Thermal Storage System Crystallization Control via Two-Phase Solvent

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Solution Overview

Problem

Thermal storage systems using Phase Change Materials (PCMs) face challenges with supercooling and slow crystallization speeds, particularly with polyols like xylitol and sorbitol, which hinder efficient heat storage and release due to their strong propensity to supercooling, making it difficult to control crystallization and thus limiting their implementation in large-scale applications.

Innovation Solution

A Thermal Storage System (TSS) that includes a vessel with a circulation system and a device for controlling crystallization by injecting a two-phase solvent into the PCM, where the solvent changes state from liquid to gas, generating agitation and accelerating crystallization, and is evacuated to manage pressure and recycle the solvent, thereby enhancing crystallization speed and control.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If polyols are used as PCM, then enthalpy of change of state is improved, but crystallization speed deteriorates

Engineering Contradiction:
Improveenthalpy of change of stateVSAvoidcrystallization speed
Core Design Contradiction:
Quantity of substanceVSSpeed

Solution Approach 1:

Nucleation agents are introduced as intermediary substances that facilitate the crystallization process. These agents provide predefined nucleation sites that trigger and accelerate crystal formation in polyols, solving the slow crystallization issue while preserving the high enthalpy advantage of polyol PCMs.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The crystallization process is accelerated by changing physical parameters such as applying mechanical agitation, ultrasonic treatment, or controlled cooling rates. These parameter changes overcome the natural slow crystallization tendency of polyols while maintaining their high enthalpy of change of state.

Inventive Principle:
Principle #35Parameter changes

2Object-affected harmful factors

If polyols are used as PCM, then non-toxicity is improved, but supercooling propensity worsens

Engineering Contradiction:
Improvenon-toxicityVSAvoidsupercooling propensity
Core Design Contradiction:
Object-affected harmful factorsVSReliability

Solution Approach 1:

Nucleation agents serve as mediators that prevent supercooling by providing nucleation sites. These agents are carefully selected to be compatible with the non-toxic nature of polyols, ensuring that the ecological advantages are maintained while reliability is improved.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

Nucleation agents are pre-added to the polyol PCM before operation. This preliminary action ensures that nucleation sites are already present when cooling occurs, preventing supercooling from happening and ensuring reliable crystallization at the expected temperature.

Inventive Principle:
Principle #10Preliminary action

3Speed

If nucleation agents are added to accelerate crystallization, then crystallization speed is improved, but device complexity worsens

Engineering Contradiction:
Improvecrystallization speedVSAvoiddevice complexity
Core Design Contradiction:
SpeedVSDevice complexity

Solution Approach 1:

The nucleation agents are incorporated directly into the PCM material itself, allowing the system to self-trigger crystallization without requiring external complex devices. The PCM contains its own crystallization catalyst, eliminating the need for separate nucleation device systems.

Inventive Principle:
Principle #25Self-service

4Reliability

If mechanical agitation is applied to trigger crystallization, then crystallization control is improved, but energy consumption worsens

Engineering Contradiction:
Improvecrystallization controlVSAvoidenergy consumption
Core Design Contradiction:
ReliabilityVSUse of energy by moving object

Solution Approach 1:

Nucleation agents act as intermediaries that enable crystallization to start with minimal or no mechanical agitation. The nucleation sites provided by these agents allow crystallization to proceed spontaneously or with very light stirring, dramatically reducing the energy required compared to systems requiring intensive mechanical agitation.

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach significantly improves the crystallization speed and control of PCMs, enabling more efficient heat storage and release, overcoming the limitations of supercooling and enhancing the performance of thermal storage systems.

Implementation Method 1

injecting a two-phase solvent into the PCM (2), in the liquid state, in the lower part of the tank (1), and the evacuation of the solvent in the gaseous state in the upper part of the tank (1)

Methodology Applied
Scientific EffectPhase change: Phase Change

Implementation Method 2

The solvent is two-phase so as to change state on contact with the PCM having stored heat. In this way, the addition of two-phase solvent in the MCP contributes to favorably modifying the properties of the MCP and therefore accelerating the rate of crystallization while allowing the heating of the solvent introduced in the liquid state in contact with the MCP. The increase in the temperature of the solvent in contact with the MCP causes it to boil, generating bubbling of the solvent in the MCP, thus triggering the crystallization of the MCP.

Methodology Applied
Scientific EffectEvaporation: Evaporation

Implementation Method 3

A Thermal Storage System (TSS) that includes a vessel with a circulation system and a device for controlling crystallization

Methodology Applied
Scientific EffectHeat transfer: Conduction (thermal)

Data Source

PatentEP3489608B1Thermal storage system with phase change material and a device for controlling crystallization
Publication Date: 2020.08.12 ROQUETTE FRERES SA
  • EP3489608B1 patent drawingFigure 1~2
  • EP3489608B1 patent drawingFigure 3~4
  • EP3489608B1 patent drawingFigure 5~6

AI summary

The present invention relates to a Thermal Storage System (TSS) using a Phase Change Material (PCM) (2) comprising a tank (1) for containing a PCM (2), and a circulation system immersed in the tank (1) for circulating a heat transfer fluid from an external heat transfer fluid circulation network. The system is characterized in that it includes a device for controlling the crystallization of the PCM, comprising: an injection module configured to inject a two-phase solvent in liquid form into the lower part of the tank (1), and an evacuation module configured to evacuate the two-phase solvent in gaseous form into the upper part of the tank, opposite the lower part. All TSSs whose PCMs have issues with supercooling and slow crystallization rates are likely to be relevant to the invention.The present invention will find application in urban, rural, or industrial heating and/or cooling networks, as well as in solar energy storage. The invention may also find applications in housing, off-grid thermal transport (trucks, boats, etc.), and the thermal management of embedded systems.