Thermoelectric Alloy Carburization for High Figure-of-Merit

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Solution Overview

Problem

Conventional thermoelectric materials have limited thermoelectric figure-of-merit, restricting their application in heat dissipation and efficiency, as they typically have a figure-of-merit around 1.0, which is not sufficient to replace compressors, and existing methods do not effectively enhance their properties.

Innovation Solution

A method involving a carburization process where a carburizing agent decomposes to generate active carbon atoms that diffuse into an oxidized thermoelectric alloy, composed of materials like germanium, tellurium, bismuth, and others, to improve thermoelectric properties by reducing thermal conductivity and increasing the power factor.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional thermoelectric materials are used, then the material can be applied in waste heat recovery, but the thermoelectric figure-of-merit is limited to about 1.0, restricting application scope and efficiency

Engineering Contradiction:
Improvethermoelectric figure-of-meritVSAvoidapplication scope
Core Design Contradiction:
ReliabilityVSAdaptability or versatility

Solution Approach 1:

The patent changes the chemical composition parameters by introducing carbon atoms into the thermoelectric alloy through carburization process. This parameter change transforms the material properties, achieving a thermoelectric figure-of-merit of about 2.0, which doubles the performance of conventional materials and enables broader applications including heat dissipation systems that previously required compressors

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite thermoelectric material by combining conventional thermoelectric alloy elements (such as Bi-Te, Pb-Te, or Si-Ge systems) with carbon atoms. This composite structure, achieved through the carburization process, integrates the beneficial properties of both the base alloy and carbon, resulting in improved thermoelectric performance and expanded application versatility

Inventive Principle:
Principle #40Composite materials

2Adaptability or versatility

If the thermoelectric figure-of-merit is increased to replace compressors for heat dissipation, then application scope expands, but conventional materials cannot achieve the required performance level

Engineering Contradiction:
Improveapplication scopeVSAvoidthermoelectric figure-of-merit
Core Design Contradiction:
Adaptability or versatilityVSReliability

Solution Approach 1:

The patent achieves the critical parameter change needed to enable compressor replacement applications by introducing carbon atoms into the thermoelectric alloy. This compositional modification increases the thermoelectric figure-of-merit to about 2.0, which is sufficient for heat dissipation applications that require high performance, thereby expanding the adaptability of thermoelectric materials to replace mechanical compressor systems

Inventive Principle:
Principle #35Parameter changes

3Ease of manufacture

If existing production methods are used, then the manufacturing process is simple, but the thermoelectric properties cannot be effectively enhanced

Engineering Contradiction:
Improvemanufacturing simplicityVSAvoidthermoelectric properties
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent modifies the manufacturing process parameters by implementing a carburization treatment step. This involves heating the thermoelectric alloy to appropriate temperatures and exposing it to a carbon-containing atmosphere, allowing carbon atoms to diffuse into the material. This parameter change in the manufacturing process effectively enhances the thermoelectric properties while maintaining reasonable manufacturing complexity

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent introduces a carburizing agent as an intermediary substance in the manufacturing process. This agent provides the carbon atoms needed for the carburization treatment, mediating between the external environment and the thermoelectric alloy. The intermediary approach allows for controlled introduction of carbon, effectively enhancing thermoelectric properties through a manageable manufacturing process

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method significantly enhances the thermoelectric figure-of-merit of the alloy, achieving values twice that of commercial alloys, thereby improving thermoelectric conversion efficiency and expanding application possibilities.

Implementation Method 1

A carburizing agent decomposes on heating to generate active carbon atoms during a carburization process

Methodology Applied
Scientific EffectThermal decomposition: Pyrolysis

Implementation Method 2

the active carbon atoms can diffuse into an as-melted thermoelectric alloy material

Methodology Applied
Scientific EffectDiffusion: Diffusion

Implementation Method 3

A starting material is provided and subjected to an oxidation process for producing an oxidized material composition

Methodology Applied
Scientific EffectOxidation: Oxidation

Data Source

PatentEP3640361B1Method for producing a thermoelectric alloy
Publication Date: 2023.03.01 NAT SUN YAT SEN UNIV
  • EP3640361B1 patent drawingFigure 1
  • EP3640361B1 patent drawingFigure 2A~2B
  • EP3640361B1 patent drawing

AI summary

The present invention relates to a thermoelectric alloy and a method for producing the same. A starting material is firstly provided, and an oxidation process is performed to the starting material to obtain an oxidized material composition. Then, the oxidized material composition and a carburizing agent are added into a quartz tube, and a sealing process is performed to the quartz tube. And then, the sealed quartz tube is subjected to a carburization process, thereby obtaining the thermoelectric alloy with excellent thermoelectric figure-of-merit.