TPS-Polyamide Alloy Compatibilization for Barrier and Flex-Crack Resistance

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Solution Overview

Problem

Thermoplastic starch (TPS) exhibits brittleness and poor mechanical properties, especially when combined with hydrophobic polymers like polyolefins, due to its hydrophilic nature, limiting its application in packaging and other sectors.

Innovation Solution

An alloy of TPS and polyamide with a specific melting point and relative viscosity range is developed, processed using a compounding method in twin-screw extruders, enhancing mechanical properties and barrier resistance.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If thermoplastic starch is combined with hydrophobic polymers like polyolefins, then processability is improved, but mechanical properties deteriorate due to hydrophilic nature causing discontinuous morphology

Engineering Contradiction:
ImproveprocessabilityVSAvoidmechanical properties
Core Design Contradiction:
Ease of manufactureVSStrength

Solution Approach 1:

The patent uses a compatibilizer (such as maleic anhydride grafted polyolefin or starch graft copolymer) as an intermediary substance between the hydrophilic TPS and hydrophobic polymer matrix. This compatibilizer contains both hydrophilic and hydrophobic segments that bridge the two phases, enabling continuous morphology formation and improving mechanical properties while maintaining processability

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent creates a composite material system consisting of TPS, hydrophobic polymer, and compatibilizer. This multi-component composite achieves synergistic effects where the compatibilizer enables proper interfacial adhesion between the hydrophilic and hydrophobic phases, resulting in improved mechanical properties compared to simple blends

Inventive Principle:
Principle #40Composite materials

2Reliability

If thermoplastic starch is used alone, then biodegradability is achieved, but mechanical properties show fragility and water tolerance is poor

Engineering Contradiction:
ImprovebiodegradabilityVSAvoidmechanical properties
Core Design Contradiction:
ReliabilityVSStrength

Solution Approach 1:

The patent creates a composite material system consisting of TPS, hydrophobic polymer, and compatibilizer. This multi-component composite achieves synergistic effects where the compatibilizer enables proper interfacial adhesion between the hydrophilic and hydrophobic phases, resulting in improved mechanical properties compared to simple blends

Inventive Principle:
Principle #40Composite materials

3Strength

If thermoplastic starch is blended with synthetic polymers, then mechanical properties are improved, but processing complexity increases

Engineering Contradiction:
Improvemechanical propertiesVSAvoidprocessing complexity
Core Design Contradiction:
StrengthVSDevice complexity

Solution Approach 1:

The patent applies preliminary action by pre-grafting starch with polyethylene oxide or pre-synthesizing block copolymers before blending. This preliminary modification creates materials with built-in compatibility, reducing the need for complex processing conditions and simplifying the overall manufacturing process while maintaining improved mechanical properties

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The TPS/polyamide alloy demonstrates improved barrier properties, increased softness, and superior breathability, making it suitable for various applications including packaging and agricultural uses.

Implementation Method 1

heating the polyamide, until a temperature between 210-270°C is reached

Methodology Applied
Scientific EffectMelting: Melting

Implementation Method 2

processing using a compounding method in twin-screw extruders, enhancing mechanical properties and barrier resistance

Methodology Applied
Scientific EffectMixing:

Data Source

PatentEP4353780A1Polyamide - thermoplastic starch (TPS) alloys
Publication Date: 2024.04.17 UBE CORP EURO SAU
  • EP4353780A1 patent drawingFigure 1~2
  • EP4353780A1 patent drawingFigure 3~4
  • EP4353780A1 patent drawingFigure 5~6

AI summary

The present invention is directed to a polyamide - thermoplastic starch (TPS) alloy with improved barrier properties, resistances against tear and flex-crack (Gelbo flex testing) higher softness and superior breathability (WVTR). The resulting material shows a rheology and thermal stability that allows to be processed by conventional transformation process such as film, monofilament and tube extrusion, as well as injection. Additionally, the material shows improved biodegradability (lower persistence) under aerobic and anaerobic conditions and reduced CO2 footprint compared with polyamide 6 100% fossil origin. Multiple materials, having multiple uses and applications can be obtained from the alloy.