Trichlorosilane Reactor Bubble Control and Heat Transfer Tube Wear

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Solution Overview

Problem

The existing apparatus for producing trichlorosilane experiences decreased reaction efficiency due to larger hydrogen chloride gas bubbles at the upper part of the reactor, leading to reduced contact area with metallurgical grade silicon powder, and wear issues on the heat transfer tube from powder collisions.

Innovation Solution

The apparatus incorporates gas flow controlling members in the central space of the reactor to suppress bubble growth, maintaining smaller bubble sizes and increasing contact area, while the heat transfer tube is positioned in an annular space to avoid collisions and wear, with a cylindrical member supporting the tube and a holed guide member facilitating easy assembly and maintenance.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If the heat transfer tube is disposed close to the center of the reactor to obtain fine bubbles of hydrogen chloride gas, then the reaction efficiency is improved, but the metallurgical grade silicon powder collides against the heat transfer tube causing wear

Engineering Contradiction:
Improvereaction efficiencyVSAvoidwear of heat transfer tube
Core Design Contradiction:
ProductivityVSReliability

Solution Approach 1:

The reactor internal space is segmented into a central space and an annular space. Gas flow controlling members are installed in the central space to manage bubble formation, while the heat transfer tube is installed in the annular space to avoid direct collision with silicon powder, thus separating the functions of bubble control and heat transfer while preventing wear on the heat transfer tube.

Inventive Principle:
Principle #1Segmentation

2Productivity

If hydrogen chloride gas is introduced from the bottom of the reactor, then the metallurgical grade silicon powder is fluidized and reaction occurs, but the bubbles become greater at the upper part resulting in decreased contact area and lower reaction efficiency

Engineering Contradiction:
Improvereaction efficiencyVSAvoidcontact area between gas bubbles and silicon powder
Core Design Contradiction:
ProductivityVSArea of stationary object

Solution Approach 1:

Gas flow controlling members are introduced as intermediary elements in the central space of the reactor. These members interact with the ascending hydrogen chloride gas bubbles, controlling their growth and distribution. This mediation prevents excessive bubble enlargement at the upper part of the reactor, maintaining adequate contact area between gas and silicon powder for sustained reaction efficiency.

Inventive Principle:
Principle #24Intermediary (Mediator)

3Speed

If the bubbles of hydrogen chloride gas grow greater, then the gas flow is enhanced, but the contact area with metallurgical grade silicon powder decreases resulting in lower reaction efficiency

Engineering Contradiction:
Improvegas flow velocityVSAvoidreaction efficiency
Core Design Contradiction:
SpeedVSProductivity

Solution Approach 1:

Different regions of the reactor are given different functional qualities. The central space contains gas flow controlling members that regulate bubble characteristics, while the annular space provides a wear-free zone for the heat transfer tube. This local differentiation allows the system to maintain optimal gas flow velocity in the central region while protecting the heat transfer components in the annular region from wear.

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This configuration enhances reaction efficiency by maintaining a larger contact area between hydrogen chloride gas and metallurgical grade silicon powder, reduces wear on the heat transfer tube, and minimizes corrosion, thereby improving the durability and performance of the reactor.

Implementation Method 1

metallurgical grade silicon powder is fluidized at the lower part of the reactor by ascending hydrogen chloride gas which is introduced from therebelow

Methodology Applied
Scientific EffectFluidization: Fluidisation

Implementation Method 2

the metallurgical grade silicon powder is contacted with the hydrogen chloride gas to cause a reaction during fluidization

Methodology Applied
Scientific EffectChemical reaction: Chemical Bonding

Implementation Method 3

a heat transfer tube through which a heating medium flows in the vertical direction is provided inside the reactor

Methodology Applied
Scientific EffectHeat conduction: Conduction (thermal)

Data Source

PatentEP2210661B1Apparatus and method for producing trichlorosilane
Publication Date: 2019.11.20 MITSUBISHI MATERIALS CORP
  • EP2210661B1 patent drawingFigure 1
  • EP2210661B1 patent drawingFigure 2A~2B
  • EP2210661B1 patent drawingFigure 3~4

AI summary

An apparatus for producing trichlorosilane in which metallurgical grade silicon powder supplied to a reactor is reacted with hydrogen chloride gas while being fluidized by the hydrogen chloride gas, thereby discharging trichlorosilane generated by the reaction from the reactor, includes: a plurality of gas flow controlling members which are installed along a vertical direction in an annular shape R from an inner peripheral wall of the reactor in an internal space of the reactor; and a heat transfer tube which is installed along the vertical direction in the annular space R and through which a heating medium passes.