021.11.09 3M INNOVATIVE PROPERTIES CO

AI summary

Crosslinkable compositions, crosslinked compositions, articles containing these compositions, and methods of making the articles are provided. The crosslinkable compositions, which include two (meth)acrylate polymers, are used to form the crosslinked compositions upon exposure to ultraviolet radiation. The crosslinkable and crosslinked compositions are free or substantially free of tackifiers. The crosslinked compositions can function as pressure-sensitive adhesives. The crosslinkable compositions are well suited for use with hot melt processing methods.