Titanium Composite Electrode Resistance Variation

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Solution Overview

Problem

Lithium titanium oxide-based negative electrodes in lithium secondary batteries face intrinsic resistance differences due to structural features, leading to varying resistance values and complexity in battery management system prediction algorithms, especially in high-output applications like automotive batteries.

Innovation Solution

A titanium-based composite is developed by doping or coating lithium titanium oxide with specific metal elements like Zr and Nb, and aluminum, optimizing the crystal plane development to achieve consistent resistance values across different SOC settings and charging rates.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Speed

If lithium titanium oxide is used as negative electrode material to achieve high operating voltage and fast charging/discharging, then charging speed and safety are improved, but reversible capacity is reduced and initial efficiency is lowered

Engineering Contradiction:
Improvecharging speedVSAvoidreversible capacity
Core Design Contradiction:
SpeedVSQuantity of substance

Solution Approach 1:

The patent modifies the crystal structure parameters of lithium titanium oxide by controlling particle size (50-200 nm range) and crystal plane orientation ((400) plane development), which changes the material's electrochemical properties to achieve both fast charging capability and improved capacity

Inventive Principle:
Principle #35Parameter changes

2Speed

If lithium titanium oxide particles are miniaturized to enlarge active surfaces and accelerate lithium diffusion, then charging speed is improved, but manufacturing complexity increases

Engineering Contradiction:
Improvelithium diffusion rateVSAvoidparticle size control complexity
Core Design Contradiction:
SpeedVSDevice complexity

Solution Approach 1:

The patent specifies precise particle size parameters (50-200 nm) and crystal plane ratios ((400)/(111) ≥ 0.76) to optimize lithium diffusion while maintaining manufacturability through controlled synthesis conditions

Inventive Principle:
Principle #35Parameter changes

3Device complexity

If intrinsic resistance differences in lithium titanium oxide are not addressed, then structural simplicity is maintained, but battery management system complexity increases and output characteristics deteriorate

Engineering Contradiction:
Improvestructural complexityVSAvoidbattery management system complexity
Core Design Contradiction:
Device complexityVSEase of operation

Solution Approach 1:

The patent optimizes crystal plane orientation parameters ((400) plane dominance with ratio ≥ 0.76) to minimize resistance variations during charge/discharge cycles, which simplifies battery management and improves output characteristics

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The titanium-based composite ensures a small resistance change rate, simplifies battery management system prediction algorithms, and enhances output characteristics by maintaining low and consistent resistance values, making it suitable for high-output applications.

Implementation Method 1

a titanium-based composite which is doped with M1 and coated with Al

Methodology Applied
Scientific EffectDoping: Dopants

Implementation Method 2

a titanium-based composite which is doped with M1 and coated with Al

Methodology Applied
Scientific EffectCoating: Coatings

Implementation Method 3

a ratio of a peak area of a plane (400) and a peak area of a plane (111) of 0.76 or more in a measured X-ray diffraction spectrum

Methodology Applied
Scientific EffectX-ray diffraction: X-Ray

Data Source

PatentEP3386012B1Negative electrode active material including titanium-based composite, method of preparing the same and lithium secondary battery including the same
Publication Date: 2020.03.04 LG CHEM LTD
  • EP3386012B1 patent drawingFigure 1~2
  • EP3386012B1 patent drawingFigure 3

AI summary

The present invention provides a lithium secondary battery, including a positive electrode including a positive electrode active material, a negative electrode including a negative electrode active material, and a separator provided between the positive electrode and the negative electrode, wherein the negative electrode active material may include a titanium-based composite, wherein, when the lithium secondary battery is charged to SOC 50 under C-rate conditions of 0.1 to 40 C, the titanium-based composite has a ratio of the peak area of a plane (400) and the peak area of a plane (111) of 0.76 or more in a measured X-ray diffraction spectrum (XRD). Therefore, the present invention may provide a lithium secondary battery having excellent output characteristics and a battery pack in which a BMS prediction algorithm is simplified.