Thermally Debondable Primer Composition for Adhesive Disassembly

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Solution Overview

Problem

Existing adhesive bonds are difficult to disassemble without damaging the substrates, as mechanical removal methods are inefficient and chemical or thermal methods can be time-consuming and risk damaging the substrates.

Innovation Solution

A thermally debondable primer composition comprising polyether urethane methacrylate resin, (meth)acrylate monomers, thermally expandable thermoplastic microspheres, and a photoinitiator, which is cured via photo-curing and can be easily debonded by applying heat.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If adhesive bonds are designed to be strong for withstanding drop or impact events and wide temperature ranges, then adhesion strength is improved, but difficulty in disassembly increases

Engineering Contradiction:
Improveadhesion strengthVSAvoiddifficulty in disassembly
Core Design Contradiction:
StrengthVSEase of operation

Solution Approach 1:

The adhesive system is segmented into two distinct layers: a permanent adhesive layer that provides strong bonding, and a removable primer layer that facilitates disassembly. This segmentation allows each layer to perform its specific function independently - the permanent adhesive maintains strong adhesion while the removable primer enables easy removal through thermal expansion

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The removable primer layer acts as an intermediary between the substrate and the permanent adhesive layer. This intermediate layer can be selectively removed through thermal expansion of microspheres, allowing the permanent adhesive to remain intact while enabling disassembly of the bonded structure

Inventive Principle:
Principle #24Intermediary (Mediator)

2Ease of operation

If mechanical processes are used to remove adhesive, then disassembly is achieved, but substrate surfaces are damaged

Engineering Contradiction:
Improvedisassembly capabilityVSAvoidsubstrate damage
Core Design Contradiction:
Ease of operationVSObject-affected harmful factors

Solution Approach 1:

The removal function is extracted from the permanent adhesive layer and transferred to a separate removable primer layer. This allows the permanent adhesive to remain on the substrate without damage, while the primer layer is removed through controlled thermal expansion, preventing substrate damage that would occur with mechanical removal methods

Inventive Principle:
Principle #2Taking out (Extraction)

3Ease of operation

If chemicals or high temperature are applied to debond, then adhesive bonding is disrupted, but substrates are damaged and process becomes time-consuming

Engineering Contradiction:
Improvedebonding effectivenessVSAvoidsubstrate damage
Core Design Contradiction:
Ease of operationVSObject-affected harmful factors

Solution Approach 1:

The thermal expansion property is localized specifically to the removable primer layer through the incorporation of thermally expandable microspheres. This localized quality ensures that only the primer layer undergoes significant volume expansion and debonding when heated, while the permanent adhesive layer and substrates remain unaffected and undamaged

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The system utilizes parameter changes in the form of thermally expandable microspheres that undergo a dramatic volume increase (up to 200 times) when exposed to heat. This parameter change is confined to the removable primer layer, enabling controlled debonding without exposing the substrates to the harsh conditions required for traditional chemical or thermal debonding methods

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The primer composition effectively weakens the bond strength by at least 50% upon heat application, allowing for efficient debonding while maintaining optimal adhesion and mechanical properties, as demonstrated by the tensile lap shear strength tests.

Implementation Method 1

the thermally debondable primer composition is cured via photo-curing

Methodology Applied
Scientific EffectPhoto-curing: Photopolymerisation

Implementation Method 2

thermally expandable thermoplastic microspheres

Methodology Applied
Scientific EffectThermal expansion: Thermal Expansion

Data Source

PatentEP4538330A1A thermally debondable primer composition
Publication Date: 2025.04.16 HENKEL KGAA
  • EP4538330A1 patent drawingFigure 1~2
  • EP4538330A1 patent drawingFigure 3~4
  • EP4538330A1 patent drawingFigure 5

AI summary

The present invention relates to a thermally debondable primer composition comprising a polyether urethane methacrylate resin; two or more (meth)acrylate monomers; thermally expandable thermoplastic microspheres; and one or more photoinitiator.