Titanium Oxide Composite Particles UV Stability

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Solution Overview

Problem

Existing coatings containing titanium oxide for fluororesin films and outdoor articles suffer from discoloration, decomposition, and photocatalysis due to ultraviolet rays, leading to changes in visible light reflectance and mechanical strength deterioration, with insufficient durability against hydrogen fluoride.

Innovation Solution

Composite particles with a three-layer structure, comprising a titanium oxide core, a silicon oxide intermediate layer, and a cerium oxide outer layer, are used to form a coating layer, which reduces photocatalysis and enhances durability against hydrogen fluoride, maintaining the inherent color and mechanical strength of the coating.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Illumination intensity

If a coating layer containing titanium oxide pigment is formed on fluororesin film to reflect visible light, then visible light transmittance is suppressed, but titanium oxide undergoes discoloration and decomposition by ultraviolet rays causing the coating layer to change color and lose mechanical strength

Engineering Contradiction:
Improvevisible light transmittanceVSAvoiddurability of coating layer
Core Design Contradiction:
Illumination intensityVSReliability

Solution Approach 1:

The invention uses a composite particle structure consisting of a titanium oxide core surrounded by a silica shell. This composite structure combines the high reflectance property of titanium oxide with the UV resistance and chemical stability of silica, allowing the coating to maintain both visible light reflection and long-term durability under outdoor exposure.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The silica layer acts as an intermediary protective barrier between the titanium oxide pigment and the harmful ultraviolet rays. This intermediate layer absorbs or scatters UV radiation before it can reach the titanium oxide core, preventing photocatalytic degradation while allowing the titanium oxide to maintain its light-reflecting function.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Illumination intensity

If titanium oxide is used as white pigment in coating layer, then visible light reflectance is improved, but photocatalysis by ultraviolet rays causes discoloration and mechanical strength deterioration of fluororesin film

Engineering Contradiction:
Improvevisible light reflectanceVSAvoidphotocatalysis damage to fluororesin film
Core Design Contradiction:
Illumination intensityVSObject-affected harmful factors

Solution Approach 1:

The composite particle structure of titanium oxide core with silica shell creates a material that combines the beneficial optical properties of titanium oxide with the protective properties of silica, eliminating the harmful photocatalytic effects on the fluororesin substrate.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The silica layer serves as a protective intermediary that blocks ultraviolet rays from reaching the fluororesin film, thereby preventing photocatalytic degradation of the substrate while allowing the titanium oxide core to provide visible light reflection.

Inventive Principle:
Principle #24Intermediary (Mediator)

3Illumination intensity

If titanium oxide undergoes photocatalysis by ultraviolet rays, then hydrogen fluoride is formed which causes color fading of pigments in coating layer

Engineering Contradiction:
Improvevisible light reflectanceVSAvoidcolor fading of pigments
Core Design Contradiction:
Illumination intensityVSLoss of substance

Solution Approach 1:

The silica layer acts as a protective barrier that prevents the formation of hydrogen fluoride by blocking UV-induced photocatalysis of titanium oxide. This intermediate protection layer preserves the color stability of all pigments in the coating by eliminating the source of HF that would otherwise cause color fading.

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composite particles effectively prevent discoloration, decomposition, and photocatalysis of titanium oxide, ensuring stable visible light reflectance and mechanical strength over a long period, even under outdoor exposure, while maintaining the coating's inherent color and adhesion.

Implementation Method 1

a method of reflecting the visible light, a method of absorbing the visible light, etc. may be mentioned

Methodology Applied
Scientific EffectLight reflection: Reflection

Implementation Method 2

a pigment having cerium oxide and dense amorphous silica precipitated on the surface of rutile-type titanium oxide

Methodology Applied
Scientific EffectUltraviolet absorption: Absorption (EM radiation)

Implementation Method 3

By photocatalysis of titanium oxide by ultraviolet rays, the fluororesin film and the coating layer are likely to undergo discoloration

Methodology Applied
Scientific EffectPhotocatalysis inhibition: Catalysis

Data Source

PatentEP2460766B1Composite particle, composition for forming coating membrane, printing ink, coating material composition, coated article, and resin film with attached coating membrane
Publication Date: 2014.04.30 AGC INC
  • EP2460766B1 patent drawingFigure 1~2
  • EP2460766B1 patent drawingFigure 3
  • EP2460766B1 patent drawingFigure 4

AI summary

Composite particles capable of constantly and highly preventing discoloration, decomposition and photocatalysis by ultraviolet rays despite containing titanium oxide; and a composition for forming a coating layer to be used as a coating material composition, particularly as a printing ink, and a coated article, employing such composite particles. Composite particles characterized in that each of them comprises, in order from the inside, a particle containing titanium oxide, a first covering layer containing silicon oxide, a second covering layer containing cerium oxide and a third covering layer containing silicon oxide, and their average particle size is from 0.15 to 3 µm. A composition for forming a coating layer and a coated article, employing the composite particles.