Tin Oxide Electrode Composition for Glass Melting

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Solution Overview

Problem

Existing tin oxide-based electrodes for glass melting applications face challenges with low thermal stability, unsuitable electrical resistivities, and macroscopic internal cracks, making it difficult to form industrial-grade electrodes with improved mechanical and optical performance.

Innovation Solution

A tin oxide-based electrode composition with a majority component of SnO2, including additives such as CuO and ZnO in specific weight percentages, and a resistivity modifying species like Sb2O3, is used to form electrodes with enhanced stability and electrical properties, avoiding excessive CuO and ZnO content to prevent cracking.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Force

If higher amounts of CuO and ZnO are used to improve densification, then density improves, but thermal stability deteriorates and macroscopic internal cracks occur

Engineering Contradiction:
ImprovedensificationVSAvoidthermal stability
Core Design Contradiction:
ForceVSStability of the object's composition

Solution Approach 1:

The patent applies parameter changes by precisely controlling the amounts of CuO and ZnO additives within narrow ranges (CuO: 0.05-0.2%, ZnO: 0.2-1.55%) to achieve optimal densification while preventing thermal instability and macroscopic cracking. This quantitative parameter optimization resolves the contradiction between densification and thermal stability.

Inventive Principle:
Principle #35Parameter changes

2Force

If higher amounts of CuO and ZnO are used to improve densification, then density improves, but electrical resistivity becomes unsuitable (too high)

Engineering Contradiction:
ImprovedensificationVSAvoidelectrical resistivity
Core Design Contradiction:
ForceVSReliability

Solution Approach 1:

The patent uses parameter changes by optimizing the CuO and ZnO content within specific ranges to simultaneously achieve proper densification and suitable electrical resistivity. The controlled additive amounts prevent excessive resistivity while maintaining density, resolving this technical contradiction.

Inventive Principle:
Principle #35Parameter changes

3Force

If higher amounts of CuO and ZnO are used to improve densification, then density improves, but manufacturing precision deteriorates due to unstable firing shrinkage

Engineering Contradiction:
ImprovedensificationVSAvoidfiring shrinkage stability
Core Design Contradiction:
ForceVSManufacturing precision

Solution Approach 1:

The patent applies parameter changes by controlling CuO and ZnO within narrow ranges (0.05-0.2% CuO, 0.2-1.55% ZnO) to achieve stable firing shrinkage and consistent manufacturing precision while maintaining adequate densification. This resolves the contradiction between densification and manufacturing precision.

Inventive Principle:
Principle #35Parameter changes

4Stability of the object's composition

If incremental modifications to additive ratios are made to improve stability, then thermal stability improves, but electrical properties and density deteriorate

Engineering Contradiction:
Improvethermal stabilityVSAvoidelectrical properties
Core Design Contradiction:
Stability of the object's compositionVSReliability

Solution Approach 1:

The patent applies parameter changes by optimizing not just additive ratios but also absolute amounts within specific ranges (0.05-0.2% CuO, 0.2-1.55% ZnO, 0.7-1.2% Sb2O3). This comprehensive parameter optimization achieves thermal stability while maintaining suitable electrical properties and density, resolving the contradiction.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composition results in electrodes with high density, low porosity, and suitable electrical resistivity, free of macroscopic internal cracks, suitable for industrial-sized glass melting applications, offering improved thermal stability and corrosion resistance.

Implementation Method 1

the tin oxide-based compositions include various components that assist in densification

Methodology Applied
Scientific EffectSintering: Sintering

Implementation Method 2

a resistivity modifying species... within a range between about 0.5 wt% and about 1.5 wt%

Methodology Applied
Scientific EffectElectrical Resistance: Electrical Resistance

Data Source

PatentEP2377130B1Tin oxide-based electrode composition
Publication Date: 2014.04.30 SAINT GOBAIN CERAMICS & PLASTICS INC
  • EP2377130B1 patent drawingFigure 1~2
  • EP2377130B1 patent drawingFigure 3~4
  • EP2377130B1 patent drawingFigure 5~6

AI summary

A tin oxide-based electrode formed from a composition including a majority component comprising tin-oxide (SnO2), and additives comprising CuO, ZnO, and a resistivity modifying species. The total amount of CuO and ZnO is not greater than about 0.3 wt%, and the ZnO is present in an amount within a range between about 0.1 wt% and about 0.19 wt%.