Tar Reformer Catalyst Regeneration via Gas Recycling

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Solution Overview

Problem

Catalyst deactivation and high energy consumption in tar reformers due to carbon coke and dust buildup, which requires controlled high-temperature oxidative burn-off and substantial steam consumption, posing challenges in maintaining catalyst performance and efficiency.

Innovation Solution

A process involving a main gas stream with controlled oxygen content and temperature, recycled to control temperature development and reduce energy consumption, using a flue gas with natural steam content instead of dedicated steam generation, and adjusting oxygen content through additional oxidant gas streams to manage carbon combustion effectively.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If high-temperature oxidative burn-off is used to remove carbon coke and dust from catalyst, then catalyst performance is restored, but temperature control becomes difficult and energy consumption increases

Engineering Contradiction:
Improvecatalyst performanceVSAvoidtemperature control
Core Design Contradiction:
ReliabilityVSTemperature

Solution Approach 1:

The patent implements a feedback control system where the gas stream exiting the reformer is recycled back to the inlet. This recycle stream acts as a feedback mechanism that automatically modulates the oxygen and temperature conditions within the reformer, preventing temperature runaways while maintaining effective carbon removal and catalyst regeneration

Inventive Principle:
Principle #23Feedback

Solution Approach 2:

The patent changes the oxygen content parameter by blending the recycled oxygen-depleted gas with fresh gas streams. This parameter adjustment allows precise control of combustion intensity during catalyst regeneration, enabling effective carbon coke removal while maintaining safe temperature levels

Inventive Principle:
Principle #35Parameter changes

2Reliability

If high-temperature oxidative burn-off is used to remove carbon coke and dust from catalyst, then catalyst performance is restored, but energy consumption increases

Engineering Contradiction:
Improvecatalyst performanceVSAvoidenergy consumption
Core Design Contradiction:
ReliabilityVSUse of energy by moving object

Solution Approach 1:

The system uses its own output stream (oxygen-depleted gas) as part of its input, creating a self-regulating cycle. The heat generated by carbon combustion is retained within the system through recycling, reducing the need for external energy input while maintaining effective regeneration temperatures

Inventive Principle:
Principle #25Self-service

Solution Approach 2:

The patent converts the harmful exothermic combustion reaction into a beneficial heat source. The heat normally considered a risk for temperature runaway is instead utilized to maintain regeneration temperatures, reducing external energy requirements while the recycle system prevents overheating

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

3Reliability

If substantial steam consumption is used for catalyst regeneration, then carbon combustion is effective, but operational costs increase

Engineering Contradiction:
Improvecatalyst regeneration effectivenessVSAvoidsteam consumption
Core Design Contradiction:
ReliabilityVSLoss of substance

Solution Approach 1:

The gas stream performs multiple functions simultaneously: it provides oxygen for carbon combustion, serves as a heat transfer medium, and acts as a diluent to control reaction intensity. This multi-functionality eliminates the need for dedicated steam injection while achieving effective catalyst regeneration

Inventive Principle:
Principle #6Universality (Multi-functionality)

Solution Approach 2:

The patent changes from steam-based regeneration to oxygen-controlled combustion using recycled gas. This parameter change in the regeneration medium eliminates substantial steam consumption while maintaining effective carbon removal through controlled oxidative burn-off

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach effectively controls temperature and reduces energy consumption, prolonging catalyst life and minimizing the risk of temperature runaways while reducing steam usage and operational costs.

Implementation Method 1

controlled high-temperature oxidative burn-off

Methodology Applied
Scientific EffectOxidative combustion: Combustion

Implementation Method 2

regeneration of a catalyst within a tar reformer

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 3

The temperature of the main gas stream at the inlet is controlled to be within the range from about 500°C to about 1000°C

Methodology Applied
Scientific EffectThermal heating: Heating

Implementation Method 4

recycling at least a part of the oxygen depleted gas exiting from the tar reformer back into the main gas stream upstream the tar reformer

Methodology Applied
Scientific EffectGas recycling: Convection

Data Source

PatentEP3234069B1Process and system for regeneration of tar reformer catalyst
Publication Date: 2020.09.09 HALDOR TOPSOE AS
  • EP3234069B1 patent drawingFigure 1
  • EP3234069B1 patent drawingFigure 2
  • EP3234069B1 patent drawingFigure 3

AI summary

The invention relates to a catalyst regeneration process for a tar reforming catalyst within a catalyst bed in a tar reformer. The process comprises the steps of: -Admitting a main gas stream with controlled temperature and oxygen content to an inlet into the tar reformer; -Passing the main gas stream through the catalyst bed to form an oxygen depleted gas stream; -Exiting the oxygen depleted gas stream from the tar reformer; and -Recycling at least a part of the oxygen depleted gas stream exiting from the tar reformer back into said main gas stream upstream said tar reformer. The temperature of said main gas stream at the inlet is controlled to be within the range from about 500˚C to about 1000˚C.