Tungsten-CFC Joined Material With Gradient Sintered Interface

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Solution Overview

Problem

The challenge lies in effectively joining high-melting point metals like tungsten with carbon materials due to poor wettability and thermal expansion differences, leading to stress concentration and difficulty in forming thick layers, which affects the durability and heat conduction of the joined material.

Innovation Solution

A joined material is created by sintering a ceramic layer with a sintering aid agent on a carbon material layer, followed by a tungsten layer, ensuring a strong anchoring effect and high heat conduction, with the ceramic layer thickness ranging from 10 µm to 500 µm to balance strength and thermal stress, and using SiC or AlN as ceramics to enhance the bonding mechanism.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If a high-melting point metal material is joined to a carbon material using a brazing material, then the joining process becomes feasible, but the metal has poor wettability with the metal making it difficult to join

Engineering Contradiction:
Improvejoining process feasibilityVSAvoidjoining quality
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent introduces a gradient intermediate layer between the carbon material and high-melting point metal. This intermediate layer has a composition that gradually transitions from carbon-rich near the carbon material to metal-rich near the high-melting point metal, improving wettability and bonding strength while eliminating the direct interface between incompatible materials.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent employs plasma treatment to modify the surface properties of the high-melting point metal before joining. By changing the surface parameters (surface energy, roughness, chemical composition) through plasma exposure, the metal achieves better wettability with the brazing material and improved bonding to the carbon material.

Inventive Principle:
Principle #35Parameter changes

2Temperature

If a high-melting point metal material is joined to a carbon material, then the thermal expansion rate difference causes stress concentration, but the resulting material becomes easier to break

Engineering Contradiction:
Improvehigh temperature resistanceVSAvoidresistance to breakage
Core Design Contradiction:
TemperatureVSStrength

Solution Approach 1:

The patent creates a gradient intermediate layer with locally varying composition and properties. Near the carbon material, the layer has properties matching carbon (lower thermal expansion, higher thermal conductivity), while near the metal, it transitions to match metal properties. This local adaptation of material properties reduces stress concentration at the interface.

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The patent uses a composite gradient structure combining carbon-containing compounds, metal compounds, and metal phases in varying proportions. This composite approach allows the intermediate layer to exhibit intermediate thermal expansion properties between carbon and metal, reducing thermal stress while maintaining structural integrity.

Inventive Principle:
Principle #40Composite materials

3Quantity of substance

If a tungsten layer is formed on a carbon material by CVD or PVD, then a metal layer is achieved, but the maximum thickness is limited to several hundred micrometers

Engineering Contradiction:
Improvemetal layer thicknessVSAvoidlayer formation capability
Core Design Contradiction:
Quantity of substanceVSEase of manufacture

Solution Approach 1:

The patent applies preliminary surface treatment and intermediate layer formation before depositing the tungsten layer. By preparing the surface with a gradient intermediate structure first, the subsequent tungsten deposition can proceed more effectively, allowing for thicker layers without compromising adhesion or quality.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The gradient intermediate layer serves as a mediator that enables thicker tungsten layer formation. The intermediate layer provides a progressive transition zone that supports the weight and stress of thicker metal deposits, allowing the tungsten layer to exceed the conventional several hundred micrometer limit while maintaining bonding integrity.

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution enables robust joining of tungsten and carbon fiber composite materials, improving flexural strength and heat conduction, while preventing peeling and cracking, and maintaining structural integrity under high temperatures, suitable for applications like nuclear fusion reactors.

Implementation Method 1

a joined material is created by sintering a ceramic layer with a sintering aid agent on a carbon material layer

Methodology Applied
Scientific EffectSintering: Sintering

Data Source

PatentEP2952496B1Joined material and method for producing same
Publication Date: 2024.04.10 TOYO TANSO KK
  • EP2952496B1 patent drawingFigure 1(a)~3(b)
  • EP2952496B1 patent drawingFigure 4(a)~4(b)
  • EP2952496B1 patent drawingFigure 5

AI summary

A joined material and a method of manufacturing the joined material are provided which enable a metal layer and a carbon material layer to be easily joined to each other while making the thickness of the metal layer larger and which can inhibit failure. A joined material includes a CFC layer (3) and a tungsten layer (4) that are joined to each other. A sintered tungsten carbide layer (5), a mixed layer (6) of SiC and WC, and SiC and WC (7) that have been sintered while intruding into the CFC layer (3), are formed between the CFC layer (3) and the tungsten layer (4), and these layers (3, 4, 5, 6, and 7) are joined to each other by sintering.