Trivalent Chromium Passivation Layer for Steel Sheet Corrosion Resistance

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Solution Overview

Problem

Existing electrolytic coating processes for steel sheets use chromium(VI)-containing electrolytes, which are environmentally and health-hazardous, necessitating a replacement to meet future regulatory bans and achieve high chromium oxide content for corrosion resistance and adhesion in packaging applications.

Innovation Solution

An electrolytic process using a trivalent chromium compound-based electrolyte solution without chromium(VI), employing a conductivity-increasing salt and acid or base to set pH, and an anode that prevents chromium(VI) formation, resulting in a passivation layer composed predominantly of chromium oxide and/or chromium hydroxide for efficient and environmentally friendly surface passivation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If chromium(VI)-containing electrolytes are used for electrolytic coating, then good adhesion and corrosion resistance are achieved, but environmental and health hazards increase

Engineering Contradiction:
Improvecorrosion resistanceVSAvoidenvironmental and health hazards
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the chemical composition parameters of the electrolyte by replacing chromium(VI) compounds with chromium(III) compounds. This parameter change eliminates the environmental and health hazards associated with chromium(VI) while maintaining the electrolytic deposition process to achieve chromium oxide passivation layers with good corrosion resistance on steel sheets

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent converts the traditionally harmful chromium(VI) electrolyte system into a beneficial chromium(III) system. By using chromium(III) sulfate as the electrolyte, the process eliminates toxicity while still producing chromium oxide passivation layers that provide corrosion protection, thus converting a harmful process into a beneficial one

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

2Reliability

If chromium(VI)-containing electrolytes are used, then passivation layer with good adhesion is obtained, but regulatory compliance deteriorates

Engineering Contradiction:
Improveadhesion for organic coatingsVSAvoidregulatory compliance
Core Design Contradiction:
ReliabilityVSAdaptability or versatility

Solution Approach 1:

The patent changes the electrolyte composition from chromium(VI) to chromium(III) compounds, which eliminates regulatory compliance issues while maintaining the ability to produce passivation layers with good adhesion for organic coatings through electrolytic deposition

Inventive Principle:
Principle #35Parameter changes

3Quantity of substance

If conventional electrolytic coating processes are used, then chromium-containing passivation layer is deposited, but chromium oxide content remains limited

Engineering Contradiction:
Improvechromium oxide contentVSAvoidprocess complexity
Core Design Contradiction:
Quantity of substanceVSEase of manufacture

Solution Approach 1:

The patent optimizes electrolyte parameters including using chromium(III) sulfate at concentrations of 20-100 g/L, maintaining pH 1-3 with sulfuric acid, and controlling temperature at 20-60°C to achieve high chromium oxide content (over 90%) in the passivation layer through electrolytic deposition

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent employs a two-stage electrolytic process: first a chromium(III) sulfate electrolyte stage to deposit chromium oxide, followed by a rinse and optional second electrolyte stage. This periodic action allows control over chromium oxide content and layer composition

Inventive Principle:
Principle #19Periodic action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process achieves a passivation layer with over 90% chromium oxide content, providing superior oxidation resistance and adhesion for organic coatings, while being completely free of chromium(VI), ensuring compliance with environmental and health regulations.

Implementation Method 1

the steel sheet is passed through a single electrolyte solution in a strip coating line at high strip speeds of more than 100 m/min, acting as the cathode

Methodology Applied
Scientific EffectElectrolysis: Electrolysis

Implementation Method 2

electrolytic deposition of a chromium metal-chromium oxide (Cr-CrOx) layer

Methodology Applied
Scientific EffectElectrodeposition: Electrodeposition

Implementation Method 3

This electrolyte solution contains a trivalent chromium compound (Cr(III)), a complexing agent, and a conductivity-enhancing salt

Methodology Applied
Scientific EffectComplexation:

Implementation Method 4

a conductivity-enhancing salt

Methodology Applied
Scientific EffectElectrical conduction: Conduction (electrical)

Data Source

PatentEP3722464A1Method for passivating the surface of a black plate or a tin plate and electrolysis system for carrying out the method
Publication Date: 2020.10.14 THYSSENKRUPP RASSELSTEIN
  • EP3722464A1 patent drawingFigure 1
  • EP3722464A1 patent drawingFigure 2
  • EP3722464A1 patent drawingFigure 3

AI summary

The invention relates to a method for passivating the surface of a black sheet or a tinplate by electrolytic deposition of a chromium oxide-containing passivation layer on the surface, wherein the electrolytic deposition of the chromium-containing passivation layer is carried out from an electrolyte solution (E) which contains a trivalent chromium compound as well as at least one salt to increase conductivity and at least one acid or base to adjust a desired pH value, wherein the electrolyte solution (E) contains no further components other than the trivalent chromium compound as well as the at least one salt and the at least one acid or base and is in particular free of organic complexing agents and free of buffering agents.