Transalkylation Process Benzene Purity Control

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Solution Overview

Problem

Current transalkylation processes for producing xylenes and benzene face challenges in achieving high-purity benzene products due to the production of benzene co-boilers, which are difficult to separate and result in catalyst deactivation, especially when processing heavy feeds, leading to reduced catalyst life and purity issues.

Innovation Solution

Implementing benzene-purity-directed operating conditions during the initial process cycle to minimize benzene co-boilers production and then transitioning to standard transalkylation conditions as the catalyst deactivates, allowing for gradual adjustments in temperature, pressure, and hydrogen-to-hydrocarbon ratio to maintain catalyst activity and achieve high-purity benzene production throughout the cycle.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If high activity transalkylation catalysts are used to increase conversion efficiency, then productivity is improved, but benzene co-boilers are produced in higher amounts making purification difficult

Engineering Contradiction:
Improvetransalkylation conversion efficiencyVSAvoidbenzene product purity
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent applies preliminary action by operating at benzene-purity-directed conditions during the initial period of the catalyst cycle, before the catalyst fully deactivates. This early intervention minimizes benzene co-boiler formation when the catalyst is most active, preventing contamination before it occurs. The conditions are then adjusted as the catalyst deactivates to maintain productivity while accepting higher co-boiler formation.

Inventive Principle:
Principle #10Preliminary action

2Productivity

If standard transalkylation conditions are used throughout the process cycle, then productivity is maintained, but benzene purity drops below 99.9% due to co-boiler formation

Engineering Contradiction:
Improvetransalkylation throughputVSAvoidbenzene purity
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent applies dynamics by dynamically adjusting operating conditions based on catalyst age and deactivation state. During the initial high-activity period, benzene-purity-directed conditions are applied to minimize co-boilers. As the catalyst deactivates and activity drops, conditions are transitioned to productivity-directed conditions to maintain throughput. This dynamic adaptation allows both high purity and high productivity to be achieved at different stages of the catalyst cycle.

Inventive Principle:
Principle #15Dynamics

3Manufacturing precision

If benzene-purity-directed conditions are applied during the initial cycle portion, then benzene purity is improved to at least 99.9%, but catalyst deactivation occurs more rapidly

Engineering Contradiction:
Improvebenzene product purityVSAvoidcatalyst life
Core Design Contradiction:
Manufacturing precisionVSDuration of action of stationary object

Solution Approach 1:

The patent applies periodic action by dividing the catalyst operational cycle into distinct periods with different operating conditions. The initial period uses benzene-purity-directed conditions to achieve high purity product while the catalyst is most active. Subsequent periods transition to standard or productivity-directed conditions as the catalyst deactivates. This periodic approach to condition adjustment optimizes both purity and catalyst utilization throughout the cycle.

Inventive Principle:
Principle #19Periodic action

4Productivity

If heavy feeds containing residual components are processed to increase xylene yield, then productivity is improved, but catalyst deactivation accelerates and benzene purity decreases

Engineering Contradiction:
Improvexylene production yieldVSAvoidbenzene purity
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent applies preliminary action by using benzene-purity-directed conditions during the initial high-activity period to prevent co-boiler formation from heavy feed components before they can contaminate the benzene product. This early prevention is particularly important when processing heavy feeds, as the preliminary high-purity operation establishes a clean product stream before catalyst deactivation and increased co-boiler formation occur.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enables the production of benzene with a purity of at least 99.9% by distillation during the initial cycle portion and maintains catalyst activity and longevity, ensuring high-purity benzene production over the entire process cycle while extending catalyst life.

Implementation Method 1

a transalkylation catalyst to contact the aromatic feed to produce the reaction product

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 2

a benzene product stream recovered after distillation to separate the products

Methodology Applied
Scientific EffectDistillation: Distillation

Data Source

PatentEP2755934B1Process for transalkylating aromatic hydrocarbons
Publication Date: 2019.06.19 UOP LLC

AI summary

The present invention is a process for transalkylating aromatic hydrocarbon compounds, the process comprising introducing an aromatic hydrocarbon feed stream into a transalkylation zone to yield high-purity benzene as a byproduct while meeting transalkylation objectives. The feed stream contacts a catalyst in the transalkylation zone under conditions adjusted to control benzene purity as well as transalkylation performance.