Transition Metal Complex Catalyst for Ethylene Trimerization

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Solution Overview

Problem

Current industrial processes for producing 1-hexene through ethylene oligomerization, particularly using chromium compounds, are limited by low activity under high pressure and lack selectivity with transition metal compounds other than chromium.

Innovation Solution

Development of novel transition metal complex compounds that form olefin oligomerization catalysts, capable of catalyzing ethylene trimerization to produce 1-hexene with high selectivity and activity, even at lower pressures, by incorporating specific structural elements such as transition metal atoms of Group 3 to Group 10 and specific ligand arrangements.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If chromium compounds are used for ethylene trimerization, then selectivity for 1-hexene is improved, but activity is reduced and high pressure is required

Engineering Contradiction:
Improveselectivity for 1-hexeneVSAvoidactivity
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The patent changes the chemical parameters by replacing chromium compounds with transition metal compounds from groups 3-10 (such as cobalt, iron, nickel, palladium, platinum) combined with specific ligands (beta-diketonates, carboxylates, phosphines, amines). This parameter change enables the catalyst to achieve both high selectivity for 1-hexene and high activity, eliminating the need for high pressure conditions while maintaining excellent trimerization performance.

Inventive Principle:
Principle #35Parameter changes

2Manufacturing precision

If chromium compounds are used for ethylene trimerization, then selectivity for 1-hexene is improved, but operating pressure must be increased to 100 bar

Engineering Contradiction:
Improveselectivity for 1-hexeneVSAvoidoperating pressure
Core Design Contradiction:
Manufacturing precisionVSStress or pressure

Solution Approach 1:

The patent changes the chemical parameters by replacing chromium compounds with transition metal compounds from groups 3-10 (such as cobalt, iron, nickel, palladium, platinum) combined with specific ligands (beta-diketonates, carboxylates, phosphines, amines). This parameter change enables the catalyst to achieve both high selectivity for 1-hexene and high activity, eliminating the need for high pressure conditions while maintaining excellent trimerization performance.

Inventive Principle:
Principle #35Parameter changes

3Quantity of substance

If transition metal compounds other than chromium are used, then cost is reduced, but selectivity for 1-hexene is poor

Engineering Contradiction:
Improvecatalyst costVSAvoidselectivity for 1-hexene
Core Design Contradiction:
Quantity of substanceVSManufacturing precision

Solution Approach 1:

The patent changes the chemical parameters by replacing chromium compounds with transition metal compounds from groups 3-10 (such as cobalt, iron, nickel, palladium, platinum) combined with specific ligands (beta-diketonates, carboxylates, phosphines, amines). This parameter change enables the catalyst to achieve both high selectivity for 1-hexene and high activity, eliminating the need for high pressure conditions while maintaining excellent trimerization performance.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates composite catalyst systems by combining transition metal compounds with specific organic ligands (beta-diketonates, carboxylates, phosphines, amines). This composite approach allows the use of abundant and cost-effective transition metals while achieving chromium-level or superior selectivity through the synergistic interaction between the metal center and the carefully designed ligand environment.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The catalysts demonstrate high activity and selectivity in producing 1-hexene, reducing production costs by operating at lower pressures and offering a more efficient alternative to traditional chromium-based methods.

Implementation Method 1

olefin oligomerization catalysts containing a transition metal complex compound with a specific structure show excellent activity and are suited for use in olefin oligomerization. In particular, the catalysts are capable of catalyzing the oligomerization of ethylene as a starting material to afford a trimer of ethylene, i.e., 1-hexene, with high selectivity.

Methodology Applied
Scientific EffectCatalysis: Catalysis

Data Source

PatentEP2174928B1Transition metal complex compound, olefin oligomerization catalyst containing the compound, and method for producing olefin oligomer performed in the presence of the catalyst
Publication Date: 2015.03.11 MITSUI CHEMICALS INC
  • EP2174928B1 patent drawingFigure 1
  • EP2174928B1 patent drawingFigure 2
  • EP2174928B1 patent drawingFigure 3

AI summary

The invention provides transition metal complex compounds, high-activity olefin oligomerization catalysts containing the compounds, and olefin oligomerization processes using the catalysts. A transition metal complex compound [A] according to the invention is represented by Formula (I) or Formula (I') below. An olefin oligomerization catalyst includes the transition metal complex compound [A]. In an olefin oligomerization process of the invention, an olefin is oligomerized in the presence of the catalyst.