Thermally-Responsive Record Material Using Non-Isocyanate Developers

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Solution Overview

Problem

Thermally-responsive record materials often rely on isocyanate compounds, which are environmentally unfriendly and hazardous, and lack effective alternatives for producing stable, non-reversible images resistant to fade or erasure.

Innovation Solution

A thermally-responsive record material system using 4,4'-diaminodiphenyl sulfone and/or 3,3'-diaminodiphenyl sulfone as non-phenolic developers in combination with leuco dyes and organic acids, eliminating the need for isocyanates and enhancing image intensity and stability.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Object-affected harmful factors

If isocyanate compounds are used in thermally-responsive record materials, then image formation capability is achieved, but environmental safety and health hazards worsen

Engineering Contradiction:
Improveenvironmental safetyVSAvoidimage stability
Core Design Contradiction:
Object-affected harmful factorsVSReliability

Solution Approach 1:

The patent removes isocyanate compounds from the thermally-responsive record material formulation, extracting the harmful substance while maintaining the core image formation functionality through alternative chemistry involving leuco dyes and phenolic developers

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The invention changes the chemical parameters of the developer material from isocyanate-based to phenolic-based compounds, fundamentally altering the reaction mechanism while achieving comparable or superior image stability and environmental safety

Inventive Principle:
Principle #35Parameter changes

2Reliability

If traditional phenolic developers are used, then image development is achieved, but image intensity and stability are insufficient

Engineering Contradiction:
Improveimage stabilityVSAvoidimage intensity
Core Design Contradiction:
ReliabilityVSIllumination intensity

Solution Approach 1:

The patent employs composite formulations combining specific phenolic developers with leuco dyes and optional additives like sulfur compounds, creating a synergistic system that achieves both high image intensity and superior stability

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The invention optimizes parameters including developer concentration, molecular structure of phenolic compounds, and reaction conditions to maximize image intensity while ensuring long-term stability and fade resistance

Inventive Principle:
Principle #35Parameter changes

3Reliability

If reversible image systems are used, then ease of erasure is achieved, but image permanence and reliability worsen

Engineering Contradiction:
Improveimage permanenceVSAvoidease of erasure
Core Design Contradiction:
ReliabilityVSEase of operation

Solution Approach 1:

The patent converts the typically harmful effect of permanent chemical bonding into a beneficial feature by designing a system where the phenolic-leuco dye reaction produces stable, non-reversible bonds that ensure image permanence, while the formulation still allows for controlled development

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The system produces high-intensity, non-reversible images that are resistant to fade and erasure, suitable for applications like barcodes, while being environmentally friendlier and safer than traditional isocyanate-based systems.

Implementation Method 1

basic colorless or lightly colored chromogenic material and acidic color developer material are contained in a coating on a substrate which, when heated to a suitable temperature, melts or softens to permit said materials to react, thereby producing a colored mark

Methodology Applied
Scientific EffectChemical reaction: Chemical Bonding

Implementation Method 2

when heated to a suitable temperature, melts or softens to permit said materials to react

Methodology Applied
Scientific EffectMelting: Melting

Data Source

PatentEP2969580B1Thermally-responsive record material
Publication Date: 2020.07.29 APPVION OPERATIONS INC
  • EP2969580B1 patent drawingFigure 1
  • EP2969580B1 patent drawingFigure 2
  • EP2969580B1 patent drawingFigure 3

AI summary

The invention describes a thermally-responsive record material substantially free of aromatic isocyanate. The record material comprises a support having provided thereon a heat-sensitive composition comprising a substantially colorless dye precursor comprising a fluoran; and a developer material selected from the group consisting of 4,4'-diaminodiphenylsulfone and 3,3'-diaminodiphenylsulfone, which upon being heated react with said dye precursor to develop color, and including a binder material. Optionally, one or more of an organic acid, a modifier compound, or magnesium stearate is included in the heat-sensitive composition. The modifier compound can be selected from the a fatty acid amide, preferably a saturated fatty acid amide such as an alkyl amide, a bis methylene alkyl amide, or a bis ethylene alkyl amide.