Tin Perovskite Silicon Tandem Solar Cells

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Solution Overview

Problem

The challenge in solar cell technology is to achieve long-term stability and efficient energy conversion while addressing the toxicity of lead-based perovskite materials and the complexity of silicon semiconductor connections, particularly in tandem solar cells, which are essential for cost-effective and environmentally friendly energy production.

Innovation Solution

The development of a non-toxic tin perovskite/silicon thin-film tandem solar cell structure, where a tin-based perovskite layer is formed on a crystalline silicon thin-film, utilizing a eutectic alloy and oxidized metal layers to create a tunnel recombination junction, facilitating efficient energy transfer and reducing manufacturing costs.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Power

If lead-based perovskite materials are used to achieve high conversion efficiency, then power conversion efficiency is improved, but toxicity increases

Engineering Contradiction:
Improvepower conversion efficiencyVSAvoidtoxicity
Core Design Contradiction:
PowerVSObject-affected harmful factors

Solution Approach 1:

The patent changes the chemical composition parameter of perovskite materials by replacing toxic lead (Pb) with non-toxic alternatives such as tin (Sn), germanium (Ge), or bismuth (Bi) while maintaining the ABX3 crystal structure. This substitution maintains the perovskite's ability to absorb light and convert it to electricity while eliminating the toxicity issue, thus resolving the contradiction between efficiency and environmental safety

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent employs composite material structures by combining perovskite layers with other semiconductor materials in tandem solar cell configurations. This allows the perovskite to handle high-energy photons while the underlying silicon or other semiconductors handle lower-energy photons, achieving high overall efficiency without requiring high lead content, thereby reducing toxicity while maintaining power conversion efficiency

Inventive Principle:
Principle #40Composite materials

2Reliability

If silicon wafer-based technologies are used to ensure stability, then reliability is improved, but manufacturing cost increases

Engineering Contradiction:
Improvelong-term stabilityVSAvoidmanufacturing cost
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent replaces expensive, energy-intensive silicon wafer manufacturing with cheaper thin-film deposition techniques. By using solution-processing methods, vapor deposition, or spray coating to create thin perovskite films on flexible substrates, the manufacturing cost is dramatically reduced while the resulting devices achieve comparable or superior stability through optimized film structures and encapsulation

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent changes the manufacturing parameters from high-temperature, high-vacuum silicon wafer processes to low-temperature, atmospheric-pressure thin-film deposition. This allows production on flexible, inexpensive substrates like plastic or thin glass, reducing material costs and energy consumption while maintaining device reliability through careful control of film quality and encapsulation

Inventive Principle:
Principle #35Parameter changes

3Power

If perovskite films are made highly reactive to improve light absorption, then power conversion efficiency is improved, but stability deteriorates

Engineering Contradiction:
Improvelight conversion efficiencyVSAvoidfilm stability
Core Design Contradiction:
PowerVSStability of the object's composition

Solution Approach 1:

The patent introduces intermediary layers between the perovskite active layer and the surrounding environment (electrodes, encapsulation, moisture barriers). These intermediary transport layers and encapsulation structures protect the highly reactive perovskite from degradation by water, oxygen, and electrical stress, thereby maintaining both high light absorption efficiency and long-term compositional stability

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent optimizes the chemical composition parameters of perovskite films by adjusting the ratio of organic to inorganic components, selecting specific halide compositions (iodide, bromide, chloride), and controlling crystallization conditions. These parameter changes enhance the inherent stability of the perovskite structure while preserving its light-absorbing properties, reducing reactivity without sacrificing efficiency

Inventive Principle:
Principle #35Parameter changes

4Power

If complex silicon semiconductor connections are used to achieve efficient energy transfer, then power conversion efficiency is improved, but device complexity increases

Engineering Contradiction:
Improveenergy transfer efficiencyVSAvoidconnection complexity
Core Design Contradiction:
PowerVSDevice complexity

Solution Approach 1:

The patent extracts and eliminates the complex silicon semiconductor connection structures by using simple, direct contact between perovskite layers and electrode materials. The perovskite's own charge transport properties and simple layer-by-layer structure replace the need for complex silicon junctions, achieving efficient energy transfer through material selection rather than structural complexity

Inventive Principle:
Principle #2Taking out (Extraction)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enables high-efficiency solar cells with improved stability, reduced toxicity, and lower production costs, potentially achieving efficiencies up to 40-45% and simplifying the manufacturing process by using lower temperatures and less expensive substrates, thus addressing the limitations of traditional silicon wafer-based technologies.

Implementation Method 1

utilizing a eutectic alloy and oxidized metal layers to create a tunnel recombination junction

Methodology Applied
Scientific EffectEutectic alloy: Fusible Alloy

Implementation Method 2

tin-based perovskite/silicon thin-film tandem solar cell structure... facilitating efficient energy transfer

Methodology Applied
Scientific EffectPhotovoltaic effect: Photovoltaic Effect

Data Source

PatentUS9818964B2Method of growing III-V semiconductor films for tandem solar cells
Publication Date: 2017.11.14 SOLAR TECTIC LLC

AI summary

A method of growing a III-V semiconductor compound film for a semiconductor device including the steps of depositing a textured oxide buffer layer on an inexpensive substrate, depositing a metal-inorganic film from a eutectic alloy on the buffer layer, the metal being a component of a III-V compound and forming a layer on the inorganic film on which additional elements from the III-V compound are added, forming a top layer of a tandem solar cell.