Transdermal Preparation Using Acetic Acid-Sodium Acetate Complex

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Solution Overview

Problem

Transdermally absorbable preparations face challenges in maintaining stability and preventing drug crystallization, especially when high concentrations of poorly soluble drugs are used, due to the instability of silicate-based complexes and the volatility of organic acids during solvent removal, leading to reduced skin permeability and bioavailability.

Innovation Solution

A transdermally absorbable preparation comprising a complex of acetic acid and sodium acetate, with a particle diameter of 1-30 µm, and optionally including silicic anhydride, which forms a stable complex that suppresses drug crystallization and enhances skin permeability, characterized by specific X-ray diffraction peaks and a specific surface area of silicic anhydride.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If a drug is blended in a high concentration to an adhesive base to improve transdermal absorbability, then transdermal absorbability is improved, but the drug crystallizes because it has low solubility to the base

Engineering Contradiction:
Improvetransdermal absorbabilityVSAvoiddrug crystallization
Core Design Contradiction:
ReliabilityVSStability of the object's composition

Solution Approach 1:

The patent introduces silicic anhydride as an intermediary substance that mediates between the drug and the adhesive base. The silicic anhydride forms a complex with the organic acid, creating a stable intermediate structure that prevents direct crystallization of the drug from the base while maintaining high drug concentration for improved transdermal absorbability.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent creates a composite material system consisting of silicic anhydride, organic acid, and drug blended in the adhesive base. This composite structure allows the drug to be dispersed in a high concentration without crystallizing, as the silicic anhydride-organic acid complex provides a stable matrix that maintains drug solubility while enabling high drug loading for enhanced transdermal absorption.

Inventive Principle:
Principle #40Composite materials

2Stability of the object's composition

If silicic anhydride is used to suppress crystallization of a drug, then crystallization is suppressed initially, but crystallization gradually proceeds after preparing the preparation due to temperature/humidity effects

Engineering Contradiction:
Improvecrystallization suppressionVSAvoidlong-term stability
Core Design Contradiction:
Stability of the object's compositionVSDuration of action of stationary object

Solution Approach 1:

The organic acid acts as an intermediary that stabilizes the drug-silicic anhydride complex. The organic acid forms hydrogen bonds with both the silicic anhydride and the drug, creating a more robust intermediate structure that is less sensitive to temperature and humidity changes, thereby preventing gradual crystallization over time.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent creates a ternary composite system of silicic anhydride, organic acid, and drug that provides enhanced long-term stability. The synergistic interaction among these three components creates a stable matrix structure that resists crystallization under varying storage conditions, maintaining drug amorphous state and preventing gradual crystallization that occurs with silicic anhydride alone.

Inventive Principle:
Principle #40Composite materials

3Stability of the object's composition

If the amount of organic acid is decreased due to volatility during solvent removal, then the complex formation stability decreases, but the organic acid having a low boiling point volatilizes during the drying process

Engineering Contradiction:
Improvecomplex formation stabilityVSAvoidorganic acid volatilization
Core Design Contradiction:
Stability of the object's compositionVSLoss of substance

Solution Approach 1:

The silicic anhydride acts as a stable intermediary that forms a robust complex with the organic acid. This complex structure protects the organic acid from volatilization during solvent removal, as the strong interaction between silicic anhydride and organic acid reduces the free organic acid available for evaporation, maintaining complex formation stability even with low boiling point acids.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent modifies the physical-chemical parameters of the organic acid by forming a complex with silicic anhydride. This complexation changes the volatility parameter of the organic acid, effectively reducing its vapor pressure and preventing loss during the drying process, while maintaining the necessary amount of organic acid for stable complex formation with the drug.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The preparation effectively suppresses drug crystallization, improves skin permeability, and maintains stability over time, allowing for high concentrations of poorly soluble drugs to be used without aggregation, thereby enhancing transdermal absorption and bioavailability.

Implementation Method 1

a transdermally absorbable preparation comprising a complex of acetic acid and sodium acetate... which forms a stable complex that suppresses drug crystallization

Methodology Applied
Scientific EffectComplex formation:

Implementation Method 2

Transdermally absorbable preparation... enhances skin permeability... enhancing transdermal absorption

Methodology Applied
Scientific EffectTransdermal absorption: Permeation

Implementation Method 3

characterized by specific X-ray diffraction peaks... having peaks at one or more positions from 13.7 ± 0.2°, 22.5 ± 0.2°, 34.9 ± 0.2° (2θ)

Methodology Applied
Scientific EffectX-ray diffraction: X-Ray

Data Source

PatentEP2258396B1Transdermally absorbable preparation
Publication Date: 2017.09.06 HISAMITSU PHARM CO INC
  • EP2258396B1 patent drawingFigure 1~2
  • EP2258396B1 patent drawingFigure 3

AI summary

Disclosed is a transdermally absorbable preparation in which the crystallization of a medicinal agent can be prevented even when the medicinal agent has poor solubility in a base material and is contained in the base material at a high concentration, and which exhibits excellent long-term stability and transdermal absorbability of the medicinal agent. By adding a complex of an organic acid and an organic acid salt and a medicinal agent to a base material, it becomes possible to produce a transdermally absorbable preparation in which the crystallization of the medicinal agent can be prevented and which has excellent preparation properties and transdermal absorbability. Also disclosed is use of a complex of an organic and an organic acid salt for preventing the crystallization of a medicinal agent in a transdermally absorbable preparation.