Tungsten CMP Slurry pH Control for Oxide Erosion

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Solution Overview

Problem

Current chemical mechanical polishing (CMP) slurries for tungsten in semiconductor manufacturing face challenges in minimizing erosion while maintaining a desirable removal rate, particularly for tungsten lines and arrays of metal lines, which can lead to dishing and erosion issues affecting device performance.

Innovation Solution

The development of CMP slurries comprising abrasive particles, oxidizing agents, and erosion-reducing agents with a pH range of 2 to 14, specifically designed to stabilize the pH between 4 and 12 after the addition of tungsten, incorporating additives such as polyacrylic acid and citric acid to maintain a pH greater than 4, thereby reducing oxide erosion and enhancing tungsten removal rates.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If conventional CMP slurries are used for tungsten polishing, then tungsten removal rate is achieved, but oxide erosion and dishing occur

Engineering Contradiction:
Improvetungsten removal rateVSAvoidoxide erosion
Core Design Contradiction:
ProductivityVSObject-affected harmful factors

Solution Approach 1:

The patent applies parameter changes by carefully controlling the pH of the slurry to be greater than 4, which fundamentally alters the chemical environment during polishing. This pH control modifies the reactivity of the slurry components, reducing oxide erosion while preserving effective tungsten removal. The specific pH parameter adjustment transforms the harmful chemical interactions into a more selective process.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent introduces an intermediary approach by using a slurry composition that mediates between the abrasive action needed for tungsten removal and the chemical reactivity that causes oxide erosion. The slurry acts as an intermediary medium that enables mechanical removal while suppressing harmful chemical etching of the dielectric oxide layer.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Productivity

If aggressive polishing is used to increase removal rate, then productivity improves, but dishing and erosion worsen

Engineering Contradiction:
Improveremoval rateVSAvoidplanarity
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent uses parameter changes by adjusting the slurry pH to greater than 4, which modifies the polishing mechanics and chemistry. This parameter adjustment enables effective material removal while suppressing the dishing effect, maintaining planarity even at higher removal rates. The pH parameter acts as a control variable that decouples removal rate from dishing.

Inventive Principle:
Principle #35Parameter changes

3Productivity

If pH is not controlled, then slurry is more reactive for removal, but oxide erosion increases

Engineering Contradiction:
Improvetungsten removal efficiencyVSAvoiddielectric erosion
Core Design Contradiction:
ProductivityVSObject-affected harmful factors

Solution Approach 1:

The patent directly applies parameter changes by controlling the pH to be greater than 4, which fundamentally changes the chemical reactivity profile of the slurry. This pH control creates a more selective chemical environment that favors tungsten removal over oxide erosion, effectively decoupling these two processes through chemical parameter management.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The proposed CMP slurries effectively reduce oxide erosion and maintain high tungsten removal rates, achieving low dielectric polish rates and minimizing dishing, thus improving the planarity and reliability of semiconductor devices.

Implementation Method 1

The polishing composition contacts a first material to be polished and a second material and removes the first material at a higher removal rate than the second material

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 2

The CMP slurries comprise abrasive particles, one or more oxidizing agents

Methodology Applied
Scientific EffectAbrasion: Abrasion

Data Source

PatentEP3597711B1Tungsten chemical mechanical polishing for reduced oxide erosion
Publication Date: 2024.08.07 VERSUM MATERIALS US LLC
  • EP3597711B1 patent drawingFigure 1
  • EP3597711B1 patent drawingFigure 2
  • EP3597711B1 patent drawingFigure 3

AI summary

This invention pertains to slurries, methods and systems that can be used in chemical mechanical planarization (CMP) of tungsten containing semiconductor device. Using the CMP slurries with additives to counter lowering of pH by tungsten polishing byproducts and maintain pH 4 or higher, the erosion of dense metal (such as tungsten) structures can be greatly diminished.