Toner Formulation Using Polyester Resins for Thermal Stability

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Solution Overview

Problem

Conventional toners face a trade-off between low-temperature fixing property and heat-resistant storage stability, with combinations of non-crystalline and crystalline polyester resins leading to degradation in thermal properties and increased oligomer components that cause adhesion issues during manufacturing.

Innovation Solution

A toner formulation using a non-crystalline polyester resin with a tetrahydrofuran soluble component of specific weight-average molecular weight, combined with a crystalline polyester resin, and a methanol extraction process to control oligomer content, ensuring a glass transition temperature difference of 2.0°C or less, thereby maintaining desired thermal properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Temperature

If the glass transition temperature and melt viscosity are reduced to achieve low-temperature fixing property, then low-temperature fixing property is improved, but heat-resistant storage stability deteriorates

Engineering Contradiction:
Improveglass transition temperatureVSAvoidheat-resistant storage stability
Core Design Contradiction:
TemperatureVSReliability

Solution Approach 1:

The patent applies parameter changes by precisely controlling the weight-average molecular weight of the non-crystalline polyester resin (3,000 to 8,000) and the glass transition temperature (40°C to 60°C) to achieve optimal balance between low-temperature fixing property and heat-resistant storage stability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses composite materials by combining non-crystalline polyester resin and crystalline polyester resin in specific proportions (non-crystalline: 70-90 mass%, crystalline: 10-30 mass%) to achieve both low-temperature fixing and heat-resistant storage stability

Inventive Principle:
Principle #40Composite materials

2Temperature

If a non-crystalline polyester resin and a crystalline polyester resin are used in combination to improve low-temperature fixing property, then low-temperature fixing property is improved, but heat-resistant storage stability deteriorates due to transesterification reaction

Engineering Contradiction:
Improvelow-temperature fixing propertyVSAvoidheat-resistant storage stability
Core Design Contradiction:
TemperatureVSReliability

Solution Approach 1:

The patent controls the composition parameters by limiting the crystalline polyester resin content to 10-30 mass% and specifying the glass transition temperature range (40°C to 60°C) to prevent excessive transesterification while maintaining low-temperature fixing property

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies local quality by using a non-modified polyester resin with specific molecular weight characteristics in the dominant phase (70-90 mass%) to maintain stability, while using a smaller amount of crystalline polyester resin (10-30 mass%) to provide low-temperature fixing enhancement

Inventive Principle:
Principle #3Local quality

3Temperature

If the weight-average molecular weight of non-crystalline polyester resin is reduced to improve low-temperature fixing property, then low-temperature fixing property is improved, but oligomer component increases causing adhesion and granulation problems

Engineering Contradiction:
Improvelow-temperature fixing propertyVSAvoidoligomer component adhesion
Core Design Contradiction:
TemperatureVSObject-generated harmful factors

Solution Approach 1:

The patent precisely controls the weight-average molecular weight parameter within the range of 3,000 to 8,000 to achieve the optimal balance between low-temperature fixing property and minimizing oligomer content that causes adhesion and granulation issues

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent specifies a particular molecular weight range (3,000 to 8,000) that replicates the optimal balance achieved in previous examples, ensuring consistent low-temperature fixing property without excessive oligomer formation

Inventive Principle:
Principle #26Copying

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution achieves superior low-temperature fixing property and heat-resistant storage stability by minimizing oligomer component elution and adhesion, while optimizing glass transition temperature and melt viscosity.

Implementation Method 1

a transesterification reaction occurs during melt-kneading due to similar composition of the resins

Methodology Applied
Scientific EffectTransesterification reaction: Chemical Bonding

Implementation Method 2

when toner particles are dispersed in an aqueous medium during a manufacturing process, the oligomer component eludes into the aqueous medium

Methodology Applied
Scientific EffectElution: Diffusion

Implementation Method 3

the toner has a glass transition temperature A before an extraction process of the toner with methanol and a glass transition temperature B after the extraction process of the toner with methanol, and a difference between A and B (B - A) is 2.0°C or less

Methodology Applied
Scientific EffectGlass transition:

Data Source

PatentEP2783258B1Toner and developer
Publication Date: 2020.07.15 RICOH CO LTD

AI summary

A toner including a non-crystalline polyester resin and a crystalline polyester resin, wherein a tetrahydrofuran soluble component of the non-crystalline polyester resin has a weight-average molecular weight of 3,000 to 8,000 measured by gel permeation chromatography, and wherein the toner has a glass transition temperature A before an extraction process of the toner with methanol and a glass transition temperature B after the extraction process of the toner with methanol, and a difference between A and B (B - A) is 2.0°C or less.